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  • 1
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 68 (1990), S. 28-32 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: The sequence of stages during precipitation of semiconductor (e.g., CdS, CdSe) clusters from supersaturated glasses exhibiting quantum-confinement effects was investigated. The rate of formation of nanometer-size "quantum dots'' distributed in a continuous glass matrix is critically determined by the time and temperature of the heat treatment given to the quenched glasses. The entire precipitation process was analyzed in terms of several decomposition stages: nucleation, normal growth, coalescence of quantum dots, and devitrification of the glass matrix itself. Experimental data obtained by differential thermal analysis were utilized to identify the heat-treatment temperature range associated with the precipitation stages. The size distribution of CdSe quantum-dot clusters was analyzed using our transmission electron microscopy data. The data of Ekimov et al. [Solid State Commun. 56, 921 (1975)] was reduced to time-temperature master plots useful for precipitating quantum dots of a given size in glasses.
    Type of Medium: Electronic Resource
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  • 2
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 76 (1994), S. 4576-4580 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: Hot-stage high-voltage (1.5 MeV) transmission electron microscopy was used to directly observe CdS nanocrystals precipitated in a silicate glass and a theoretical framework of nanocrystal coarsening kinetics more appropriate than the popularly used Lifshitz–Slyozov–Wagner theory was developed. Nanocrystallite nucleation and coarsening were monitored in situ by video taping of bright-field images of the edges of thin (less than 2 μm) glass fragments heated in the hot stage; crystallite size distribution was obtained from the taped experimental observations. The effects of electron-beam heating and diffusion out of the nanocrystals were included in developing the theoretical analysis of coarsening kinetics which were used, in turn, to interpret the experimental size distribution curves.
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  • 3
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 76 (1994), S. 3041-3044 
    ISSN: 1089-7550
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We report on the observation of the quantum confinement effect by using photothermal deflection spectroscopy (PDS) experiment and the time dependence of optically induced degradation in CdS and CdSe semiconductor-doped glasses. The observed absorption peaks in the PDS experiment, together with a simple model, were used to evaluate the average radius of semiconductor microcrystals. It is found that the estimated average radii of quantum dots are consistent with that obtained from other methods. This result demonstrates that the PDS technique provides an alternative tool for the study of the optical properties of semiconductor microscrystals. The time dependence of the luminescence degradation of the impurity band, which is attributed to the process of Auger ionization, follows a stretched-exponential function. The inconsistency with the previously proposed exponential relaxation may be due to the size distribution of CdS and CdSe microcrystals.
    Type of Medium: Electronic Resource
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  • 4
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 64 (1993), S. 1723-1733 
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: The absolute x-ray response of three X-UV photodiodes was measured over an energy range of 1.5–17.5 keV so that they could be used to calibrate x-ray imaging systems for the ASCA satellite mission. An intense electron-beam x-ray generator was used to test both the dc and ac x-ray response at 1.5, 4.5, 8.0, and 17.5 keV, and an 55Fe source was used to examine one of the photodiodes at 5.9 keV. The x-ray response was determined by comparing the X-UV diode signal to that of a previously calibrated silicon surface barrier diode (SBD). The X-UV detector response was similar to the SBD response at low energies (1.5 and 4.5 keV). At 8 keV, the X-UV detectors exhibited about 70% of the SBD response, and at 17.5 keV, about 50%. This result is surprising, because the X-UV diodes actually have a greater silicon thickness than the SBD. In contrast to our findings for SBDs in the past, this implies that not the entire physical volume of these detectors comprises the active volume. The X-UV detector x-ray response was also examined as a function of the applied bias voltage. No significant bias voltage dependence of the x-ray signal was found, which indicates that the depletion layer thickness does not determine the active volume either. However, the detector noise was found to decrease substantially as the applied bias was raised from zero to a few volts. Response of these detectors, operated in pulse mode, to 226Ra α particles indicated large charge carrier recombination in the bulk silicon. This feature renders these detectors unsuitable for most charged-particle spectroscopy applications.
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  • 5
    Electronic Resource
    Electronic Resource
    [S.l.] : American Institute of Physics (AIP)
    Review of Scientific Instruments 59 (1988), S. 1721-1722 
    ISSN: 1089-7623
    Source: AIP Digital Archive
    Topics: Physics , Electrical Engineering, Measurement and Control Technology
    Notes: We have examined the feasibility of a fusion γ-ray diagnostic for the Compact Ignition Tokamak (CIT), which is expected to produce 1020 (d, t) fusion reactions per second. Gamma rays at 16.7 MeV are produced by the t(d, γ)He5 fusion reaction. A Monte Carlo coupled neutron–photon transport code is used to model the expected γ-ray spectrum incident upon a Compton spectrometer backed by a Cerenkov detector. The results indicate that a signal of ∼3×104 counts/s and a signal-to-noise ratio of ∼30 can be achieved.
    Type of Medium: Electronic Resource
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  • 6
    Electronic Resource
    Electronic Resource
    Woodbury, NY : American Institute of Physics (AIP)
    Applied Physics Letters 63 (1993), S. 1648-1650 
    ISSN: 1077-3118
    Source: AIP Digital Archive
    Topics: Physics
    Notes: We have obtained nanometer sized silicon remnants sequestered in glass matrices by terminating the reaction of pure silicon powders dispersed in the viscous melt at a temperature of 1400 °C. Repeated use of this truncated melt-particle reaction process dilutes the amount and size of silicon remnants, and bulk samples containing nanosize silicon crystallites embedded in a glass matrix were eventually obtained. These quantum dot sized silicon-in-glass materials emit greenish luminescence with peak wavelengths from ≈480 to 530 nm, considerably shorter than the reddish luminescence (at about 700–850 nm) observed in porous silicon structures prepared by electrochemical etching techniques; upon complete digestion of Si particles by the melt, the luminescence peaks disappear. Since our silicon-in-glass preparation method does not involve etching, the origin of the luminescence is not likely to be due to Si-O-H compounds (e.g., siloxene) postulated recently. The location of the luminescence peaks and the observed silicon crystallite size suggest quantum confinement leading to a widened silicon band gap arising from remnants in the glass matrix smaller than the exciton diameter of bulk silicon (10 nm).
    Type of Medium: Electronic Resource
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  • 7
    Publication Date: 2015-12-23
    Description: We observe experimentally the spectral and spatial reshaping of fluorescence emission in dye-doped dielectric-metal core-shell resonators that support multipolar electric and magnetic-based cavity plasmon resonances. By comparing the experimental fluorescence spectra with analytical calculations based on Mie theory, we are able to demonstrate that the strong reshaping effects are the results of the coupling of dye molecules to those narrow-band cavity plasmon resonances. In addition, we show that the polarization of the fluorescence emission can also be modified by selectively coupling the molecules to the magnetic or electric based cavity plasmons.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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  • 8
    Publication Date: 2016-06-14
    Description: 30-80 nm thick yttrium iron garnet (YIG) films are grown by pulsed laser deposition on a 5 nm thick sputtered Pt atop gadolinium gallium garnet substrate (GGG) (110). Upon post-growth rapid thermal annealing, single crystal YIG(110) emerges as if it were epitaxially grown on GGG(110) despite the presence of the intermediate Pt film. The YIG surface shows atomic steps with the root-mean-square roughness of 0.12 nm on flat terraces. Both Pt/YIG and GGG/Pt interfaces are atomically sharp. The resulting YIG(110) films show clear in-plane uniaxial magnetic anisotropy with a well-defined easy axis along 〈001〉 and a peak-to-peak ferromagnetic resonance linewidth of 7.5 Oe at 9.32 GHz, similar to YIG epitaxially grown on GGG. Both spin Hall magnetoresistance and longitudinal spin Seebeck effects in the inverted bilayers indicate excellent Pt/YIG interface quality.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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  • 9
    Publication Date: 2015-01-07
    Description: We have studied experimentally the Landau level (LL) spectrum of a two-dimensional electron gas (2DEG) in an In 0.53 Ga 0.47 As/InP quantum well structure by means of low-temperature magneto-transport coincidence measurement in vector magnetic fields. It is well known that LL crossing occurs in tilted magnetic fields due to a competition between cyclotron energy and Zeeman effect. Remarkably, here we observe an additional type of level-crossing resulting from a competition between Rashba and Zeeman splitting in a small magnetic field, consistent with the theoretical prediction for strongly spin-orbit coupled 2DEG.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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  • 10
    Publication Date: 2018-06-08
    Description: Observations of aerosol scattering and absorption offer valuable information about aerosol composition. We apply a simulation of the Ultraviolet Aerosol Index (UVAI), a method of detecting aerosol absorption from satellite observations, to interpret UVAI values observed by the Ozone Monitoring Instrument (OMI) from 2005 to 2015 to understand global trends in aerosol composition. We conduct our simulation using the vector radiative transfer model VLIDORT with aerosol fields from the global chemical transport model GEOS-Chem. We examine the 2005–2015 trends in individual aerosol species from GEOS-Chem and apply these trends to the UVAI simulation to calculate the change in simulated UVAI due to the trends in individual aerosol species. We find that global trends in the UVAI are largely explained by trends in absorption by mineral dust, absorption by brown carbon, and scattering by secondary inorganic aerosol. Trends in absorption by mineral dust dominate the simulated UVAI trends over North Africa, the Middle East, East Asia, and Australia. The UVAI simulation resolves observed negative UVAI trends well over Australia, but underestimates positive UVAI trends over North Africa and Central Asia near the Aral Sea and underestimates negative UVAI trends over East Asia. We find evidence of an increasing dust source from the desiccating Aral Sea that may not be well represented by the current generation of models. Trends in absorption by brown carbon dominate the simulated UVAI trends over biomass burning regions. The UVAI simulation reproduces observed negative trends over central South America and West Africa, but underestimates observed UVAI trends over boreal forests. Trends in scattering by secondary inorganic aerosol dominate the simulated UVAI trends over the eastern United States and eastern India. The UVAI simulation slightly overestimates the observed positive UVAI trends over the eastern United States and underestimates the observed negative UVAI trends over India. Quantitative simulation of the OMI UVAI offers new insight into global trends in aerosol composition.
    Print ISSN: 1680-7316
    Electronic ISSN: 1680-7324
    Topics: Geosciences
    Published by Copernicus on behalf of European Geosciences Union.
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