ALBERT

Description: Atmospheric flux inversions use observations of atmospheric CO2 to provide anthropogenic and biogenic CO2 flux estimates at a range of spatio-temporal scales. Inversions require prior flux, a forward model and observation errors to estimate posterior fluxes and uncertainties. Here, we investigate the forward transport error and the associated biogenic feedback in an Earth system model (ESM) context. These errors can occur from uncertainty in the initial meteorology, the analysis fields used, or the advection schemes and physical parameterisation of the model. We also explore the spatio-temporal variability and flow-dependent error covariances. We then compare the error with the atmospheric response to uncertainty in the prior anthropogenic emissions. Although transport errors are variable, average total-column CO2 (XCO2) transport errors over anthropogenic emission hotspots (0.1–0.8 ppm) are comparable to, and often exceed, prior monthly anthropogenic flux uncertainties projected onto the same space (0.1–1.4 ppm). Average near-surface transport errors at three sites (Paris, Caltech and Tsukuba) range from 1.7 to 7.2 ppm. The global average XCO2 transport error standard deviation plateaus at ∼0.1 ppm after 2–3 d, after which atmospheric mixing significantly dampens the concentration gradients. Error correlations are found to be highly flow dependent, with XCO2 spatio-temporal correlation length scales ranging from 0 to 700 km and 0 to 260 min. Globally, the average model error caused by the biogenic response to atmospheric meteorological uncertainties is small (

Description: Climate change mitigation efforts require information on the current greenhouse gas atmospheric concentrations and their sources and sinks. Carbon dioxide (CO2) is the most abundant anthropogenic greenhouse gas. Its variability in the atmosphere is modulated by the synergy between weather and CO2 surface fluxes, often referred to as CO2 weather. It is interpreted with the help of global or regional numerical transport models, with horizontal resolutions ranging from a few hundreds of kilometres to a few kilometres. Changes in the model horizontal resolution affect not only atmospheric transport but also the representation of topography and surface CO2 fluxes. This paper assesses the impact of horizontal resolution on the simulated atmospheric CO2 variability with a numerical weather prediction model. The simulations are performed using the Copernicus Atmosphere Monitoring Service (CAMS) CO2 forecasting system at different resolutions from 9 to 80 km and are evaluated using in situ atmospheric surface measurements and atmospheric column-mean observations of CO2, as well as radiosonde and SYNOP observations of the winds. The results indicate that both diurnal and day-to-day variability of atmospheric CO2 are generally better represented at high resolution, as shown by a reduction in the errors in simulated wind and CO2. Mountain stations display the largest improvements at high resolution as they directly benefit from the more realistic orography. In addition, the CO2 spatial gradients are generally improved with increasing resolution for both stations near the surface and those observing the total column, as the overall inter-station error is also reduced in magnitude. However, close to emission hotspots, the high resolution can also lead to a deterioration of the simulation skill, highlighting uncertainties in the high-resolution fluxes that are more diffuse at lower resolutions. We conclude that increasing horizontal resolution matters for modelling CO2 weather because it has the potential to bring together improvements in the surface representation of both winds and CO2 fluxes, as well as an expected reduction in numerical errors of transport. Modelling applications like atmospheric inversion systems to estimate surface fluxes will only be able to benefit fully from upgrades in horizontal resolution if the topography, winds and prior flux distribution are also upgraded accordingly. It is clear from the results that an additional increase in resolution might reduce errors even further. However, the horizontal resolution sensitivity tests indicate that the change in the CO2 and wind modelling error with resolution is not linear, making it difficult to quantify the improvement beyond the tested resolutions. Finally, we show that the high-resolution simulations are useful for the assessment of the small-scale variability of CO2 which cannot be represented in coarser-resolution models. These representativeness errors need to be considered when assimilating in situ data and high-resolution satellite data such as Greenhouse gases Observing Satellite (GOSAT), Orbiting Carbon Observatory-2 (OCO-2), the Chinese Carbon Dioxide Observation Satellite Mission (TanSat) and future missions such as the Geostationary Carbon Observatory (GeoCarb) and the Sentinel satellite constellation for CO2. For these reasons, the high-resolution CO2 simulations provided by the CAMS in real time can be useful to estimate such small-scale variability in real time, as well as providing boundary conditions for regional modelling studies and supporting field experiments.

Description: The Copernicus Atmosphere Monitoring Service (CAMS) reanalysis is the latest global reanalysis dataset of atmospheric composition produced by the European Centre for Medium-Range Weather Forecasts (ECMWF), consisting of three-dimensional time-consistent atmospheric composition fields, including aerosols and chemical species. The dataset currently covers the period 2003–2016 and will be extended in the future by adding 1 year each year. A reanalysis for greenhouse gases is being produced separately. The CAMS reanalysis builds on the experience gained during the production of the earlier Monitoring Atmospheric Composition and Climate (MACC) reanalysis and CAMS interim reanalysis. Satellite retrievals of total column CO; tropospheric column NO2; aerosol optical depth (AOD); and total column, partial column and profile ozone retrievals were assimilated for the CAMS reanalysis with ECMWF's Integrated Forecasting System. The new reanalysis has an increased horizontal resolution of about 80 km and provides more chemical species at a better temporal resolution (3-hourly analysis fields, 3-hourly forecast fields and hourly surface forecast fields) than the previously produced CAMS interim reanalysis. The CAMS reanalysis has smaller biases compared with most of the independent ozone, carbon monoxide, nitrogen dioxide and aerosol optical depth observations used for validation in this paper than the previous two reanalyses and is much improved and more consistent in time, especially compared to the MACC reanalysis. The CAMS reanalysis is a dataset that can be used to compute climatologies, study trends, evaluate models, benchmark other reanalyses or serve as boundary conditions for regional models for past periods.

Description: Accurate and consistent monitoring of anthropogenic combustion is imperative because of its significant health and environmental impacts, especially at city-to-regional scale. Here, we assess the performance of the Copernicus Atmosphere Monitoring Service (CAMS) global prediction system using measurements from aircraft, ground sites, and ships during the Korea-United States Air Quality (KORUS-AQ) field study in May to June 2016. Our evaluation focuses on CAMS CO and CO2 analyses as well as two higher-resolution forecasts (16 and 9 km horizontal resolution) to assess their capability in predicting combustion signatures over east Asia. Our results show a slight overestimation of CAMS CO2 with a mean bias against airborne CO2 measurements of 2.2, 0.7, and 0.3 ppmv for 16 and 9 km CO2 forecasts, and analyses, respectively. The positive CO2 mean bias in the 16 km forecast appears to be consistent across the vertical profile of the measurements. In contrast, we find a moderate underestimation of CAMS CO with an overall bias against airborne CO measurements of −19.2 (16 km), −16.7 (9 km), and −20.7 ppbv (analysis). This negative CO mean bias is mostly seen below 750 hPa for all three forecast/analysis configurations. Despite these biases, CAMS shows a remarkable agreement with observed enhancement ratios of CO with CO2 over the Seoul metropolitan area and over the West (Yellow) Sea, where east Asian outflows were sampled during the study period. More efficient combustion is observed over Seoul (dCO/dCO2=9 ppbv ppmv−1) compared to the West Sea (dCO/dCO2=28 ppbv ppmv−1). This “combustion signature contrast” is consistent with previous studies in these two regions. CAMS captured this difference in enhancement ratios (Seoul: 8–12 ppbv ppmv−1, the West Sea: ∼30 ppbv ppmv−1) regardless of forecast/analysis configurations. The correlation of CAMS CO bias with CO2 bias is relatively high over these two regions (Seoul: 0.64–0.90, the West Sea: ∼0.80) suggesting that the contrast captured by CAMS may be dominated by anthropogenic emission ratios used in CAMS. However, CAMS shows poorer performance in terms of capturing local-to-urban CO and CO2 variability. Along with measurements at ground sites over the Korean Peninsula, CAMS produces too high CO and CO2 concentrations at the surface with steeper vertical gradients (∼0.4 ppmv hPa−1 for CO2 and 3.5 ppbv hPa−1 for CO) in the morning samples than observed (∼0.25 ppmv hPa−1 for CO2 and 1.7 ppbv hPa−1 for CO), suggesting weaker boundary layer mixing in the model. Lastly, we find that the combination of CO analyses (i.e., improved initial condition) and use of finer resolution (9 km vs. 16 km) generally produces better forecasts.

Description: Airborne observations of greenhouse gases are a very useful reference for validation of satellite-based column-averaged dry air mole fraction data. However, since the aircraft data are available only up to about 9–13 km altitude, these profiles do not fully represent the depth of the atmosphere observed by satellites and therefore need to be extended synthetically into the stratosphere. In the near future, observations of CO2 and CH4 made from passenger aircraft are expected to be available through the In-Service Aircraft for a Global Observing System (IAGOS) project. In this study, we analyse three different data sources that are available for the stratospheric extension of aircraft profiles by comparing the error introduced by each of them into the total column and provide recommendations regarding the best approach. First, we analyse CH4 fields from two different models of atmospheric composition – the European Centre for Medium-Range Weather Forecasts (ECMWF) Integrated Forecasting System for Composition (C-IFS) and the TOMCAT/SLIMCAT 3-D chemical transport model. Secondly, we consider scenarios that simulate the effect of using CH4 climatologies such as those based on balloons or satellite limb soundings. Thirdly, we assess the impact of using a priori profiles used in the satellite retrievals for the stratospheric part of the total column. We find that the models considered in this study have a better estimation of the stratospheric CH4 as compared to the climatology-based data and the satellite a priori profiles. Both the C-IFS and TOMCAT models have a bias of about −9 ppb at the locations where tropospheric vertical profiles will be measured by IAGOS. The C-IFS model, however, has a lower random error (6.5 ppb) than TOMCAT (12.8 ppb). These values are well within the minimum desired accuracy and precision of satellite total column XCH4 retrievals (10 and 34 ppb, respectively). In comparison, the a priori profile from the University of Leicester Greenhouse Gases Observing Satellite (GOSAT) Proxy XCH4 retrieval and climatology-based data introduce larger random errors in the total column, being limited in spatial coverage and temporal variability. Furthermore, we find that the bias in the models varies with latitude and season. Therefore, applying appropriate bias correction to the model fields before using them for profile extension is expected to further decrease the error contributed by the stratospheric part of the profile to the total column.

Description: During the African Monsoon Multidisciplinary Analyses (AMMA) program, which included a special observing period that took place over West Africa in 2006, a major effort was devoted to monitor the atmosphere and its water cycle. The radiosonde network was upgraded and enhanced, and GPS receivers deployed. Among all sondes released in the atmosphere, a significant number were Vaisala RS80-A sondes, which revealed a significant dry bias relative to Vaisala RS92 (a maximum of 14% in the lower atmosphere, reaching 20% in the upper levels). This paper makes use of a simple but robust statistical approach to correct the bias. Comparisons against independent GPS data show that the bias is almost removed at night, whereas for daytime conditions, a weak dry bias (5%) still remains. The correction enhances CAPE by a factor of about 4 and, thus, becomes much more in line with expected values over the region.

Description: Tropical Cyclone Gert (1999) experienced an extratropical transition while it merged with an extratropical cyclone upstream. The upstream extratropical cyclone had started to intensify before it merged with the transitioning tropical cyclone, and it continued intensifying afterward (12 hPa in 12 h, according to the Met Office analysis). The question addressed in this paper is the following: what was the impact of the transitioning tropical cyclone on this intensification of the upstream extratropical cyclone? Until now, in the literature, tropical cyclones that experience extratropical transition have been found to have either no impact or a positive impact on the development of extratropical cyclogenesis events. The positive impact involves either a triggering of the development of the extratropical cyclone or simply a contribution to its deepening. However, the case studied here proves to have a negative impact on the developing extratropical cyclone upstream by diminishing its intensification. Forecasts are performed with and without the tropical cyclone in the initial conditions. They show that when Gert is not present in the initial conditions, the peak intensity of the cyclone upstream occurs 9 h earlier and it is 10 hPa deeper than when Gert is present. Thus, Gert acts to weaken the development by contributing to the filling of the extratropical surface low upstream. Quasigeostropic (QG) diagnostics show that the negative impact on the extratropical development is linked to the fact that the transitioning tropical cyclone interacts with a warm front inducing a negative QG vertical velocity over the developing extratropical low upstream. This interpretation is consistent with other contrasting cases in which the transitioning tropical cyclone interacts with a cold front and induces a positive QG vertical velocity over the developing low upstream, thus enhancing its development. The results are also in agreement with idealized experiments in the literature that are aimed at studying the predictability of extratropical storms. These idealized experiments yielded similar results using synoptic-scale and mesoscale vortices as perturbations on warm and cold fronts.

Description: The field experiment of the African Monsoon Multidisciplinary Analysis (AMMA) project during the 2006 wet monsoon season provided an unprecedented amount of radiosonde/dropsonde data over the West African region. This paper explores the usage and impacts of this invaluable dataset in the European Centre for Medium-Range Weather Forecasts analyses and forecasts. These soundings are the only source of data that can provide 3D information on the thermodynamic and dynamic structures of the lower troposphere over continental West Africa. They are particularly important for the Sahel region located between 12° and 20°N, which is characterized by large gradients in temperature and moisture in the lower troposphere. An assimilation experiment comparison between the pre-AMMA and AMMA radiosonde networks shows that the extra AMMA soundings have a significant analysis impact on the low-level temperature over the Sahel and on the structure of the African easterly jet. However, the impacts of the extra AMMA data on the forecast disappear after 24 h. The soundings reveal large model biases in boundary layer temperature over the northern and eastern Sahel, which are consistent with the well-known model biases in cloud, rainfall, and radiation. Large analysis increments in temperature lead to increments in divergence and subsidence, which act to suppress convection. Thus, the analysis increments appear to have an undesirable feedback on the cloud and temperature model biases. The impact of the AMMA soundings on the African easterly jet is to enhance and extend the jet streak to 15°E, that is, toward the eastern part of the Sahel. No observations are assimilated east of 15°E at the level of the African easterly jet to support the jet enhancement farther east. Comparisons with independent atmospheric cloud motion vectors indicate that the African easterly jet in the analysis is too weak over this data-sparse region. This could have implications for the development of African easterly waves in the model forecast. Further experimentation by assimilating atmospheric motion vectors—currently not used—could address this problem.