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  • 61.16  (1)
  • 68,35.Fx  (1)
  • 79.20.Rf  (1)
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  • 1
    Digitale Medien
    Digitale Medien
    Springer
    Applied physics 53 (1991), S. 369-376 
    ISSN: 1432-0630
    Schlagwort(e): 68.55.−a ; 68,35.Fx ; 61.16.Fk
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Maschinenbau , Physik
    Notizen: Abstract The growth of Pt(111) by Pt vapour deposition is studied by He diffraction as a function of substrate temperature and deposition rate. At a deposition rate of about 2.5×10−2 monolayers/second several growth modes are observed: layer-by-layer (2D-) growth at 450 K≲T s≲800 K, multilayer (3D-) growth at 340 K≲T s≲450 K and reentrant layer-by-layer (2D-) growth at T s≲340 K. The observed growth modes and in particular the reentrant 2D-growth are shown to be characteristic of growing Pt(111) under clean conditions, i.e. not influenced by contaminants. The influence of the intra- and interlayer mass transport on the growth mode is discussed in the light of experimental and simulation results. The 3D-growth mode is attributed to the existence of an activation barrier which suppresses the descent of adatoms from the top of the growing adatom islands onto the lower terraces. The barrier can be overcome by thermal adatoms at T s≳450 K enabling interlayer mass transport which leads to 2D-growth. The reentrant 2D-growth occurs due to a break down of this barrier for small, irregularly shaped islands.
    Materialart: Digitale Medien
    Standort Signatur Erwartet Verfügbarkeit
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  • 2
    Digitale Medien
    Digitale Medien
    Springer
    Applied physics 60 (1995), S. 147-153 
    ISSN: 1432-0630
    Schlagwort(e): 68.55 ; 61.16 ; 34.00
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Maschinenbau , Physik
    Notizen: Abstract The adsorption of Xe on Pt(111) has been investigated from the arrival of the very first atoms up to completion of the monolayer using a variable-temperature Scanning Tunneling Microscope (STM). Surprisingly, in the initial stages of the adsorption Xe preferentially binds to a low coordination site, theupper edge of the platinum steps. The strong binding to these sites leads to a local repulsive interaction with further Xe atoms. Therefore, the Xe atoms located at the upper edge of the steps do not serve as nuclei for 2D Xe islands, which, instead, form on the terraces and at thelower edges of the platinum steps. Only during completion of the monolayer do these islands make contact with the atoms adsorbed at the beginning in the upper-edge positions. The full monolayer exhibits the Hexagonal Incommensurate Rotated (HIR) phase already known from earlier helium-diffraction experiments.
    Materialart: Digitale Medien
    Standort Signatur Erwartet Verfügbarkeit
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  • 3
    Digitale Medien
    Digitale Medien
    Springer
    Applied physics 41 (1986), S. 91-93 
    ISSN: 1432-0630
    Schlagwort(e): 68.35.Bs ; 79.20.Rf
    Quelle: Springer Online Journal Archives 1860-2000
    Thema: Maschinenbau , Physik
    Notizen: Abstract The structural analysis of the physisorption system Xe/Pt(111) by means of high-resolution helium diffraction shows that the Xe monolayer exhibits a variety of structural phases: commensurate, incommensurate and “incommensurate” rotated. The observed buckling of the rotated phase demonstrates that a fraction of the Xe atoms is locked in high symmetry sites in agreement with the theoretical “coincident site lattice” concept of Fuselier et al., i.e. the rotated phase is a higher-order commensurate phase.
    Materialart: Digitale Medien
    Standort Signatur Erwartet Verfügbarkeit
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