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    A temperature dependence kinetics study of the reactions of Cl/2-P-3/2/ with O3, CH4, and H2O2 (1976)
    In:  Other Sources
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    Publication Date: 2011-08-16
    Description: The temperature dependence of two chlorine atom reactions of considerable fundamental importance to stratospheric chemistry was studied using the technique of flash photolysis-resonance fluorescence. The reactions of interest were: (1) Cl + O3 yields ClO + O2 studied at 220-350 K, and (2) Cl + CH4 yields CH3 + HCl studied at 218-401 K. In addition, the reaction Cl + H2O2 yields HCl + HO2 was studied at 300 K. The corresponding rate constants are provided for the three reactions. The new rate data implies the need to revise downward by a factor of 2.4-3 the magnitude of the ozone perturbation due to the presence of ClO/x/ species in the stratosphere, predicted by earlier model calculations.
    Keywords: INORGANIC AND PHYSICAL CHEMISTRY
    Type: Journal of Chemical Physics; 65; Sept. 15
    Format: text
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