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  • 1
    Electronic Resource
    Electronic Resource
    On the frequency factor in electron transfer reactions and its role in the highly exothermic regime (1981)
    New York, NY : Wiley-Blackwell
    International Journal of Chemical Kinetics 13 (1981), S. 865-872 
    Details
    ISSN: 0538-8066
    Keywords: Chemistry ; Physical Chemistry
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: Consideration of current information on the dependence of the electron transfer rate on the radial separation distance and on the reactants′ radial distribution function suggests for adiabatic transfers a frequency factor closer to 1012M-1 s-1 than to 1011M-1 s-1. One effect is to raise the λ values estimated from self-exchange rate constants, and to extend thereby the range of ΔG°'s in which the “inverted region′” is masked by a diffusion-controlled reaction rate.
    Additional Material: 1 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/kin.550130910
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