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  • 1
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    Method development estimating ambient oxidized mercury concentration from monitored mercury wet deposition (2013)
    Copernicus
    Details
    Publication Date: 2013-11-21
    Description: To quantify mercury dry deposition, the Atmospheric Mercury Network (AMNet) of the National Atmospheric Deposition Program (NADP) was established recently to monitor the speciated atmospheric mercury (i.e. gaseous elemental mercury (GEM), gaseous oxidized mercury (GOM) and particulate-bound mercury (PBM)). However, the spatial coverage of AMNet is far less than the long-established Mercury Deposition Network (MDN) for wet deposition monitoring. The present study describes the first attempt linking ambient concentration of the oxidized mercury (GOM + PBM) with wet deposition aiming to estimate GOM + PBM roughly at locations and/or times where such measurement is not available but where wet deposition is monitored. The beta distribution function is used to describe the distribution of GOM + PBM and is used to predict GOM + PBM from monitored wet deposition. The mean, median, mode, standard deviation, and skewness of the fitted beta distribution parameters were generated using data collected in 2009 at multiple monitoring superstations. The established beta distribution function from the 2009 GOM + PBM data is used to construct a model that predicts GOM + PBM from wet deposition data. The model is validated using 2010 data at multiple stations, and the predicted monthly GOM + PBM concentrations agree reasonably well with measurements. The model has many potential applications after further improvements and validation using different data sets.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 2
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    Method development estimating ambient mercury concentration from monitored mercury wet deposition (2013)
    Copernicus
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    Publication Date: 2013-05-14
    Description: Speciated atmospheric mercury data have recently been monitored at multiple locations in North America; but the spatial coverage is far less than the long-established mercury wet deposition network. The present study describes a first attempt linking ambient concentration with wet deposition using Beta distribution fitting of a ratio estimate. The mean, median, mode, standard deviation, and skewness of the fitted Beta distribution parameters were generated using data collected in 2009 at 11 monitoring stations. Comparing the normalized histogram and the fitted density function, the empirical and fitted Beta distribution of the ratio shows a close fit. The estimated ambient mercury concentration was further partitioned into reactive gaseous mercury and particulate bound mercury using linear regression model developed by Amos et al. (2012). The method presented here can be used to roughly estimate mercury ambient concentration at locations and/or times where such measurement is not available but where wet deposition is monitored.
    Electronic ISSN: 1680-7375
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 3
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    Mapping of satellite Earth observations using moving window block kriging (2014)
    Copernicus
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    Publication Date: 2014-08-08
    Description: Global gridded maps (a.k.a. Level 3 products) of Earth system properties observed by satellites are central to understanding the spatiotemporal variability of these properties. They also typically serve either as inputs into biogeochemical models, or as independent data for evaluating such models. Spatial binning is a common method for generating contiguous maps, but this approach results in a loss of information, especially when the measurement noise is low relative to the degree of spatiotemporal variability. Such "binned" fields typically also lack a quantitative measure of uncertainty. Geostatistical mapping has previously been shown to make higher spatiotemporal resolution maps possible, and also provides a measure of the uncertainty associated with the gridded products. This study proposes a flexible moving window block kriging method that can be used as a tool for creating high spatiotemporal resolution maps from satellite data. It relies only on the assumption that the observed physical quantity exhibits spatial correlation that can be inferred from the observations. The method has several innovations relative to previously applied methods: (1) it provides flexibility in the spatial resolution of the contiguous maps (2) it is applicable for physical quantities with varying spatiotemporal coverage (i.e., density of measurements) by utilizing a more general and versatile data sampling approach, and (3) it provides rigorous assessments of the uncertainty associated with the gridded products. The method is demonstrated by creating Level 3 products from observations of column-integrated carbon dioxide (XCO2) from the GOSAT satellite, and solar induced fluorescence (SIF) from the GOME-2 instrument.
    Print ISSN: 1991-9611
    Electronic ISSN: 1991-962X
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 4
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    Mapping of satellite Earth observations using moving window block kriging (2015)
    Copernicus
    Details
    Publication Date: 2015-10-20
    Description: Global gridded maps (a.k.a. Level 3 products) of Earth system properties observed by satellites are central to understanding the spatiotemporal variability of these properties. They also typically serve either as inputs into biogeochemical models or as independent data for evaluating such models. Spatial binning is a common method for generating contiguous maps, but this approach results in a loss of information, especially when the measurement noise is low relative to the degree of spatiotemporal variability. Such "binned" fields typically also lack a quantitative measure of uncertainty. Geostatistical mapping has previously been shown to make higher spatiotemporal resolution maps possible, and also provides a measure uncertainty associated with the gridded products. This study proposes a flexible moving window block kriging method that can be used as a tool for creating high spatiotemporal resolution maps from satellite data. It relies only on the assumption that the observed physical quantity exhibits spatial correlation that can be inferred from the observations. The method has several innovations relative to previously applied methods: (1) it provides flexibility in the spatial resolution of the contiguous maps, (2) it is applicable for physical quantities with varying spatiotemporal coverage (i.e., density of measurements) by utilizing a more general and versatile data sampling approach, and (3) it provides rigorous assessments of the uncertainty associated with the gridded products. The method is demonstrated by creating Level 3 products from observations of column-integrated carbon dioxide (XCO2) from the GOSAT (Greenhouse Gases Observing Satellite) satellite, and solar induced fluorescence (SIF) from the GOME-2 (Global Ozone Monitoring Experiment-2) instrument.
    Print ISSN: 1991-959X
    Electronic ISSN: 1991-9603
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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  • 5
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    On the diurnal variability in F2-region plasma density above the EISCAT Svalbard radar (2008)
    Copernicus
    Details
    Publication Date: 2008-08-06
    Description: Two long runs of EISCAT Svalbard Radar (ESR), in February 2001 and October 2002, have been analysed with respect to variability in the F2 region peak density and altitude. The diurnal variation in the F2 peak density exhibits one maximum around 12:00 MLT and another around 23:00 MLT, consistent with solar wind controlled transport of EUV ionized plasma across the polar cap from day to night. High density plasma patch material is drawn in through the cusp inflow region independent of IMF BY. There is no apparent IMF BY asymmetry on the intake of high density plasma, but the trajectory of its motion is strongly BY dependent. Comparison with the international reference ionosphere model (IRI2001) clearly demonstrates that the model does not take account of the cross-polar transport of F2-region plasma, and hence has limited applicability in polar cap regions.
    Print ISSN: 0992-7689
    Electronic ISSN: 1432-0576
    Topics: Geosciences , Physics
    Published by Copernicus on behalf of European Geosciences Union.
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