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  • AMER GEOPHYSICAL UNION  (1)
  • American Association for the Advancement of Science (AAAS)  (1)
  • 1
    Publication Date: 2019
    Description: 〈p〉Black carbon (BC) contributes to Arctic climate warming, yet source attributions are inaccurate due to lacking observational constraints and uncertainties in emission inventories. Year-round, isotope-constrained observations reveal strong seasonal variations in BC sources with a consistent and synchronous pattern at all Arctic sites. These sources were dominated by emissions from fossil fuel combustion in the winter and by biomass burning in the summer. The annual mean source of BC to the circum-Arctic was 39 ± 10% from biomass burning. Comparison of transport-model predictions with the observations showed good agreement for BC concentrations, with larger discrepancies for (fossil/biomass burning) sources. The accuracy of simulated BC concentration, but not of origin, points to misallocations of emissions in the emission inventories. The consistency in seasonal source contributions of BC throughout the Arctic provides strong justification for targeted emission reductions to limit the impact of BC on climate warming in the Arctic and beyond.〈/p〉
    Electronic ISSN: 2375-2548
    Topics: Natural Sciences in General
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  • 2
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    AMER GEOPHYSICAL UNION
    In:  EPIC3Journal of Geophysical Research-Atmospheres, AMER GEOPHYSICAL UNION, 115(D12), ISSN: 0148-0227
    Publication Date: 2019-07-16
    Description: The eruptions of the Kasatochi volcano on 7 and 8 August 2008 led to an enhanced stratospheric aerosol load which was studied with the Koldewey Aerosol Raman Lidar (KARL) and the Micro Pulse Lidar (MPL) at the French-German Arctic Research Base AWIPEV in Ny-Ålesund, Spitsbergen at 78.55°N, 11.56°E. During all KARL measurements from 15 August to 24 September 2008 (approximately 30 h of data), we detected distinct layers of enhanced aerosol backscatter in the lower stratosphere and the tropopause region, whose origination at the Kasatochi site can be shown by trajectory calculations. We found a 125% increase in aerosol optical depth compared to the mean values from 2004 to 2007 at 3 weeks after the eruption, validated by sunphotometer measurements. Differences in volume depolarization and color ratio signatures of the layers indicate a sinking movement of the bigger particles to the layer bottom. Furthermore, within higher stratospheric aerosol layers monitored after 25 August 2008, we observed the volume depolarization maximum to be up to 0.8 km below the backscatter maximum. Backscatter and depolarization measurements from 1 September 2008, on which data were collected over 13 h during daylight and darkness, are analyzed in detail. Calculations of the lidar ratio in the lowest aerosol layer as well as the estimation of microphysical parameters of the aerosol particles were performed.
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , isiRev
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