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  • 42.65  (2)
  • Springer  (2)
  • American Institute of Physics (AIP)
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  • Springer  (2)
  • American Institute of Physics (AIP)
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  • 1
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 93 (1994), S. 205-211 
    ISSN: 1434-6036
    Keywords: 42.65 ; 71.35
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract We describe the dielectric response of the semiconductor band edge in a dynamic density matrix model. Our treatment is based on a set of χ3-relevant constitutive equations involving two-, four- and six-point density matrices. We demonstrate that under certain conditions all contributions to the third order susceptibility can be expressed in terms of excitonic and biexcitonic transitions. As a first application of these χ3-relevant equations we investigate the influence of the biexciton on the optical Stark effect in CuCl. We calculate shifts and lineshapes. Our results turn out to be in excellent agreement with experiments as well as with other theoretical predictions.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    Springer
    The European physical journal 93 (1994), S. 195-204 
    ISSN: 1434-6036
    Keywords: 42.65 ; 71.35 ; 71.45
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract We discuss the interaction of coherent electromagnetic fields with the semiconductor band edge in a dynamic density matrix model. Due to the influence of the Coulomb-interaction then-point density matrices are coupled in an infinite hierarchy of equations of motion. We show how this hierarchy is related to an expansion of the density matrices in terms of powers of the exciting field. We make use of the above results to set up a closed set of equations of motion involving two-, four-and six-point correlation functions, from which all third order contributions to the polarization can be calculated exactly. Comparison of our treatment of the hierarchy with the widely used RPA decoupling on the two-point level, gives interesting insight into the validity of the RPA. In particular we find, that a RPA-like factorization for two of the relevant density-matrices yields a solution of their respective equations of motion to lowest order in the electric field.
    Type of Medium: Electronic Resource
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