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  • Sulfur dioxide  (2)
  • Meteorology and Climatology  (1)
  • 1
    Electronic Resource
    Electronic Resource
    Springer
    Journal of atmospheric chemistry 17 (1993), S. 1-13 
    ISSN: 1573-0662
    Keywords: Sulfur dioxide ; dimethyl sulfide ; carbon disulfide ; Pacific troposphere ; volcanic impacts
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Geosciences
    Notes: Abstract Boundary-layer and free-troposphere measurements of sulfur dioxide, dimethyl sulfide, and carbon disulfide were made during transits of the central and southern Pacific Ocean between Hawaii and Australia. Sulfur dioxide was generally less than 100 pptv and highly variable with no correlation with respect to geographic location or altitude. Dimethyl sulfide in the boundary layer had a concentration range of 〈10 to 200 pptv. Highest concentrations of DMS were in the equatorial region of the southern hemisphere although the concentrations were dependent on location and meteorological regime. In the region of the Fiji Islands several boundary layer samples had SO2, DMS, and CS2. In 1989, additional SO2 measurements were made between Hawaii and the equator and to the west of Hawaii downwind of the Kilauea volcano plumes.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Springer
    Journal of atmospheric chemistry 9 (1989), S. 331-346 
    ISSN: 1573-0662
    Keywords: Sulfur dioxide ; arctic ; troposphere ; stratosphere ; vertical distribution
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Geosciences
    Notes: Abstract Determinations of atmospheric sulfur dioxide were made across the North American Aretic using gas chromatography with a detection limit of 25 parts per trillion by volume and a precision of 25% or better. The vertical distribution of sulfur dioxide in the Arctic atmosphere in April, 1986 was highly variable, with concentrations ranging from the detection limit to 15 parts-per-billion by volume (ppbv). While SO2 exceeded 10 ppbv in an exceptional haze layer in the Alaskan Arctic, sulfur dioxide was sometimes in the 1 – 5 ppbv range when the haze was absent. This was particularly true for the Canadian Arctic in the vicinity of Alert. In the lower stratosphere over Ellesmere Island, sulfur dioxide was 0.85 ppbv.
    Type of Medium: Electronic Resource
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  • 3
    Publication Date: 2019-07-10
    Description: We present the results of aerosol forecast during the Aerosol Characterization Experiment (ACE-Asia) field experiment in spring 2001, using the Georgia Tech/Goddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model and the meteorological forecast fields from the Goddard Earth Observing System Data Assimilation System (GEOS DAS). The aerosol model forecast provides direct information on aerosol optical thickness and concentrations, enabling effective flight planning, while feedbacks from measurements constantly evaluate the model, making successful model improvements. We verify the model forecast skill by comparing model predicted total aerosol extinction, dust, sulfate, and SO2 concentrations with those quantities measured by the C-130 aircraft during the ACE-Asia intensive operation period. The GEOS DAS meteorological forecast system shows excellent skills in predicting winds, relative humidity, and temperature for the ACE-Asia experiment area as well as for each individual flight, with skill scores usually above 0.7. The model is also skillful in forecast of pollution aerosols, with most scores above 0.5. The model correctly predicted the dust outbreak events and their trans-Pacific transport, but it constantly missed the high dust concentrations observed in the boundary layer. We attribute this missing dust source to the desertification regions in the Inner Mongolia Province in China, which have developed in recent years but were not included in the model during forecasting. After incorporating the desertification sources, the model is able to reproduce the observed high dust concentrations at low altitudes over the Yellow Sea. Two key elements for a successful aerosol model forecast are correct source locations that determine where the emissions take place, and realistic forecast winds and convection that determine where the aerosols are transported. We demonstrate that our global model can not only account for the large-scale intercontinental transport, but also produce the small-scale spatial and temporal variations that are adequate for aircraft measurements planning.
    Keywords: Meteorology and Climatology
    Format: application/pdf
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