Publication Date:
2016-01-07
Description:
Now that evasion of carbon dioxide (CO 2 ) from inland waters is accounted for in global carbon models, it is crucial to quantify how these fluxes have changed in the past and forecast how they may alter in the future in response to local and global change. Here, we developed a sediment proxy for the concentration of summer surface dissolved CO 2 concentration and used it to reconstruct changes over the past 150 years for three large lakes that have been affected by climate warming, changes in nutrient load and detrital terrigenous supplies. Initially CO 2 -neutral to the atmosphere, all three lakes subsequently fluctuated between near-equilibrium and supersaturation. Although catchment inputs have supplied CO 2 to the lakes, internal processes and re-allocation have ultimately regulated decadal changes in lake surface CO 2 concentration. Nutrient concentration has been the dominant driver of CO 2 variability for a century although the reproducible, non-monotonic relationship of CO 2 to nutrient concentration suggests an interplay between metabolic and chemical processes. Yet, for two of these lakes, climatic control of CO 2 concentrations has been important over the last 30 years, promoting higher surface CO 2 concentrations, likely by decreasing hypolimnetic carbon storage. This new approach offers the unique opportunity to scale, a posteriori , the long-term impact of human activities on lake CO 2 .
Print ISSN:
0886-6236
Electronic ISSN:
1944-9224
Topics:
Biology
,
Chemistry and Pharmacology
,
Geography
,
Geosciences
,
Physics
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