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  • 73.40  (1)
  • 78.40. - q  (1)
  • 81.20
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  • 1
    Electronic Resource
    Electronic Resource
    Springer
    Applied physics 62 (1996), S. 19-27 
    ISSN: 1432-0630
    Keywords: 42.25.Fx ; 78.20.Dj ; 78.40. - q ; 82.70.Dd
    Source: Springer Online Journal Archives 1860-2000
    Topics: Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Physics
    Notes: Abstract Formation of particle aggregates of arbitrary size and shape by lumping of small particles yields extinction and scattering of light that differ from those of isolated particles. The aggregation process can be followed from extinction and angle-resolved light scattering measurements. Introducing new parameters in angular light scattering, systems containing only isolated clusters were efficiently distinguished from cluster-aggregate systems. This was achieved by evaluation of the measured data in forward and backward scattering direction and at a scattering angle of 90°, resulting in a distinct separation of isolated-cluster systems and cluster-aggregate systems. For measuring the angle-resolved light scattering by noble metal colloidal particle systems, a common photogoniometer setup had to be modified. Changes in scattering and extinction data were qualitatively described by a model that takes into account electromagnetic coupling among clusters in the aggregate.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 12 (1989), S. 505-514 
    ISSN: 1434-6079
    Keywords: 36.40 ; 42.20 ; 78.00 ; 81.20 ; 81.40 ; 82.70
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract First, some general remarks concerning macroscopic “cluster matter” are given. In the second part, three recent, mainly optically and electron-microscopically performed investigations are discussed which deal with special properties of noble metal cluster systems forming the building units of this kind of matter:(1) dressed Au-55 clusters,(2) electromagnetic coupling effects among coagulated clusters,(3) the transition towards compact inhomogeneous matter caused by coalescence of clusters.
    Type of Medium: Electronic Resource
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  • 3
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 26 (1993), S. 242-245 
    ISSN: 1434-6079
    Keywords: 41.70 ; 61.55 ; 73.40 ; 82.70
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Extinction spectra of Agx-Au(1−x)-alloy particles embedded in glass are compared to spectra of gold coated silver clusters and silver coated gold clusters. It is shown, that the optical extinction of alloy particles is described by the Mie theory applying the homogeneous dielectric function $$\hat \varepsilon $$ (ω,R, x) measured by Paquet. The absorption of core-shell clusters was calculated deriving an extension of the Mie theory to spheres with arbitrary numbers of shells of arbitrary materials. Comparison to measured spectra points to s-electron motion in the clusters with only slight scattering at the interior interface. The appearance of two distinct Mie peaks however proves the existence of the sharp Ag-Au interface. The extended Mie formalism was also applied to a multilayer system consisting of sodium and a dielectric substance as an example for a spherical hetero structure.
    Type of Medium: Electronic Resource
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