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  • 1
    Publication Date: 2022-05-26
    Description: Author Posting. © American Geophysical Union, 2014. This article is posted here by permission of American Geophysical Union for personal use, not for redistribution. The definitive version was published in Geophysical Research Letters 41 (2014): 961-968, doi:10.1002/2013GL058121.
    Description: Freshwater in the Arctic Ocean plays an important role in the regional ocean circulation, sea ice, and global climate. From salinity observed by a variety of platforms, we are able, for the first time, to estimate a statistically reliable liquid freshwater trend from monthly gridded fields over all upper Arctic Ocean basins. From 1992 to 2012 this trend was 600±300 km3 yr−1. A numerical model agrees very well with the observed freshwater changes. A decrease in salinity made up about two thirds of the freshwater trend and a thickening of the upper layer up to one third. The Arctic Ocean Oscillation index, a measure for the regional wind stress curl, correlated well with our freshwater time series. No clear relation to Arctic Oscillation or Arctic Dipole indices could be found. Following other observational studies, an increased Bering Strait freshwater import to the Arctic Ocean, a decreased Davis Strait export, and enhanced net sea ice melt could have played an important role in the freshwater trend we observed.
    Description: This work was supported by the cooperative project 03F0605E, funded by the German Federal Ministry for Education and Research (BMBF), and by the European Union Sixth Framework Programme project DAMOCLES, contract 018509GOCE.
    Description: 2014-08-12
    Keywords: Arctic ; Liquid freshwater ; Observation ; Model
    Repository Name: Woods Hole Open Access Server
    Type: Article
    Format: application/pdf
    Format: text/plain
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  • 2
    Electronic Resource
    Electronic Resource
    Amsterdam : Elsevier
    Phytochemistry 36 (1994), S. 785-788 
    ISSN: 0031-9422
    Keywords: Cinnamomum philippinense ; Lauraceae ; antioxidative activity. ; antiplatelet aggregation ; cinnamophilin ; lignans ; roots ; vasorelaxing effect
    Source: Elsevier Journal Backfiles on ScienceDirect 1907 - 2002
    Topics: Biology , Chemistry and Pharmacology
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    Hoboken, NJ : Wiley-Blackwell
    AIChE Journal 31 (1985), S. 957-964 
    ISSN: 0001-1541
    Keywords: Chemistry ; Chemical Engineering
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology
    Notes: Six char samples generated from two coals were impregnated by solutions with different concentrations of Na2CO3 and /or K2CO3. The catalyst solution penetration was studied, the catalyst uptake was measured, and the effects of impregnation on the char pore structure were determined experimentally. The results indicate that the impregnated catalysts reside only on particle exteriors without significant penetration. The overall rate of reaction is therfore the combination of catalytic reaction on particle exteriors and noncatalytic reaction on the pore surfaces inside the particle. A kinetic model is presented that takes these findings into account.
    Additional Material: 8 Ill.
    Type of Medium: Electronic Resource
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  • 4
    Electronic Resource
    Electronic Resource
    Hoboken, NJ : Wiley-Blackwell
    AIChE Journal 31 (1985), S. 965-972 
    ISSN: 0001-1541
    Keywords: Chemistry ; Chemical Engineering
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology
    Notes: Oxidation rates of Na2CO3- and K2CO3-impregnated char samples were measured in an isothermal kinetic control regime. The results were analyzed by a previously developed model to extract the intrinsic catalytic reactivities, freed from superimposed noncatalytic and structural effects. Although the overall catalyzed rates are only several times greater than their uncatalyzed counterparts, the intrinsic catalytic rates were found to be four orders of magnitude greater. The results further indicate that the function of the catalyst is to increase the number of active sites without affecting the activation energy. The overall reaction kinetics are demonstrated to contain the combined contributions of both catalytic and noncatalytic reactions, and in this context the effects of multiple catalysts as well as of the pore structure development during reaction can be understood and interpreted.
    Additional Material: 11 Ill.
    Type of Medium: Electronic Resource
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  • 5
    Electronic Resource
    Electronic Resource
    Hoboken, NJ : Wiley-Blackwell
    AIChE Journal 31 (1985), S. 973-981 
    ISSN: 0001-1541
    Keywords: Chemistry ; Chemical Engineering
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology
    Notes: Prior studies have demonstrated that char gasification rates vary with conversion, showing a maximum at an intermediate level. In this work experimentally determined char-air reaction rates and corresponding pore structures are compared to assess the applicability of a previously proposed random pore model and to extract pertinent chemical and physical parameters. Results on six different chars are presented and analyzed to obtain structure parameters, intrinsic kinetics, and activation energies. Agreement between two independent evaluations of the structure parameters demonstrates the degree of applicability of the random pore model and supports the view that rate variations with conversion are controlled by pore structural changes, even though overall rates also include contributions of intrinsic reactivity.
    Additional Material: 17 Ill.
    Type of Medium: Electronic Resource
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  • 6
    Electronic Resource
    Electronic Resource
    Hoboken, NJ : Wiley-Blackwell
    AIChE Journal 31 (1985), S. 1725-1727 
    ISSN: 0001-1541
    Keywords: Chemistry ; Chemical Engineering
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology , Process Engineering, Biotechnology, Nutrition Technology
    Additional Material: 1 Ill.
    Type of Medium: Electronic Resource
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