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  • 2020-2024
  • 2020-2022  (1)
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  • 2020-2024
  • 2020-2022  (1)
  • 2010-2014  (3)
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  • 1
    Publication Date: 2014-04-22
    Description: Recently developed analytical techniques to determine the abundances of noble gases in sediment pore water allow noble-gas concentrations and isotope ratios to be measured easily and routinely in lacustrine sediments. We applied these techniques for the first time to ocean sediments to investigate an active cold methane seepage system located in the South Pacific off the coast of the North Island of New Zealand using 3He/4He ratios determined in the sediment pore water. The results show that more 3He-rich fluids are released in the vicinity of the Pacific–Australian subduction zone than at the forearc stations located closer to the New Zealand coast. However, the He isotope signature in the sediment column indicates that only a minor part of the He emanating from deeper strata originates from a depleted mantle source. Hence, most He in the pore water is produced locally by the radioactive decay of U and Th in the sediment minerals or in the underlying crustal rocks. Such an occurrence of isotopically heavy crustal He also suggests that the source of the largest fraction of methane is a near-surface geochemical reservoir. This finding is in line with a previous δ13C study in the water column which concluded that the emanating methane is most likely of biological origin and is formed in the upper few meters of the sediment column. Moreover, the prevalence of isotopically heavy He agrees well with the outcome of other previous studies on island arc systems which indicate that the forearc regions are characterized by crustal He emission, whereas the volcanic arc region is characterized by the presence of mantle He associated with rising magma.
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  • 2
    Publication Date: 2014-04-22
    Description: Changes in the hydrological regime of the saline closed basin Lake Van, a large, deep lake in eastern Turkey, resulted in a lake level increase by about 2 m between 1988 and 1995, followed by a 1.5 m decrease until 2003 and a relatively constant lake level thereafter. Based on measurements of transient tracers (sulfur hexafluoride, CFC-12, 3H, 3He, 4He, Ne), dissolved oxygen, light transmission, conductivity-temperature-depth profiles, and thermistor data, we investigate the implications associated with lake level fluctuations for deep-water renewal and oxygenation. Our data suggest that deep-water renewal was significantly reduced in Lake Van between 1990 and 2005. This change in mixing conditions resulted in the formation of a more than 100 m thick anoxic deep-water body below 325 m depth. Apparently, the freshwater inflows responsible for the lake level rise between 1988 and 1995 decreased the salinity of the surface water sufficiently that the generation of density plumes during winter cooling was substantially reduced compared to that in the years before the lake level rise. Significant renewal and oxygenation of the deep water did not occur until at least 2005, although by 2003 the lake level was back to almost the same level as in 1988. This study suggests that short-term changes in the hydrological regime, resulting in lake level changes of a couple of meters, can lead to significant and long-lasting changes in deep-water renewal and oxic conditions in deep saline lakes.
    Type: Article , PeerReviewed
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  • 3
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    Elsevier
    In:  Geochimica et Cosmochimica Acta, 75 (10). pp. 2848-2864.
    Publication Date: 2014-04-22
    Description: In this study, the largest ever carried out to measure noble gases in the pore water of unconsolidated sediments in lakes, the emission of terrigenic He through the sediment column of Lake Van was successfully mapped on the local scale. The main input of He to the water body occurs at the borders of a deep basin within the lake, which is probably the remains of a collapsed caldera. The 3He/4He3He/4He ratio identifies the He injected into the sedimentary column of Lake Van as a mixture of He released from a mantle source and radiogenic He of crustal origin (3He/4He∼2.6-4.1×10-6)(3He/4He∼2.6-4.1×10-6). During passage through the pore space, terrigenic He seems to be further enriched in radiogenic He that is most likely produced in the sediment column. In fact, two distinct trends in isotopic composition can be distinguished in the He injected from the lake basement into the sediments. One of these characterizes samples from the shallow water, the other characterizes samples from the deep basin. However, both of these trends are related to the same source of terrigenic He. The He fluxes determined seem to be characteristic of each sampling location and might be considered as a proxy for the fluid permeability of the deep sediment column. These new findings provide insight into the process of fluid transport within the sediments and into the process of formation of the lake basin. Moreover, the isotopic signature of the He that emanates into the water column of Lake Van is strongly affected by the mixing conditions prevailing in the overlying water body. This fact misled previous studies to interpret the terrigenic He in Lake Van as being solely of mantle origin (3He/4He∼10-5)(3He/4He∼10-5).
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  • 4
    Publication Date: 2021-07-12
    Type: Conference or Workshop Item , NonPeerReviewed
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