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Partial oxidation of methane to synthesis gas (1990)

Vernon, Patrick D. F. ; Green, Malcolm L. H. ; Cheetham, Anthony K. ; [et al.]

Springer

Catalysis letters 6 (1990), S. 181-186

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ISSN: 1572-879X

Keywords: Metals for catalysis “syngas” ; oxidation ; nickel ; platinum group metals

Source: Springer Online Journal Archives 1860-2000

Topics: Chemistry and Pharmacology

Notes: Abstract Partial oxidation of methane to synthesis gas has been carried out over a number of transition metal catalysts under a range of conditions. It is found that the metals Ni, Ru, Rh, Pd, Ir and Pt, either supported on alumina or present in mixed metal oxide precursors, will bring the system to equilibrium. The yield of CO and H2 improves with increasing temperature in the range 650–1050 K, and decreases with increasing pressure between 1 and 20 atm. An excellent yield (∼92%) is obtained with a 4∶2∶1 N2∶CH4∶O2 ratio at 1050 K and atmospheric pressure, with a space velocity of 4×104 hour−1.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1007/BF00774718

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