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  • PANGAEA  (259)
  • AGU (American Geophysical Union)  (25)
  • American Meteorological Society  (8)
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  • 1
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    In situ Quality Assessment of a Novel Underwater pCO2 Sensor Based on Membrane Equilibration and NDIR Spectrometry (2014)
    American Meteorological Society
    Details
    Publication Date: 2014-01-01
    Description: This paper presents a detailed quality assessment of a novel underwater sensor for the measurement of CO2 partial pressure (pCO2) based on surface water field deployments carried out between 2008 and 2011. The commercially available sensor, which is based on membrane equilibration and nondispersive IR (NDIR) spectrometry is small and can be integrated into mobile platforms. It is calibrated in water against a proven flow-through pCO2 instrument within a custom-built calibration setup. The aspect of highest concern with respect to achievable data quality of the sensor is the compensation for signal drift inevitably connected to absorption measurements. Three means are used to correct for drift effects: (i) a filter correlation or dual-beam setup, (ii) regular zero gas measurements realized automatically within the sensor, and (iii) a zero-based transformation of two sensor calibrations flanking the time of sensor deployment. Three sensors were tested against an underway pCO2 system during two major research cruises, providing an in situ temperature range from 7.4° to 30.1°C and pCO2 values between 289 and 445 μatm. The average difference between sensor and reference pCO2 was found to be −0.6 ±3.0 μatm with an RMSE of 3.7 μatm.
    Print ISSN: 0739-0572
    Electronic ISSN: 1520-0426
    Topics: Geography , Geosciences , Physics
    Published by American Meteorological Society
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  • 2
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    In Situ CO2and O2Measurements on a Profiling Float (2013)
    American Meteorological Society
    Details
    Publication Date: 2013-01-01
    Print ISSN: 0739-0572
    Electronic ISSN: 1520-0426
    Topics: Geography , Geosciences , Physics
    Published by American Meteorological Society
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  • 3
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    CORRIGENDUM (2014)
    American Meteorological Society
    Details
    Publication Date: 2014-07-01
    Print ISSN: 0739-0572
    Electronic ISSN: 1520-0426
    Topics: Geography , Geosciences , Physics
    Published by American Meteorological Society
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  • 4
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    Pressure Response of Aanderaa and Sea-Bird Oxygen Optodes (2015)
    American Meteorological Society
    Details
    Publication Date: 2015-12-01
    Description: This study investigated the effect of hydrostatic pressure of up to 6000 dbar on Aanderaa and Sea-Bird oxygen optodes both in the laboratory and in the field. The overall pressure response is a reduction in the O2 reading by 3%–4% per 1000 dbar, which is closely linear with pressure and increases with temperature. Closer inspection reveals two superimposed processes with an opposite effect: an O2-independent pressure response on the luminophore that increases optode O2 readings and an O2-dependent change in luminescence quenching that decreases optode O2 readings. The latter process dominates and is mainly due to a shift in the equilibrium between the sensing membrane and seawater under elevated pressures. If only the dominant O2-dependent process is considered, then the Aanderaa and Sea-Bird optodes differ in their pressure response. Compensation of the O2-independent process, however, yields a uniform O2 dependence for Aanderaa optodes with standard foil and fast-response foil as well as for Sea-Bird optodes. A new scheme to calculate optode O2 from raw data is proposed to account for the two processes. The overall uncertainty of the optode pressure correction amounts to 0.3% per 1000 dbar, which is mainly due to variability between the sensors.
    Print ISSN: 0739-0572
    Electronic ISSN: 1520-0426
    Topics: Geography , Geosciences , Physics
    Published by American Meteorological Society
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  • 5
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    Tackling Oxygen Optode Drift: Near-Surface and In-Air Oxygen Optode Measurements on a Float Provide an Accurate in Situ Reference (2015)
    American Meteorological Society
    Details
    Publication Date: 2015-08-01
    Description: A yet unexplained drift of (some) oxygen optodes during storage/transport and thus significant deviations from factory/laboratory calibrations have been a major handicap for autonomous oxygen observations. Optode drift appears to be systematic and is predominantly a slope effect due to reduced oxygen sensitivity. A small contribution comes from a reduced luminophore lifetime, which causes a small positive offset. A reliable in situ reference is essential to correct such a drift. Traditionally, this called for a ship-based reference cast, which poses some challenges for opportunistic float deployments. This study presents an easily implemented alternative using near-surface/in-air measurements of an Aanderaa optode on a 10-cm stalk and compares it to the more traditional approaches (factory, laboratory, and in situ deployment calibration). In-air samples show a systematic bias depending on the water saturation, which is likely caused by occasional submersions of the standard-height stalk optode. Linear regression of measured in-air supersaturation against in-water supersaturation (using ancillary meteorological data to define the saturation level) robustly removes this bias and thus provides a precise (0.2%) and accurate (1%) in situ correction that is available throughout the entire instrument’s lifetime.
    Print ISSN: 0739-0572
    Electronic ISSN: 1520-0426
    Topics: Geography , Geosciences , Physics
    Published by American Meteorological Society
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  • 6
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    Changes in the Ventilation of the Oxygen Minimum Zone of the Tropical North Atlantic (2010)
    American Meteorological Society
    Details
    Publication Date: 2010-08-01
    Description: Changes in the ventilation of the oxygen minimum zone (OMZ) of the tropical North Atlantic are studied using oceanographic data from 18 research cruises carried out between 28.5° and 23°W during 1999–2008 as well as historical data referring to the period 1972–85. In the core of the OMZ at about 400-m depth, a highly significant oxygen decrease of about 15 μmol kg−1 is found between the two periods. During the same time interval, the salinity at the oxygen minimum increased by about 0.1. Above the core of the OMZ, within the central water layer, oxygen decreased too, but salinity changed only slightly or even decreased. The scatter in the local oxygen–salinity relations decreased from the earlier to the later period suggesting a reduced filamentation due to mesoscale eddies and/or zonal jets acting on the background gradients. Here it is suggested that latitudinally alternating zonal jets with observed amplitudes of a few centimeters per second in the depth range of the OMZ contribute to the ventilation of the OMZ. A conceptual model of the ventilation of the OMZ is used to corroborate the hypothesis that changes in the strength of zonal jets affect mean oxygen levels in the OMZ. According to the model, a weakening of zonal jets, which is in general agreement with observed hydrographic evidences, is associated with a reduction of the mean oxygen levels that could significantly contribute to the observed deoxygenation of the North Atlantic OMZ.
    Print ISSN: 0022-3670
    Electronic ISSN: 1520-0485
    Topics: Geosciences , Physics
    Published by American Meteorological Society
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  • 7
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    High Quality Oxygen Measurements from Profiling Floats: A Promising New Technique (2005)
    American Meteorological Society
    Details
    Publication Date: 2005-03-01
    Description: Two state-of-the-art profiling floats were equipped with novel optode-based oceanographic oxygen sensors. Both floats were simultaneously deployed in the central Labrador Sea gyre on 7 September 2003. They drift at a depth of 800 db and perform weekly profiles of temperature, salinity, and oxygen in the upper 2000 m of the water column. The initial results from the first 6 months of operation are presented. Data are compared with a small hydrographic oxygen survey of the deployment site. They are further examined for measurement quality, including precision, accuracy, and drift aspects. The first 28 profiles obtained are of high quality and show no detectable sensor drift. A method of long-term drift control is described and a few suggestions for the operation protocol are provided.
    Print ISSN: 0739-0572
    Electronic ISSN: 1520-0426
    Topics: Geography , Geosciences , Physics
    Published by American Meteorological Society
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  • 8
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    Strong CO2 emissions from the Arabian Sea during South-West Monsoon (1997)
    AGU (American Geophysical Union)
    In:  Geophysical Research Letters, 24 . pp. 1763-1766.
    Details
    Publication Date: 2018-02-13
    Description: The partial pressure of CO2 (pCO2) was measured during the 1995 South-West Monsoon in the Arabian Sea. The Arabian Sea was characterized throughout by a moderate supersaturation of 12–30 µatm. The stable atmospheric pCO2 level was around 345 µatm. An extreme supersaturation was found in areas of coastal upwelling off the Omani coast with pCO2 peak values in surface waters of 750 µatm. Such two-fold saturation (218%) is rarely found elsewhere in open ocean environments. We also encountered cold upwelled water 300 nm off the Omani coast in the region of Ekman pumping, which was also characterized by a strongly elevated seawater pCO2 of up to 525 µatm. Due to the strong monsoonal wind forcing the Arabian Sea as a whole and the areas of upwelling in particular represent a significant source of atmospheric CO2 with flux densities from around 2 mmol m−2 d−1 in the open ocean to 119 mmol m−2 d−1 in coastal upwelling. Local air masses passing the area of coastal upwelling showed increasing CO2 concentrations, which are consistent with such strong emissions.
    Type: Article , PeerReviewed
    Format: text
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  • 9
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    Alkalinity of the Mediterranean Sea (2007)
    AGU (American Geophysical Union)
    In:  Geophysical Research Letters, 34 (15).
    Details
    Publication Date: 2019-09-23
    Description: Total alkalinity (AT) was measured during the Meteor 51/2 cruise, crossing the Mediterranean Sea from west to east. AT concentrations were high (∼2600 μmol kg−1) and alkalinity-salinity-correlations had negative intercepts. These results are explained by evaporation coupled with high freshwater AT inputs into coastal areas. Salinity adjustment of AT revealed excess alkalinity throughout the water column compared to mid-basin surface waters. Since Mediterranean waters are supersaturated with respect to calcite and aragonite, the excess alkalinity likely reflects alkalinity inputs to coastal areas close to regions of deep and intermediate water formation. An alkalinity budget shows that main alkalinity inputs come from the Black Sea and from rivers, whereas the Strait of Gibraltar is a net sink. The major sink appears to be carbonate sedimentation. The basin-average net calcification rate and CaCO3 sedimentation was estimated to be 0.38 mol m−2 yr−1. The estimated residence time of AT is ∼160 yr.
    Type: Article , PeerReviewed
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  • 10
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    Biological and physical controls on N2, O2, and CO2 distributions in contrasting Southern Ocean surface waters (2015)
    AGU (American Geophysical Union) | Wiley
    In:  Global Biogeochemical Cycles, 29 (7). pp. 994-1013.
    Details
    Publication Date: 2019-07-11
    Description: We present measurements of pCO2, O2 concentration, biological oxygen saturation (ΔO2/Ar), and N2 saturation (ΔN2) in Southern Ocean surface waters during austral summer, 2010–2011. Phytoplankton biomass varied strongly across distinct hydrographic zones, with high chlorophyll a (Chl a) concentrations in regions of frontal mixing and sea ice melt. pCO2 and ΔO2/Ar exhibited large spatial gradients (range 90 to 450 µatm and −10 to 60%, respectively) and covaried strongly with Chl a. However, the ratio of biological O2 accumulation to dissolved inorganic carbon (DIC) drawdown was significantly lower than expected from photosynthetic stoichiometry, reflecting the differential time scales of O2 and CO2 air-sea equilibration. We measured significant oceanic CO2 uptake, with a mean air-sea flux (~ −10 mmol m−2 d−1) that significantly exceeded regional climatological values. N2 was mostly supersaturated in surface waters (mean ΔN2 of +2.5%), while physical processes resulted in both supersaturation and undersaturation of mixed layer O2 (mean ΔO2phys = 2.1%). Box model calculations were able to reproduce much of the spatial variability of ΔN2 and ΔO2phys along the cruise track, demonstrating significant effects of air-sea exchange processes (e.g., atmospheric pressure changes and bubble injection) and mixed layer entrainment on surface gas disequilibria. Net community production (NCP) derived from entrainment-corrected surface ΔO2/Ar data, ranged from ~ −40 to 〉 300 mmol O2 m−2 d−1 and showed good coherence with independent NCP estimates based on seasonal mixed layer DIC deficits. Elevated NCP was observed in hydrographic frontal zones and stratified regions of sea ice melt, reflecting physical controls on surface water light fields and nutrient availability.
    Type: Article , PeerReviewed , info:eu-repo/semantics/article
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