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  • 1
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    Buffering of stratospheric circulation by changing amounts of tropical ozone - A Pinatubo case study (1992)
    In:  Other Sources
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    Publication Date: 2011-08-24
    Description: Stratospheric aerosol from Mount Pinatubo heated the tropical lower stratosphere by about 0.3 K/day mainly due to absorption of terrestrial infrared radiation. This heating was dissipated by: (1) an observed increase in stratospheric temperatures, which enhanced the radiation cooling; (2) additional mean upward motion, observed for the aerosol cloud, which led to adiabatic cooling; and (3) reductions in ozone concentrations resulting from enhanced upward motions. Each of these processes operated on a different time scale: maximum temperatures were observed after about 90 days; maximum ozone losses of about -1.5 ppm occurred after 140 days when the enhanced vertical velocities effectively lifted the ozone profile by about 2 km. We believe this shows that ozone plays an important role in buffering vertical motion in the tropical lower stratosphere, and hence the residual Brewer Dobson circulation of the whole stratosphere.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters (ISSN 0094-8276); 19; 19; p. 1927-1930.
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  • 2
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    Condensed nitrate, sulfate, and chloride in Antarctic stratospheric aerosols (1989)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: The 1987 Airborne Antarctic Ozone Experiment, in which the NO3, Cl, and SO4 contents of stratospheric aerosols were estimated, is discussed. The aerosol size and chemical composition measurements were carried out on samples collected during August 17 to September 4, 1987. The data indicate that condensed nitrate is found below a threshold temperature of 193.6 + or - 3.0 K, which is generally found at latitudes exceeding 64 deg S. A negative correlation exists between condensed nitrate and ozone correlation.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 94; 11271-11
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  • 3
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    Denitrification of the polar winter stratosphere - Implications of SAM II cloud formation temperatures (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: The SAM II extinction profiles and the associated temperature profiles are used to determine the amount of denitrification of the winter polar stratospheres. Clear evidence of the denitrification process in the Antarctic data is seen. There are indications in the Arctic data that denitrification mechanisms may be at work there also. At the latitudes observed by the SAM II satellite system, denitrification begins before the formation of extensive ice clouds and may be due to sedimentation of nitric acid particles. However, the possibility of dinitrification by type II PSCs at latitudes not observed by SAM II cannot be excluded.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters, Supplement (ISSN 0094-8276); 17; 441-444
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  • 4
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    Aerosol nucleation in the winter Arctic and Antarctic stratospheres (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: The formation rate of sulfuric-acid-water aerosol particles is calculated as a function of altitude for the conditions of the winter Arctic and Antarctic stratospheres. The theoretical results indicate that sulfate particle formation can occur in the polar winter stratosphere. Conditions for new particle formation are increasingly favorable as the altitude increases between 20 and 30 km because of the decrease in surface area of preexisting particles and increasing sulfuric-acid vapor supply. The theoretical predictions are consistent with observations of a high-altitude CN layer over Antarctica in the spring. Available vapor-pressure data indicate that ternary particles composed of sulfuric acid, nitric acid, and water are not thermodynamically stable under winter stratospheric conditions.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters, Supplement (ISSN 0094-8276); 17; 417-420
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  • 5
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    Airborne lidar observations in the wintertime Arctic stratosphere - Ozone (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Large-scale distributions of ozone (O3) were measured with an airborne lidar system as part of the 1989 Airborne Arctic Stratospheric Expedition. Measurements of O3 distributions were obtained between January 6 and February 15, 1989, on 15 long-range flights into the polar vortex from the Solar Air Station, Norway. The observed O3 distribution was found to clearly indicate the edge of the polar vortex and to be an effective tracer of dynamical processes in the lower stratosphere. On the last two flights of the expedition, large regions with reduced O3 levels were observed by the lidar inside the polar vortex. Ozone had decreased by as much as 17 percent in the center of these areas, and using the in situ measurements made on the ER-2 aircraft, it was concluded that this decline was due to chemical O3 destruction.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters, Supplement (ISSN 0094-8276); 17; 325-328
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  • 6
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    Airborne lidar observations in the wintertime Arctic stratosphere - Polar stratospheric clouds (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Polar stratospheric cloud (PSC) distributions in the wintertime Arctic stratosphere and their optical characteristics were measured with a multiwavelength airborne lidar system as part of the 1989 Airborne Arctic Stratospheric Expedition. PSCs were observed on 10 flights between January 6 and February 2, 1989, into the polar vortex. The PSCs were found in the 14-27 km altitude range in regions where the temperatures were less than 195 K. Two types of aerosols with different optical characteristics (Types 1a and 1b) were observed in PSCs thought to be composed of nitric acid trihydrate. Water ice PSCs (Type 2) were observed to have high scattering ratios (greater than 10) and high aerosol depolarizations (greater than 10 percent) at temperatures less than 190 K.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters, Supplement (ISSN 0094-8276); 17; 385-388
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  • 7
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    Radiative effects of polar stratospheric clouds (1990)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Radiative transfer calculations are performed for polar stratospheric clouds (PSCs) using newly acquired PSC properties and polar atmospheric data. PSC radiative effects depend strongly on upwelling thermal radiation and vary from infrared heating over warm polar surfaces, such as oceans, to cooling over cold surfaces, such as the Antarctic plateau. Heating and cooling rates of nitric acid PSCs are smaller than + or - 0.1 K/day. Rates for optically thicker ice PSCs vary from 1.0 to -0.2 K/day, those for orographically forced ice PSCs even from 3.0 to -0.5 K/day. Frequently observed optically thick cirrus decks near the tropopause provide a very cold radiative surface. These clouds not only act to prevent heating and enhance cooling in ice PSCs to -0.5 K/day and orographic ice PSCs to 2 K/day, but such cirrus cloud decks also cool the entire stratosphere by up to -0.5 K/day over warm surfaces, even in the absence of PSCs.
    Keywords: GEOPHYSICS
    Type: Geophysical Research Letters, Supplement (ISSN 0094-8276); 17; 373-376
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  • 8
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    Antarctic stratospheric ice crystals (1989)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: Ice crystals were replicated over the Palmer Peninsula at approximately 72 deg S on six occasions during the 1987 Airboirne Antarctic Ozone Experiment. The sampling altitude was between 12.5 and 18.5 km (45-65 thousand ft pressure altitude) with the temperature between 190 and 201 K. The atmosphere was subsaturated with respect to ice in all cases. The collected crystals were predominantly solid and hollow columns. The largest crystals were sampled at lower altitudes where the potential temperature was below 400 K. While the crystals were larger than anticipated, their low concentration results in a total surface area that is less than one tenth of the total aerosol surface area. The large ice crystals may play an important role in the observed stratospheric dehydration processes through sedimentation. Evidence of scavenging of submicron particles further suggests that the ice crystals may be effective in the removal of stratospheric chemicals.
    Keywords: GEOPHYSICS
    Type: Journal of Geophysical Research (ISSN 0148-0227); 94; 16449-16
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  • 9
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    A multidimensional model for aerosols - Description of computational analogs (1988)
    In:  Other Sources
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    Publication Date: 2011-08-19
    Description: The numerical algorithms used to simulate the advection, diffusion, sedimentation, coagulation, and condensational growth of atmospheric aerosols are described. The model can be used in one, two, or three spatial dimensions. The continuity equation in a generalized horizontal and vertical coordinate system is developed, which allows the model to be quickly adapted to a wide variety of dynamical models of global or regional scale. Algorithms are developed to treat the various physical processes, and the results of simulations are presented, which show the strengths and weaknesses of these algorithms. Although the emphasis is on the modeling of aerosols, the work is also applicable to the simulations of the transport of gases.
    Keywords: GEOPHYSICS
    Type: Journal of the Atmospheric Sciences (ISSN 0022-4928); 45; 2123-214
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  • 10
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    Particles above the tropopause - Measurements and models of stratospheric aerosols, meteoric debris, nacreous clouds, and noctilucent clouds (1981)
    In:  Other Sources
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    Publication Date: 2011-08-18
    Description: An outline is presented of the present status of knowledge of stratospheric aerosols, meteoric debris, nacreous clouds, and noctilucent clouds. Considerable progress has been made in studies of these particles during the previous decade and it is appropriate to synthesize the information to provide a background for studies planned for the 1980s. Numerical models of the formation, growth, and evolution are considered and a description is given of the physical processes involved, taking into account aspects of nucleation, coagulation, condensational growth, sedimentation, and questions of dynamical transport. A schematic outline of the physical and chemical processes included in a model of stratospheric aerosols is provided.
    Keywords: GEOPHYSICS
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