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  • American Institute of Physics (AIP)  (2)
  • 1
    Electronic Resource
    Electronic Resource
    The interphase between jellium and a hard sphere electrolyte: Capacity–charge characteristics and dipole potentials (1986)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 85 (1986), S. 1650-1657 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: The jellium/hard sphere electrolyte model for the electric double layer is reconsidered and extended in several ways. The effect of various approximations for the electronic density profile on the calculated capacity values is investigated. On the whole, the new calculations, which are performed with a higher accuracy, confirm our previous results. A heuristic formula for the dielectric response of the ensemble of hard spheres to high electric fields is presented; capacity–charge characteristics calculated from this formula show a capacity maximum close to the potential of zero charge. The dipole potential at the uncharged interface is also calculated; its variation with the metal agrees well with the values derived by Trasatti from experimental data.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.451819
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  • 2
    Electronic Resource
    Electronic Resource
    The capacitance for a single crystal face of an fcc metal/electrolyte interface (1985)
    College Park, Md. : American Institute of Physics (AIP)
    The Journal of Chemical Physics 82 (1985), S. 2825-2826 
    Details
    ISSN: 1089-7690
    Source: AIP Digital Archive
    Topics: Physics , Chemistry and Pharmacology
    Notes: Our earlier calculation of the "inner layer'' interfacial capacitance of a jellium/hard sphere fluid model of the double layer is extended to metal single crystal faces by means of a pseudopotential. The agreement with experiment for Ag is qualitatively satisfactory with the capacitances of the crystal faces ordered correctly and with the relative differences δC/C given with good accuracy.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1063/1.448281
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    Paper (German National Licenses)
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