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  • Prebiotic  (6)
  • Springer  (6)
  • 2020-2024
  • 2010-2014
  • 1970-1974  (6)
  • 1945-1949
  • 1
    Electronic Resource
    Electronic Resource
    Further studies of urea-catalyzed phosphorylation reactions (1973)
    Springer
    Journal of molecular evolution 2 (1973), S. 231-234 
    Details
    ISSN: 1432-1432
    Keywords: Phosphorylation ; Nucleotides ; Nucleoside Polyphosphates ; Oligonucleotides ; Urea ; Prebiotic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology
    Notes: Summary We have analyzed the products formed when mixtures of a nucleoside and ammonium dihydrogen phosphate are heated with an excess of urea. If there is more phosphate than nucleoside in the mixture, compounds containing pyrophosphate bonds are obtained. If uridine, as nucleoside, is in excess over phosphate, di- and oligonucleotides are formed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01654004
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  • 2
    Electronic Resource
    Electronic Resource
    Studies in prebiotic synthesis. VII (1972)
    Springer
    Journal of molecular evolution 1 (1972), S. 249-257 
    Details
    ISSN: 1432-1432
    Keywords: Prebiotic ; Nucleosides ; Dry-phase ; Seawater
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology
    Notes: Summary The purine nucleosides (adenosine, guanosine, inosine, xanthosine) are formed when the corresponding purine bases and D-ribose are heated together in the presence of certain salts and minerals. The salts remaining after the evaporation of seawater are particularly effective in these syntheses. The relevance of these reactions for prebiological evolution is discussed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01660244
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  • 3
    Electronic Resource
    Electronic Resource
    On the possible role of crystals in the origins of life (1974)
    Springer
    Journal of molecular evolution 3 (1974), S. 141-150 
    Details
    ISSN: 1432-1432
    Keywords: Adsorption ; Clay ; Montmorillonite ; Phosphoramidates ; Polymerization ; Prebiotic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology
    Notes: Summary Nucleoside phosphoramidates derived from polyamines containing at least three amine groups are strongly adsorbed by sodium and magnesium montmorillonite clays even from very dilute solutions. Heating the dried clay-phosphoramidate mixture results in the production of small amounts of the dinucleotides.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01796559
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  • 4
    Electronic Resource
    Electronic Resource
    Catalysts for the self-polymerization of adenosine cyclic 2′,3′-phosphate (1973)
    Springer
    Journal of molecular evolution 2 (1973), S. 303-316 
    Details
    ISSN: 1432-1432
    Keywords: Polymerization ; Phosphorylation ; Adenosine Cyclic 2′,3′-phosphate ; Oligonucleotides ; Amines ; 2-Aminoethanol ; Amino Acids ; Prebiotic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology
    Notes: Summary When adenosine cyclic 2′,3′-phosphate is evaporated from solution in the presence of simple catalysts such as aliphatic diamines at alkaline pH, and maintained in a dry state at moderate temperatures (25-85°C), self-polymerization to give oligonucleotides of chainlength up to at least 6 is observed. The products contain an excess of [3′→5′]-linkages over [2′→5′]-linkages. The effects of different catalysts and reaction conditions on the efficiency of the reaction are described. The prebiological relevance of these reactions is discussed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01654098
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  • 5
    Electronic Resource
    Electronic Resource
    The possible role of inorganic thiophosphate as a prebiotic phosphorylating agent (1974)
    Springer
    Journal of molecular evolution 3 (1974), S. 317-321 
    Details
    ISSN: 1432-1432
    Keywords: Thiophosphate ; Thymidine ; Phosphorylation of Nucleosides ; Prebiotic
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology
    Notes: Summary It is proposed that inorganic thiophosphate was a versatile and highly reactive constituent of the primitive earth. Some of the ramifications of this assumption with regard to prebiotic chemistry stem from the dual nature of thiophosphate as the most superior nucleophilic agent and an energy rich phosphate. The Michael addition of thiophosphate to acrylonitrile yieldsS-cyanoethylphosphorothioate in high yield. This compound in turn can be used to phosphorylate 2′-deoxythymidine in organic solvents and in the solid state. A mixture of 5′ and 3′-dTMP were identified via chromatography, elementary analysis and NMR spectroscopy.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01796047
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  • 6
    Electronic Resource
    Electronic Resource
    Polyphosphate and trimetaphosphate formation under potentially prebiotic conditions (1972)
    Springer
    Journal of molecular evolution 1 (1972), S. 241-248 
    Details
    ISSN: 1432-1432
    Keywords: Urea ; Ammonium Dihydrogen Phosphate ; Nucleoside ; Prebiotic ; Polyphosphate ; Trimetaphosphate
    Source: Springer Online Journal Archives 1860-2000
    Topics: Biology
    Notes: Summary When ammonium dihydrogen phosphate is heated with urea to temperatures in the range 85–100°C, it polymerizes almost quantitatively to give polyphosphates containing, on the average, more than ten (PO3) residues. Similar experiments carried out at 72°C give polyphosphate in more than 60% yield. If a nucleoside (thymidine or 3′-deoxythymidine) is added to the reaction mixture, up to 23% of trimetaphosphate can be obtained at 100°C. The prebiotic significance of these reactions is discussed.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01660243
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