ALBERT

Description: Trajectory calculations with convective influence diagnosed from geostationary-satellite cloud measurements are used to evaluate the relative importance of different Tropical Tropopause Layer (TTL) transport pathways for establishing the distribution of carbon monoxide (CO) at 100 hPa as observed by the Microwave Limb Sounder (MLS) on board the Aura satellite. Carbon monoxide is a useful tracer for investigating TTL transport and convective influence because the CO lifetime is comparable to the time require for slow ascent through the TTL (a couple of months). Offline calculations of TTL radiative heating are used to determine the vertical motion field. The simple trajectory model does a reasonable job of reproducing the MLS CO distributions during Boreal wintertime and summertime. The broad maximum in CO concentration over the Pacific is primarily a result of the strong radiative heating (indicating upward vertical motion) associated with the abundant TTL cirrus in this region. Sensitivity tests indicate that the distinct CO maximum in the Asian monsoon anticyclone is strongly impacted by extreme convective systems with detrainment of polluted air above 360 K potential temperature. The relative importance of different CO source regions will also be discussed.

Description: Processes maintaining the localized maxima in lower stratospheric watervapor over the boreal summer Asian monsoon region are investigated usingtrajectory and cloud models that resolve the detailed cloudmicrophysical processes, with observation-based convection and radiationschemes. We examine the impact of convective influence along parceltrajectories on cloud formation and dehydration by tracing thetrajectories through time-dependent fields of convective cloud topheights estimated from global rainfall and geostationary brightnesstemperatures. Parameters such as the rainfall threshold used foridentification of deep convection are derived by comparison with theCloudSat deep convective cloud top product as enhanced by colocatedCALIOP measurements. The simulated water vapor field at the 100 hPalevel and cloud occurrence frequencies in the tropical tropopause layer(TTL) are constrained by corresponding observations from MLS andCALIPSO, respectively. The observed maximum in the 100 hPa level watervapor field over the Asian monsoon region is only present in thesimulation with convective influence, indicating the importance ofconvective hydration for the summertime water vapor distribution.Convection moistens the 100 hPa level over the Asian monsoon by 1 ppmv,where 75 of this moistening is due to convection occurring locallywithin the monsoon region. Convection also increases the cloudoccurrence frequency in the TTL over the southern sector of the Asianmonsoon anticyclone by 20. Parcels are convectively hydrated in thesoutheastern sector of the anticyclone, transported westward by theanticyclonic circulation, and dehydrated in the southwestern sector. Therelative importance of extreme convective events that inject ice andwater vapor near or above the tropopause will also be examined.