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Mechanism of potassium-catalyzed carbon/CO2 reaction (1986)

Sams, D. A. ; Shadman, Farhang

Hoboken, NJ : Wiley-Blackwell

AIChE Journal 32 (1986), S. 1132-1137

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ISSN: 0001-1541

Keywords: Chemistry ; Chemical Engineering

Source: Wiley InterScience Backfile Collection 1832-2000

Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology

Notes: The mechanism of potassium-catalyzed C/CO2 reaction is studied by a temperature and concentration programmed reaction (TCPR) technique. The proposed redox mechanism contains three surface complexes: -CO2K, -COK, and -CK. The oxide groups are the intermediates during C/CO2 gasification. The completely reduced form, -CK, is the end product of catalyst reduction and is the precursor for K loss. The stoichiometries of these surface groups are confirmed by oxygen and potassium balances.

Additional Material: 6 Ill.

Type of Medium: Electronic Resource

URL: http://dx.doi.org/10.1002/aic.690320710

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