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  • 01.01. Atmosphere  (3)
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  • 1
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    Biogenic Aerosol in the Artic from Eight Years of MSA Data from Ny Ålesund (Svalbard Islands) and Thule (Greenland) (2019)
    Details
    Publication Date: 2022-06-09
    Description: In remote marine areas, biogenic productivity and atmospheric particulate are coupled through dimethylsulfide (DMS) emission by phytoplankton. Once in the atmosphere, the gaseous DMS is oxidized to produce H2SO4 and methanesulfonic acid (MSA); both species can a ect the formation of cloud condensation nuclei. This study analyses eight years of biogenic aerosol evolution and variability at two Arctic sites: Thule (76.5 N, 68.8 W) and Ny Ålesund (78.9 N, 11.9 E). Sea ice plays a key role in determining the MSA concentration in polar regions. At the beginning of the melting season, in April, up to June, the biogenic aerosol concentration appears inversely correlated with sea ice extent and area, and positively correlated with the extent of the ice-free area in the marginal ice zone (IF-MIZ). The upper ocean stratification induced by sea ice melting might have a role in these correlations, since the springtime formation of this surface layer regulates the accumulation of phytoplankton and nutrients, allowing the DMS to escape from the sea to the atmosphere. The multiyear analysis reveals a progressive decrease in MSA concentration in May at Thule and an increase in July August at Ny Ålesund. Therefore, while the MSA seasonal evolution is mainly related with the sea ice retreat in April, May, and June, the IF-MIZ extent appears as the main factor a ecting the longer-term behavior of MSA.
    Description: MIUR PRIN 2007 and PRIN 2009, PNRA 2010-2012, PNRA 2015-2016, PNRA 2016-2018
    Description: Published
    Description: id 349
    Description: 5A. Ricerche polari e paleoclima
    Description: JCR Journal
    Keywords: biogenic aerosol, Arctic, sea ice extent, MSA ; 01.01. Atmosphere
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 2
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    The impact of Mount Etna sulfur emissions on the atmospheric composition and aerosol properties in the central Mediterranean: A statistical analysis over the period 2000–2013 based on observations and Lagrangian modelling (2018)
    Details
    Publication Date: 2022-06-09
    Description: The emission of gases and aerosols due to volcanic activity may impact significantly atmospheric composition, cloud occurrence and properties, and the regional and global climate. While the effects of strong explosive (stratospheric) eruptions are relatively well known, limited information on the impacts of small to moderate volcanic activities, including passive degassing, is available. In this paper, the downwind impact of Mount Etna's sulfur emissions on the central Mediterranean is investigated on a statistical basis over the period 2000e2013 using: (a) daily sulfur dioxide emission rates measured near crater at Mount Etna with ground-based ultraviolet spectrophotometers, (b) Lagrangian trajectories and simulated plume dispersion obtained with the FLEXPART (FLEXible PARTicle dispersion) model, and (c) long-term observations of column SO2 concentration and aerosol Ångstr€om exponent a at Lampedusa (35.5 N, 12.6 E). This statistical analysis has allowed, for the first time, the characterization of decadal impact of Mount Etna's sulfur emissions on the sulfur dioxide and the aerosol microphysical/optical properties in the central Mediterranean. On average, statistically significant higher SO2 concentrations and smaller aerosol sizes are present when air masses from Mount Etna overpass Lampedusa. Despite being upwind of Lampedusa for only 5% of the time, Mount Etna is potentially responsible for up to 40% and 20% of the SO2 and a extreme values (exceedances of a fixed threshold), respectively, at this location. The most important factor determining this perturbation is the prevailing dynamics, while the magnitude of the SO2 emission rates from Mount Etna appears to be likely important only for relatively strong emissions. The observed perturbations to the aerosol size distribution are expected to produce a direct regional radiative effect in this area.
    Description: Published
    Description: 77-88
    Description: 6V. Pericolosità vulcanica e contributi alla stima del rischio
    Description: JCR Journal
    Keywords: 04.08. Volcanology ; 01.01. Atmosphere ; climatology
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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  • 3
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    On the Radiative Impact of Biomass-Burning Aerosols in the Arctic: The August 2017 Case Study (2022)
    MDPI
    Details
    Publication Date: 2023-03-30
    Description: Boreal fires have increased during the last years and are projected to become more intense and frequent as a consequence of climate change. Wildfires produce a wide range of effects on the Arctic climate and ecosystem, and understanding these effects is crucial for predicting the future evolution of the Arctic region. This study focuses on the impact of the long-range transport of biomass-burning aerosol into the atmosphere and the corresponding radiative perturbation in the shortwave frequency range. As a case study, we investigate an intense biomass-burning (BB) event which took place in summer 2017 in Canada and subsequent northeastward transport of gases and particles in the plume leading to exceptionally high values (0.86) of Aerosol Optical Depth (AOD) at 500 nm measured in northwestern Greenland on 21 August 2017. This work characterizes the BB plume measured at the Thule High Arctic Atmospheric Observatory (THAAO; 76.53∘N, 68.74∘W) in August 2017 by assessing the associated shortwave aerosol direct radiative impact over the THAAO and extending this evaluation over the broader region (60∘N–80∘N, 110∘W–0∘E). The radiative transfer simulations with MODTRAN6.0 estimated an aerosol heating rate of up to 0.5 K/day in the upper aerosol layer (8–12 km). The direct aerosol radiative effect (ARE) vertical profile shows a maximum negative value of −45.4 Wm−2 for a 78∘ solar zenith angle above THAAO at 3 km altitude. A cumulative surface ARE of −127.5 TW is estimated to have occurred on 21 August 2017 over a portion (∼3.1×106 km2) of the considered domain (60∘N–80∘N, 110∘W–0∘E). ARE regional mean daily values over the same portion of the domain vary between −65 and −25 Wm−2. Although this is a limited temporal event, this effect can have significant influence on the Arctic radiative budget, especially in the anticipated scenario of increasing wildfires.
    Description: This research was partially funded by the Italian Ministry of University and Research (MIUR) within the framework of OASIS-YOPP—Observations of the Arctic Stratosphere In Support of YOPP (PNRA 2016–2018); CLARA2—CLouds And Radiation in the Arctic and Antarctica (PNRA 2019–2021), and ECAPAC—Effects of changing albedo and precipitation on the Arctic climate (PRA 2021–2023). The work of F. Calì Quaglia and G. Muscari was also partially funded under the INGV environmental project MACMAP—A Multidisciplinary Analysis of Climate change indicators in the Mediterranean And Polar regions (2020–2023). The NCAR FTIR observation program at Thule, Greenland is supported under contract by the National Aeronautics and Space Administration (NASA). The National Center for Atmospheric Research (NCAR) is sponsored by the U.S. National Science Foundation (NSF). The Thule work is also supported by the NSF Office of Polar Programs (OPP).
    Description: Published
    Description: 313
    Description: 5A. Ricerche polari e paleoclima
    Description: JCR Journal
    Keywords: biomass-burning (BB) ; wildfires ; Arctic ; aerosol radiative effect ; 01.01. Atmosphere
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
    Type: article
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