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  • 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases  (8)
  • 03. Hydrosphere::03.01. General::03.01.01. Analytical and numerical modeling  (3)
  • 1
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    Geochemical monitoring of groundwaters (1998-2001) at Vesuvius volcano (Italy) (2005)
    Elsevier
    Details
    Publication Date: 2017-04-04
    Description: This work presents the results of hydrogeochemical studies carried out at Vesuvius during the period May 1998 - December 2001, mostly focusing on compositional time variations observed during this time. Based on their chemistry, groundwater samples are distinguished into two groups, 1 and 2, representative of water circulation in the southern and northern sectors of the volcano, respectively. Waters from group 1 are typically more acidic, warmer,and more saline than those of group 2. They also have higher CO2 and CH4 contents, attributed to enhanced input of deep-rising volatiles and prolonged water-rock interactions. Time-series highlight the fairly constant chemical composition of the entire aquifer. Groundwater temperature, pH, bicarbonate content and dissolved CO2 display quite stable values in the study period, particularly in deep wells (piezometric level more than 100 m deep). Shallower water bodies present more evident temporal variations, related to seasonal and anthropogenic effects. This paper also describes some important variations in water chemistry which had occurred by the time of the seismic event in early October 1999, particularly in the Olivella spring located on the northern flank of the volcano. At this site, a great decrease in water pH and redox potential, and increased dissolved CO2 contents and 3He/4He ratios were observed. These changes in chemical and isotope composition support the hypothesis of an input of magma-derived helium and carbon dioxide into the aquifer feeding the Olivella spring by the time of the earthquake.
    Description: Published
    Description: 81-104
    Description: partially_open
    Keywords: Vesuvius ; volcanic surveillance ; groundwater ; hydro-geochemistry ; oxygen-18 ; 03. Hydrosphere::03.04. Chemical and biological::03.04.03. Chemistry of waters ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases ; 03. Hydrosphere::03.04. Chemical and biological::03.04.06. Hydrothermal systems ; 04. Solid Earth::04.08. Volcanology::04.08.06. Volcano monitoring
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 2
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    Methane emission from the mud volcanoes of Sicily (Italy) (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: Mud volcanoes represent the largest expression of natural methane release into the atmosphere; however, the gas flux has never been investigated in detail. Methane output from vents and diffuse soil degassing is herewith reported for the first time. Measurements were carried out at 5 mud volcano fields around Sicily (Italy). Each mud volcano is characterized by tens of vents and bubbling pools. In the quiescent phase, methane emission from single vents ranges between 0.01 and 6.8 kg/day. Diffuse soil leakage around the vents is in the order of 102–104 mg m 2 d 1. An exceptional flux of 106 mg m 2 d 1 was recorded close to an everlasting fire. Soil CH4 flux is positive even at large distances from the mud volcano fields suggesting a diffuse microseepage over wider areas. A total of at least 400 tons CH4 per year can be estimated over the area investigated alone ( 1.5 km2).
    Description: Published
    Description: 1215
    Description: partially_open
    Keywords: methane ; flux measurements ; Sicily ; 01. Atmosphere::01.01. Atmosphere::01.01.02. Climate ; 03. Hydrosphere::03.04. Chemical and biological::03.04.02. Carbon cycling ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 3
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    Chemical and isotopic composition of waters and dissolved gases in some thermal springs of sicily and adjacent volcanic islands, Italy. (2007)
    Birkhauser
    Details
    Publication Date: 2017-04-04
    Description: Hydrochemical (major and some minor constituents), stable isotope (dDH2O and d18OH2O; d13CTDIC total dissolved inorganic carbon) and dissolved gas composition have been determined on 33 thermal discharges located throughout Sicily (Italy) and its adjacent islands. On the basis of major ion contents, four main water types have been distinguished: (1) a Na-Cl type; (2) a Ca-Mg〉Na- SO4-Cl type; (3) a Ca-Mg-HCO3 type and (4) a Na-HCO3 type water. Most waters are meteoric in origin or resulting from mixing between meteoric water and heavy-isotope end members. In some samples, d18O values reflect the effects of equilibrium processes between thermal waters and rocks (positive 18O-shift) or thermal waters and CO2 (negative 18O-shift). Dissolved gas composition indicates the occurrence of gas/ water interaction processes in thermal aquifers. N2/O2 ratios higher than air-saturated water (ASW), suggest the presence of geochemical processes responsible for dissolved oxygen consumption. High CO2 contents (more than 3000 cc/litre STP) dissolved in the thermal waters indicate the presence of an external source of carbon dioxide-rich gas. TDIC content and d13CTDIC show very large ranges from 4.6 to 145.3 mmol/Kg and from )10.0& and 2.8&, respectively. Calculated values indicate the significant contribution from a deep source of carbon dioxide inorganic in origin. Interaction with Mediterranean magmatic CO2 characterized by heavier carbon isotope ratios (d13CCO2 value from )3 to 0& vs V-PDB (CAPASSO et al., 1997, GIAMMANCO et al., 1998; INGUAGGIATO et al., 2000) with respect to MORB value and/ or input of CO2-derived from thermal decomposition of marine carbonates have been inferred.
    Description: Published
    Description: 781-807
    Description: JCR Journal
    Description: reserved
    Keywords: Thermal waters, ; chemical and isotope composition, ; dissolved gases ; d13C ; Sicily. ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases ; 03. Hydrosphere::03.04. Chemical and biological::03.04.06. Hydrothermal systems ; 03. Hydrosphere::03.04. Chemical and biological::03.04.07. Radioactivity and isotopes
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 4
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    A simple method to determine the δ13C content of total dissolved inorganic carbon (2005)
    The Mexican Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: A simple method for determining the d13C of TDIC (Total Dissolved Inorganic Carbon) in natural waters was developed and tested. The proposed method is based on chemical and physical stripping of CO2 from water samples. The sampling apparatus consists of a glass bottle (ca 100 ml) totally filled with water sample in the field and sealed by gas-tight rubber/teflon plug. In the laboratory, we introduce 10 ml of pure Ar as host gas into the bottles and draw out an equal volume of water. About 0.5 ml of 37% extra-pure HCl is then injected into the bottle. Water pH decreases to values close to 1 and, therefore, the only carbon species present is CO2 both as dissolved and gaseous phase. Then the bottle is connected to a vacuum line to extract CO2 gas and to purify it by means of standard techniques for CO2 purification. In order to test this method, several sea water samples were prepared and analysed, as well as a series of standard solutions of Na2CO3 at known isotopic composition of carbon. The accuracy of these measurements was ± 0.2 %° vs V-PDB and their reproducibility was better than 0.2 %° vs V-PDB.
    Description: -National Group for Volcanology, Italy.
    Description: Published
    Description: 313-320
    Description: reserved
    Keywords: Carbon isotopes ; TDIC,CO2 ; HCO3 ; CO2- water interaction ; 03. Hydrosphere::03.01. General::03.01.01. Analytical and numerical modeling ; 03. Hydrosphere::03.04. Chemical and biological::03.04.02. Carbon cycling ; 03. Hydrosphere::03.04. Chemical and biological::03.04.04. Ecosystems ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases ; 03. Hydrosphere::03.04. Chemical and biological::03.04.07. Radioactivity and isotopes ; 03. Hydrosphere::03.04. Chemical and biological::03.04.08. Instruments and techniques
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 5
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    Geochemistry and potential use of groundwater in the Rocca Busambra Area (Sicily, Italy) (2009)
    Springer
    Details
    Publication Date: 2017-04-04
    Description: In the Rocca Busambra area (mid-west Sicily, Italy), from November 1999 to July 2002, 23 water points including wells and springs were sampled and studied for their chemical and isotopic compositions. Two rain gauges were also installed at different altitudes, and rainwater was collected monthly to determine the isotopic composition. The obtained results revealed the Rocca Busambra carbonate complex as being the main recharge area on account of its high permeability value. From a chemical view point, two main groups of water can be distinguished: calcium– magnesium–bicarbonate-type and calcium–magnesium– chloride–sulphate-type waters. The first group reflects the dissolution of the carbonate rocks; the second group probably originates from circulation within flyschoid sediments. Three water wells differ from the other samples due to their relatively high Na and K content, which probably is to be referred to a marked interaction with the ‘‘Calcareniti di Corleone’’ formation, which is rich in glauconite [(K, Na)(Fe3+, Al, Mg)2(Si, Al)4O10(OH)2]. In accordance with WHO guidelines for drinking water (2004), almost all the samples collected can be considered drinkable, with the exception of four of them, whose NO3 -, F- and Na+ contents exceed the limits. On the contrary, the sampled groundwater studied is basically suitable for irrigation.
    Description: Published
    Description: 885-898
    Description: 2.4. TTC - Laboratori di geochimica dei fluidi
    Description: JCR Journal
    Description: reserved
    Keywords: Water quality ; Environmental isotopes ; Geochemistry ; Sicily ; 03. Hydrosphere::03.01. General::03.01.01. Analytical and numerical modeling
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 6
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    Nitrogen isotopes in thermal fluids of a forearc region (Jalisco Block, Mexico): evidence for heavy nitrogen from continental crust (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: The Jalisco Block (JB) is a geologically and tectonically complex part of northwestern Mexico characterized by active subduction-type volcanism, rifting, and old stable structures. Thermal springs and groups of springs are widely distributed over JB. Bubbling gas from seven thermal springs located within different tectonic environments of the JB was analyzed for He, 20Ne, and N2 concentrations and d15N ratios. All gases are N2-dominant (〉84%) with the exception of one sample (Rio´ Purificacio´n), which has a significant CH4 content (about 50%). All collected gas samples are relatively high in He, up to 1500 ppm vol and with 3He/4He values ranging from 0.6 to 4.5 Ra. All measured nitrogen isotope ratios are heavier than air with d15N values ranging from 0.5 to 5.0%. The relative N2 excess with respect to air-saturated water computed on the basis of N2 and 20Ne contents indicates the contribution of a nonatmospheric N2 source. All the samples show a good correlation between d15N and the relative excess of N2 with d15N +5.3% for the maximum N2 excess of 100%. Due to a presumed lack of seafloor sediment involved in the subduction process, such a d15N positive value seems to reflect the addition to the fluids of a heavy nitrogen originating from metamorphism processes of rocks occurring within the overlying continental crust.
    Description: Published
    Description: 1-9
    Description: partially_open
    Keywords: bubbling gases ; forearc region ; Jalisco Block-Mexico ; nitrogen isotopes ; subduction-related volcanism ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases ; 03. Hydrosphere::03.04. Chemical and biological::03.04.06. Hydrothermal systems ; 04. Solid Earth::04.07. Tectonophysics::04.07.06. Subduction related processes ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases ; 05. General::05.02. Data dissemination::05.02.01. Geochemical data
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 7
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    Reply to comment by A. Kopf on ‘‘Methane emission from the mud volcanoes of Sicily (Italy)’’, and notice on CH4 flux data from European mud volcanoes (2005)
    American Geophysical Union
    In:  Etiope G., Caracausi A., Favara R., Italiano F., Baciu C. (2002) Methane emission from the mud volcanoes of Sicily (Italy). Geoph. Res. Letters 29, 14340-14343.
    Details
    Publication Date: 2017-04-04
    Description: The paper ‘‘Methane emission from the mud volcanoes of Sicily (Italy)’’ by Etiope et al. [2002] represents the first report ever done on experimental CH4 output data from subaerial mud volcanoes (MV). A review of available CH4 flux data and detailed discussion about the global implications of mud volcanic CH4 emission has been made elsewhere [Etiope and Klusman, 2002; Morner and Etiope, 2002]. [2] The comment by Kopf [2003] contributes to open discussions and to make the readership aware on how important this subject is. In this reply we wish to clarify that precise data of CH4 flux from geologic sources are beginning to be available only now. It would be opportune that the MV-expert community could agree in using a common unit for the gas flux. We propose t y 1 and Mt y 1, and not metres cubed, consistently with the data reported for the methane sources/sinks budget by the IPCC. [3] Sicilian MVs, the first to be measured in detail, are considerably much smaller than the Azeri Ashgil MV, mentioned by Kopf [2003], and it is therefore obvious to expect a lower gas flux. Anyway the Dashgil mud volcano flux data are not based on exact measurements but only on visual estimates of the bubbles [Hovland et al., 1997]. In order to fully reply to Kopf [2003], hereafter we briefly discuss the problem of how to estimate the total number of MVs in the world and present new data from other European MVs, recently investigated. Finally, we outline the global importance of mud volcanic CH4 emission, as Kopf [2003] and recent literature is stressing.
    Description: Published
    Description: 1094
    Description: partially_open
    Keywords: methane ; mud volcanoes ; helium ; 01. Atmosphere::01.01. Atmosphere::01.01.02. Climate ; 02. Cryosphere::02.03. Ice cores::02.03.02. Atmospheric Chemistry ; 03. Hydrosphere::03.04. Chemical and biological::03.04.02. Carbon cycling ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 8
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    Active geodynamics of the central Mediterranean Sea: Tensional tectonic evidences in western Sicily from mantle-derived helium (2005)
    American Geophysical Union
    Details
    Publication Date: 2017-04-04
    Description: We report results on the measured high 3He/4He isotope ratio in western Sicily, interpreted together with the heat data. The study of this sector of the Europe-Africa interaction is crucial to a better understanding of the tectonics and the geodynamical evolution of the central Mediterranean area. The estimated mantle-derived helium fluxes in the investigated areas are up to 2–3 orders of magnitude greater than those of a stable continental area. The highest flux, found in the southernmost area near the Sicily Channel, where recent eruptions of the Ferdinandea Island occurred 20 miles out to sea off Sciacca, has been associated with a clear excess of heat flow. Our results indicate that there is an accumulation of magma below the continental crust of western Sicily that is possibly intruding and out-gassing through roughly N-S trending deep fault systems linked to the mantle, that have an extensional component. Although the identification of these faults is not sufficiently constrained by our data, they could possibly be linked to the pre-existing faults that originated during the Mesozoic extensional-transtensional tectonic phases.
    Description: Published
    Description: L04312
    Description: partially_open
    Keywords: helium isotopes ; heat production ; tectonics ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases ; 03. Hydrosphere::03.04. Chemical and biological::03.04.06. Hydrothermal systems ; 03. Hydrosphere::03.04. Chemical and biological::03.04.07. Radioactivity and isotopes ; 04. Solid Earth::04.02. Exploration geophysics::04.02.03. Heat flow ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry ; 04. Solid Earth::04.07. Tectonophysics::04.07.03. Heat generation and transport ; 04. Solid Earth::04.07. Tectonophysics::04.07.07. Tectonics
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 9
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    Isotopic, chemical and dissolved gas constraints on spring water from Popocatepetl volcano (Mexico): evidence of gas–water interaction between magmatic component and shallow fluids (2005)
    Elsevier
    Details
    Publication Date: 2017-04-04
    Description: Geochemical research was carried out on cold and hot springs at Popocatepetl (Popo) volcano (Mexico) in 1999 to identify a possible relationship with magmatic activity. The chemical and isotopic composition of the fluids is compatible with strong gas–water interaction between deep and shallow fluids. In fact, the isotopic composition of He and dissolved carbon species is consistent with a magmatic origin. The presence of a geothermal system having a temperature of 80–1008 C was estimated on the basis of liquid geothermometers. A large amount of dissolved CO2 in the springs was also detected and associated with high CO2 degassing.
    Description: Published
    Description: 91– 108
    Description: partially_open
    Keywords: Popocatepetl volcano ; helium isotope composition ; carbon isotope composition ; dissolved gases ; gas–water interaction ; 03. Hydrosphere::03.02. Hydrology::03.02.03. Groundwater processes ; 03. Hydrosphere::03.04. Chemical and biological::03.04.05. Gases ; 03. Hydrosphere::03.04. Chemical and biological::03.04.06. Hydrothermal systems ; 04. Solid Earth::04.04. Geology::04.04.12. Fluid Geochemistry ; 04. Solid Earth::04.08. Volcanology::04.08.01. Gases
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 10
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    Inverse and forward modelling of groundwater circulation in a seismically active area (Monferrato, Piedmont, NW Italy): insights into stress-induced variations in water chemistry (2007)
    Details
    Publication Date: 2017-04-04
    Description: Reaction path modelling, coupled with preparatory inverse modelling, was applied to test this model’s ability to reproduce the wide compositional range of ground waters circulating in a restricted area in Piedmont, Italy. This approach is based on the assumption that the chemistry of groundwater evolves through a series of partial equilibria with secondary minerals until it reaches its final composition. PHREEQC (Purkhurst and Appelo, 1999) and EQ3/6 (Wolery and Daveler, 1992) software packages were used to effect simulations. Reaction-path modelling was performed in time mode, taking into account the different rates of dissolution of each dissolving mineral. Data from literature regarding the kinetic parameters of dissolving minerals and the mineralogical composition of the host-rock were used. The results of the reaction-path modelling show that the composition of the analysed water samples was adequately reproduced, notwithstanding the hydrogeological complexity of the studied area. Modelling results provided very different water compositions as an effect of the chemical maturity, the physico-chemical parameters (fCO2, fO2, and temperature) and the variable amounts of gypsum among dissolving rock-forming minerals, which occur in Miocene levels of the sedimentary sequence. Further variability is related to the occasional contribution of brackish waters trapped in euxinic marly sediments, locally sealed by overlying clays, that have assumed an artesian character. The composition of some of the water samples can only be predicted by simulation runs performed at a temperature higher than that of the outlet (40°C). These warm waters probably circulate in a restricted area near the town of Nizza Monferrato. The same area has recently been affected by moderate seismicity, which has been accompanied by changes in either the temperature or chemistry, or both, of the ground waters. The changes recorded, interpreted as having been triggered by variations in the local/regional stress load and/or seismic activity, have to be ascribed to the vertical heterogeneity of the aquifers, where waters of different temperature, salinity and chemical composition circulate and occasionally mix.
    Description: In press
    Description: 2.4. TTC - Laboratori di geochimica dei fluidi
    Description: JCR Journal
    Description: open
    Keywords: reaction-path modelling ; EQ3/6 ; Inverse modelling ; Tertiary Piedmont Basin ; Monferrato ; Seismicity ; 03. Hydrosphere::03.01. General::03.01.01. Analytical and numerical modeling
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: manuscript
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