ALBERT

Description: Changes induced by perturbed aerosol conditions in moderately deep mixed-phase convective clouds (cloud top height ∼ 5 km) developing along sea-breeze convergence lines are investigated with high-resolution numerical model simulations. The simulations utilise the newly developed Cloud–AeroSol Interacting Microphysics (CASIM) module for the Unified Model (UM), which allows for the representation of the two-way interaction between cloud and aerosol fields. Simulations are evaluated against observations collected during the COnvective Precipitation Experiment (COPE) field campaign over the southwestern peninsula of the UK in 2013. The simulations compare favourably with observed thermodynamic profiles, cloud base cloud droplet number concentrations (CDNC), cloud depth, and radar reflectivity statistics. Including the modification of aerosol fields by cloud microphysical processes improves the correspondence with observed CDNC values and spatial variability, but reduces the agreement with observations for average cloud size and cloud top height. Accumulated precipitation is suppressed for higher-aerosol conditions before clouds become organised along the sea-breeze convergence lines. Changes in precipitation are smaller in simulations with aerosol processing. The precipitation suppression is due to less efficient precipitation production by warm-phase microphysics, consistent with parcel model predictions. In contrast, after convective cells organise along the sea-breeze convergence zone, accumulated precipitation increases with aerosol concentrations. Condensate production increases with the aerosol concentrations due to higher vertical velocities in the convective cores and higher cloud top heights. However, for the highest-aerosol scenarios, no further increase in the condensate production occurs, as clouds grow into an upper-level stable layer. In these cases, the reduced precipitation efficiency (PE) dominates the precipitation response and no further precipitation enhancement occurs. Previous studies of deep convective clouds have related larger vertical velocities under high-aerosol conditions to enhanced latent heating from freezing. In the presented simulations changes in latent heating above the 0∘C are negligible, but latent heating from condensation increases with aerosol concentrations. It is hypothesised that this increase is related to changes in the cloud field structure reducing the mixing of environmental air into the convective core. The precipitation response of the deeper mixed-phase clouds along well-established convergence lines can be the opposite of predictions from parcel models. This occurs when clouds interact with a pre-existing thermodynamic environment and cloud field structural changes occur that are not captured by simple parcel model approaches.

Description: The COnvective Precipitation Experiment (COPE) was designed to investigate the origins of heavy convective precipitation over the southwestern UK, a region that experiences flash flooding due to heavy precipitation from slow-moving convective systems. In this study, the microphysical and dynamical characteristics of developing turrets during 4 days in July and August 2013 are analyzed. In situ cloud microphysical measurements from the University of Wyoming King Air and vertically pointing W-band radar measurements from Wyoming Cloud Radar are examined, together with data from the ground-based NXPol radar. The 4 days presented here cover a range of environmental conditions in terms of wind shear and instability, resulting in a similarly wide variability in observed ice crystal concentrations, both across days as well as between clouds on individual days. The highest concentration of ice was observed on the days in which there was an active warm-rain process supplying precipitation-sized liquid drops. The high ice concentrations observed (〉100 L−1) are consistent with the production of secondary ice particles through the Hallett–Mossop process. Turrets that ascended through remnant cloud layers above the 0 ∘C level had higher ice particle concentrations, suggesting that entrainment of ice particles from older clouds or previous thermals may have acted to aid in the production of secondary ice through the Hallett–Mossop process. Other mechanisms such as the shattering of frozen drops may be more important for producing ice in more isolated clouds.

Description: Changes induced by perturbed aerosol conditions in moderately deep (cloud top at about 5 km) mixed-phase convective clouds developing along sea-breeze convergence lines are investigated with high-resolution numerical model simulations (grid spacing of 250 m). The simulations utilise the newly developed Cloud-AeroSol Interacting Microphysics module (CASIM) for the Unified Model, which allows for the representation of the two-way interaction between cloud and aerosol fields. Simulations are evaluated against observations collected during the COPE field campaign over the southwestern peninsula of the UK in 2013. The simulations compare favourably with observed thermodynamic profiles, cloud-base cloud droplet number concentrations (CDNC), cloud depth, and radar reflectivity statistics. Including the modification of aerosol fields by cloud microphysical processes in the simulations improves the match to observed cloud-base CDNC, increases the CDNC variability and leads to a larger decrease of CDNC with height above cloud base. However, it also reduces the average cloud size and cloud top height, which is less compatible with observations. Before clouds become organised along the sea-breeze convergence lines, precipitation is suppressed by increasing aerosol due to less efficient precipitation production by warm-phase microphysics. The precipitation suppression is less evident if aerosol processing is taken into account. After the sea breeze convergence zone is established, accumulated precipitation from the on average deeper and wider clouds increases with aerosol concentrations as long as cloud top heights are not limited by an upper level stable layer. The precipitation enhancement is controlled by changes in condensate production and precipitation efficiency. Enhanced condensate production in high aerosol scenarios is related to higher vertical velocities in the convective cores, i.e., convective invigoration, and stronger latent heating below the 0 °C level, while changes in latent heating in the mixed-phase region are negligible. Perturbed aerosol concentrations alter the cloud field structure with fewer larger cells developing in high aerosol environments, but inducing only small changes in cloud fraction. It is hypothesised that the stronger latent heating from convection is related to the changes in the cloud field structure reducing the mixing of environmental air into the convective core. For very high aerosol concentrations, the translation of convective invigoration into deeper clouds and enhanced precipitation is limited by thermodynamic constraints. The aerosol-induced changes in shallow warm-phase clouds prior to the development of a strong convergence zone is consistent with ideas based on parcel models. However, the precipitation response of the deeper mixed-phase clouds along well-established convergence lines suggest that when clouds begin to interact with the pre-existing thermodynamic environment and modifications to the cloud field structure occur, i.e., processes other than microphysics effect the cloud evolution, and the precipitation behaviour can be opposite to predictions from parcel models.

Description: The COnvective Precipitation Experiment (COPE) was designed to investigate the origins of heavy convective precipitation over the South Western UK, a region that experiences flash flooding due to heavy precipitation from slow-moving convective systems. In this study, the microphysical and dynamical characteristics of developing turrets during four days in July and August, 2013 are analyzed. In situ cloud microphysical measurements from the University of Wyoming King Air and vertically pointing W-band radar measurements from Wyoming Cloud Radar are examined, together with data from the ground-based NXPol radar. The four days presented here cover a range of environmental conditions in terms of wind shear and instability, resulting in a similarly wide variability in observed ice crystal concentrations, both across days as well as between clouds on individual days. The highest concentration of ice was observed on the days in which there was an active warm rain process supplying precipitation-sized liquid drops. The high ice concentrations observed (〉100L−1) are consistent with the production of secondary ice particles through the Hallett-Mossop process. Turrets that ascended through remnant cloud layers above the 0°C level had higher ice particle concentrations, suggesting that entrainment of ice particles from older clouds or previous thermals may have acted to aid in the production of secondary ice through the Hallett-Mossop process. Other mechanisms such as the shattering of frozen drops may be more important for producing ice in more isolated clouds.

Description: Heavy rainfall from convective clouds can lead to devastating flash flooding, and observations of aerosols and clouds are required to improve cloud parameterisations used in precipitation forecasts. We present measurements of boundary layer aerosol concentration, size, and composition from a series of research flights performed over the southwest peninsula of the UK during the COnvective Precipitation Experiment (COPE) of summer 2013. We place emphasis on periods of southwesterly winds, which locally are most conducive to convective cloud formation, when marine air from the Atlantic reached the peninsula. Accumulation-mode aerosol mass loadings were typically 2–3 µg m−3 (corrected to standard cubic metres at 1013.25 hPa and 273.15 K), the majority of which was sulfuric acid over the sea, or ammonium sulfate inland, as terrestrial ammonia sources neutralised the aerosol. The cloud condensation nuclei (CCN) concentrations in these conditions were  ∼  150–280 cm−3 at 0.1 % and 400–500 cm−3 at 0.9 % supersaturation (SST), which are in good agreement with previous Atlantic measurements, and the cloud drop concentrations at cloud base ranged from 100 to 500 cm−3. The concentration of CCN at 0.1 % SST was well correlated with non-sea-salt sulfate, meaning marine sulfate formation was likely the main source of CCN. Marine organic aerosol (OA) had a similar mass spectrum to previous measurements of sea spray OA and was poorly correlated with CCN. In one case study that was significantly different to the rest, polluted anthropogenic emissions from the southern and central UK advected to the peninsula, with significant enhancements of OA, ammonium nitrate and sulfate, and black carbon. The CCN concentrations here were around 6 times higher than in the clean cases, and the cloud drop number concentrations were 3–4 times higher. Sources of ice-nucleating particles (INPs) were assessed by comparing different parameterisations used to predict INP concentrations, using measured aerosol concentrations as input. The parameterisations based on total aerosol produced INP concentrations that agreed within an order of magnitude with measured first ice concentrations at cloud temperatures as low as −12 °C. Composition-specific parameterisations for mineral dust, fluorescent particles, and sea spray OA were 3–4 orders of magnitude lower than the measured first ice concentrations, meaning a source of INPs was present that was not characterised by our measurements and/or one or more of the composition-specific parameterisations greatly underestimated INPs in this environment.