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Platinum particle size effect on the oxidative dehydrogenation of aqueous ethanol (1996)

Tillaart, J. A. A. ; Kuster, B. F. M. ; Marin, G. B.

Springer

Catalysis letters 36 (1996), S. 31-36

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ISSN: 1572-879X

Keywords: ethanol ; kinetics ; oxidation ; oxydehydrogenation ; platinum ; structure sensitivity

Source: Springer Online Journal Archives 1860-2000

Topics: Chemistry and Pharmacology

Notes: Abstract The effect of the platinum particle size was investigated for the catalytic oxidative dehydrogenation of aqueous ethanol to ethanal at a temperature of 303 K, an ethanol concentration of 260 mol m−3, a partial oxygen pressure 60 kPa, a pH of 9, and an ethanal and ethanoate concentration of 20 mol m−3. A particle size effect on the turnover frequency was observed but only for particle sizes smaller than 2 nm. Hence, the reaction shows a limited structure sensitivity.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1007/BF00807202

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