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  • Analytical Chemistry and Spectroscopy  (29)
  • Atomic, Molecular and Optical Physics  (5)
  • 11.80.Et  (3)
  • 25.70.Cd  (3)
  • 42.75
  • 2000-2004  (2)
  • 1990-1994  (38)
Collection
Keywords
Publisher
Years
Year
  • 1
    Electronic Resource
    Electronic Resource
    Refractive scattering and reactions, comparison of two systems:16O+16O and20Ne+12C (1993)
    Springer
    The European physical journal 346 (1993), S. 189-200 
    Details
    ISSN: 1434-601X
    Keywords: 24.10.-i ; 24.10.Eq ; 24.20.Ht ; 25.70.Cd
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Elastic, inelastic scattering as well as one-neutron transfer channels have been measured over a wide angular range for systems16O+16O at the incident energy of 350 MeV and20Ne+12C at 390 MeV, respectively, using the Q3D magnetic spectrometer. In both cases differential cross sections have been measured down to about 50 nb/sr (or dσ/dσ R≤10−4) at large angles. For the16O+16O system refractive contributions are found at the level of these cross sections, whereas in the20Ne+12C case a steeper decrease of the differential cross section with the angle is observed and the refractive contribution can not be determined. The elastic scattering data have been analyzed using standard Woods-Saxon potentials and potentials calculated in different versions of the double-folding model. Some properties of these potentials are tested in the calculations for inelastic scattering and one-neutron transfer within the DWBA. With the refractive pattern observed for the16O+16O system, the scattering and transfer data are found to be sensitive to the interaction potential at small internuclear distances down to about 2.5 fm.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01306079
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  • 2
    Electronic Resource
    Electronic Resource
    Measurements of the antiproton-proton elastic cross section in the beam momentum range between 180 and 600 MeV/c (1991)
    Springer
    The European physical journal 339 (1991), S. 367-377 
    Details
    ISSN: 1434-601X
    Keywords: 13.75.Cs ; 11.80.Et
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The differential cross section for antiproton-proton elastic scattering has been measured for the beam momenta between 180 and 600 MeV/c. The real-to-imaginary ratio of the forward elastic scattering amplitude is derived from the Coulomb-nuclear interference. The ratio is found to be close to zero between 180 and 500 MeV/c with a minimum ofρ=−0.14 at 260 MeV/c. This result is contrary to model predictions. The phase shifts for thes-,p- andd-waves are extracted. The partial wave compositions of the elastic and inelastic cross sections have been determined. A large contribution of thep-wave is identified in the antiproton-proton interactions at small momenta.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01560639
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  • 3
    Electronic Resource
    Electronic Resource
    Measurements of the antiproton-proton annihilation cross-section in the beam momentum range between 180 and 600 MeV/c (1990)
    Springer
    The European physical journal 335 (1990), S. 217-229 
    Details
    ISSN: 1434-601X
    Keywords: 13.75.Cs ; 11.80.Et
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The antiproton-proton annihilation cross-section has been mesasured for antiproton beam momenta between 180 and 600 MeV/c. The annihilation cross-section is found to be larger than the geometrical limit of thes-wave inelastic cross-section in this momentum range, indicating a significantp-wave contribution even at low momenta.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01294477
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  • 4
    Electronic Resource
    Electronic Resource
    Ranges of interaction in $$p\bar p$$ scattering at low energies (1991)
    Springer
    The European physical journal 339 (1991), S. 379-382 
    Details
    ISSN: 1434-601X
    Keywords: 13.75.Cs ; 11.80.Et
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract Thep¯ p cross sections at low energies are analysed in the framework of the optical model. It is shown that the annihilation range is closely related to the size of the proton as measured in electromagnetic and hadronic interactions. At larger distances thep¯ p interaction has the similar character as the NN one.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01560640
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  • 5
    Electronic Resource
    Electronic Resource
    Mass spectroscopy of13Be (1992)
    Springer
    The European physical journal 343 (1992), S. 489-490 
    Details
    ISSN: 1434-601X
    Keywords: 21.10.Dr ; 25.70.Cd ; 27.20.+n
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The mass of 13 Be has been measured with the reaction 13 C(14 C,14 O)13 Be at E Lab =337 MeV. A Q-value of Q 0=−37.02(5) MeV was obtained and the mass excess is M.E.=35.16(5) MeV. If the observed line corresponds to the ground state,13 Be is particle unstable with respect to the oneneutron emission by 2.01 MeV. The observed line width of 0.3(2) MeV supports an assignment ofJ π=5/2+ or 1/2−, but excludesJ π=1/2+. An excited state is seen at 3.12(7) MeV; there are indications of a second excited state at 6.5(2) MeV.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01289828
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  • 6
    Electronic Resource
    Electronic Resource
    Solution of the10Li-Puzzle (1993)
    Springer
    The European physical journal 344 (1993), S. 381-393 
    Details
    ISSN: 1434-601X
    Keywords: 21.10.Dr ; 25.70.Cd ; 27.20.+ n
    Source: Springer Online Journal Archives 1860-2000
    Topics: Physics
    Notes: Abstract The mass of10Li has been measured with two different reactions:9Be(13C,12N)10Li,E Lab=336 MeV, and13C(14C,17F)10Li,E Lab=337 MeV. The mass excess of 33.445(50) MeV is deduced from theQ-value measurement.10Li is found to be particle-unstable with respect to one-neutron emission by 0.42(5) MeV. In the analysis of the first reaction a low lying excited state is found at 0.38(8) MeV. This state and the ground state can be most probably identified as the 1+/2+-doublet coupled from the [π 1p3/2 ⊗ν 1p 1/2] configuration, the 1+-state being the ground state. The (13C,12N)-reaction populates the 1+-state strongly due to a spin-isospin-flip character of the dominant part of the transition amplitude. The 2+-member corresponds to the mass given by Wilcox et al. A second excited state is observed at 4.05(10) MeV with a width of 0.7(2) MeV, it can be associated with theν 1d 5/2-strength. The second reaction is fully supporting the interpretation of the ground state doublet. The excited state at 4.05 MeV is not observed in this reaction and indeed it should not, because the reaction does not populate in first order excited neutron configurations. The levels are well described by mean field calculations including pairing correlations. The lowest resonance in the calculations is theν 1/2−-configuration, whereas theν 1/2+-configuration shows at the neutron threshold a strong non-resonant contribution.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01283193
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  • 7
    Electronic Resource
    Electronic Resource
    Intermolecular interactions with the direct reaction field method (1990)
    New York, NY : Wiley-Blackwell
    International Journal of Quantum Chemistry 38 (1990), S. 181-189 
    Details
    ISSN: 0020-7608
    Keywords: Computational Chemistry and Molecular Modeling ; Atomic, Molecular and Optical Physics
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: The direct reaction field (DRF) method, developed to incorporate the effects of a (large) semiclassical environment into the Hamiltonian of a quantum mechanical system, is briefly reviewed. It is shown that the DRF method behaves - at least - like a supermolecule SCF calculation. With the water dimer as an example, the similarity with the SCF procedure is demonstrated, and an application to the interaction between the active site of papain and the remaining 3000 or so atoms of this protein shows the inadequacy of dielectric constant models and the necessity of including atomic polarizabilities in model force fields.
    Additional Material: 3 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/qua.560380213
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  • 8
    Electronic Resource
    Electronic Resource
    Papain in aqueous solution and the role of Asp-158 in the mechanism: An Ab InitioSCF + DRF + BEM study (1991)
    New York, NY : Wiley-Blackwell
    International Journal of Quantum Chemistry 40 (1991), S. 49-59 
    Details
    ISSN: 0020-7608
    Keywords: Computational Chemistry and Molecular Modeling ; Atomic, Molecular and Optical Physics
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: The effects of the solvent on the stability of the zwitterion in the active site of papain is investigated with numerical methods. The solvent is represented by a homogeneous dielectric continuum surrounding a cavity, defined by a fragment of the protein enclosed by a surface obtained following Connolly's method. The discretisized boundary surface is used to solve the Poisson equation in its integral form by means of a numerical approximation based on the boundary element method (BEM), resulting in a set of surface polarization charges. The solvent effect on the proton transfer in papain is studied on the basis of MO-SCF-direct reaction field (DRF) calculations of the energy and charge distribution of the fragment in the field of the surface charges. The role of Asp-158 in the proton transfer in the active site of papain is reevaluated in the presence of the solvent. It is concluded that the effect of the negative charge of Asp-158 is nearly completely screened by the solvent.
    Additional Material: 5 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/qua.560400710
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  • 9
    Electronic Resource
    Electronic Resource
    Computation of scanning tunneling microscope images (1991)
    New York, NY : Wiley-Blackwell
    International Journal of Quantum Chemistry 40 (1991), S. 687-702 
    Details
    ISSN: 0020-7608
    Keywords: Computational Chemistry and Molecular Modeling ; Atomic, Molecular and Optical Physics
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: This article describes the computation of the tunnel current in a scanning tunneling microscope (STM). The calculation accounts for the three-dimensional scattering taking place simultaneously in the first atomic layers of the sample and in the apex of the probing tip. The model is built with the following ingredients: (a) the tip is represented by a cluster of atoms attached to an otherwise planar, free-electron metal surface, and (b) the analyzed sample is a planar free-electron metal with a local potential corrugation induced by an isolated molecule or adatom. The potential barrier includes the strong bending effect due to the image-charge formation occurring as the tunneling electron crosses the gap between the tip and the sample. The specific theoretical approach designed to solve this scattering problem exploits the fast Fourier transform algorithm to construct a transfer matrix in a mixed real- and momentum-spaces representation. The total current is obtained by summing the contributions of all scattered waves traveling in the barrier between the tip and the sample, and it is studied in this article for various positions of the tip relative to the adsorbed atomic cluster. The theory is used here to simulate the scan of a model-aluminum atom on a free-electron metal substrate using electrons focused by a single-atom tungsten tip.
    Additional Material: 8 Ill.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1002/qua.560400860
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  • 10
    Electronic Resource
    Electronic Resource
    Comprehensive Two-Dimensional Gas Chromatography with a Rotating Thermal Desorption Modulator and Independently Temperature-Programmable Columns (2000)
    Weinheim : Wiley-Blackwell
    Journal of High Resolution Chromatography 23 (2000), S. 189-196 
    Details
    ISSN: 0935-6304
    Keywords: Comprehensive two-dimensional gas chromatography ; thermal desorption modulator ; temperature programming ; Chemistry ; Analytical Chemistry and Spectroscopy
    Source: Wiley InterScience Backfile Collection 1832-2000
    Topics: Chemistry and Pharmacology
    Notes: ---In comprehensive two-dimensional gas chromatography, two individual separations are coupled by means of a rotating thermal desorption modulator interface. The injection pulse introduced via the interface onto the second column should be as short as possible. Parameters affecting the modulator operation are studied. In the set-up used in this study, the temperature of the second column can be programmed independently from that of the first column. Optimization of the second-dimension separation to minimize peak broadening and maximize resolution is discussed and an elegant approach to determine second-dimension retention times using a non-constant modulation frequency is demonstrated. The high separation power of the comprehensive system is demonstrated by the analysis of technical and biota samples containing chlorinated biphenyls and toxaphene.
    Additional Material: 7 Ill.
    Type of Medium: Electronic Resource
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