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  • Articles  (5)
  • Wiley  (5)
  • American Association for the Advancement of Science (AAAS)
  • Cell Press
  • Global Biogeochemical Cycles  (5)
  • 7532
  • Chemistry and Pharmacology  (5)
  • Mathematics
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  • Articles  (5)
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  • 1
    Publication Date: 2011-12-09
    Description: A carbon budget for the Nordic Seas is derived by combining recent inorganic carbon data from the CARINA database with relevant volume transports. Values of organic carbon in the Nordic Seas' water masses, the amount of carbon input from river runoff, and the removal through sediment burial are taken from the literature. The largest source of carbon to the Nordic Seas is the Atlantic Water that enters the area across the Greenland-Scotland Ridge; this is in particular true for the anthropogenic CO2. The dense overflows into the deep North Atlantic are the main sinks of carbon from the Nordic Seas. The budget show that presently 12.3 ± 1.4 Gt C yr−1 is transported into the Nordic Seas and that 12.5 ± 0.9 Gt C yr−1 is transported out, resulting in a net advective carbon transport out of the Nordic Seas of 0.17 ± 0.06 Gt C yr−1. Taking storage into account, this implies a net air-to-sea CO2 transfer of 0.19 ± 0.06 Gt C yr−1 into the Nordic Seas. The horizontal transport of carbon through the Nordic Seas is thus approximately two orders of magnitude larger than the CO2 uptake from the atmosphere. No difference in CO2 uptake was found between 2002 and the preindustrial period, but the net advective export of carbon from the Nordic Seas is smaller at present due to the accumulation of anthropogenic CO2.
    Print ISSN: 0886-6236
    Electronic ISSN: 1944-9224
    Topics: Biology , Chemistry and Pharmacology , Geography , Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 2
    Publication Date: 2012-07-28
    Description: Using in situ measurements, we find a semiannual oscillation (SAO) in the midtropospheric and surface CO2. Chemistry transport models (2-D Caltech/JPL model, 3-D GEOS-Chem, and 3-D MOZART-2) are used to investigate possible sources for the SAO signal in the midtropospheric and surface CO2. From model sensitivity studies, it is revealed that the SAO signal in the midtropospheric CO2 originates mainly from surface CO2 with a small contribution from transport fields. It is also found that the source for the SAO signal in surface CO2 is mostly related to the CO2 exchange between the biosphere and the atmosphere. By comparing model CO2 with in situ CO2 measurements at the surface, we find that models are able to capture both annual and semiannual cycles well at the surface. Model simulations of the annual and semiannual cycles of CO2 in the tropical middle troposphere agree reasonably well with aircraft measurements.
    Print ISSN: 0886-6236
    Electronic ISSN: 1944-9224
    Topics: Biology , Chemistry and Pharmacology , Geography , Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 3
    Publication Date: 2017-06-07
    Description: While the number of surface ocean CO 2 partial pressure (pCO 2 ) measurements has soared the recent decades, the Southern Ocean remains undersampled. Williams et al . [2017] now present pCO 2 estimates based on data from pH-sensor equipped Bio-Argo floats, which have been measuring in the Southern Ocean since 2014. The authors demonstrate the utility of these data for understanding the carbon cycle in this region, which has a large influence on the distribution of CO 2 between the ocean and atmosphere. Biogeochemical sensors deployed on autonomous platforms hold the potential to shape our view of the ocean carbon cycle in the coming decades.
    Print ISSN: 0886-6236
    Electronic ISSN: 1944-9224
    Topics: Biology , Chemistry and Pharmacology , Geography , Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 4
    Publication Date: 2017-02-14
    Description: We present the first estimate of the full global ocean 13 C Suess effect since preindustrial times, based on observations. This has been derived by first using the method of Olsen and Ninnemann [2010] to calculate 13 C Suess effect estimates on sections spanning the world ocean, which were next mapped on a global 1°x1° grid. We find a strong 13 C Suess effect in the upper 1000 m of all basins, with strongest decrease in the Subtropical Gyres of the Northern Hemisphere, where δ 13 C of dissolved inorganic carbon has decreased by more than 0.8‰ since the industrial revolution. At greater depths, a significant 13 C Suess effect can only be detected in the northern parts of the North Atlantic Ocean. The relationship between the 13 C Suess effect and the concentration of anthropogenic carbon varies strongly between water masses, reflecting the degree to which source waters are equilibrated with the atmospheric 13 C Suess effect before sinking. Finally, we estimate a global ocean inventory of anthropogenic CO 2 of 92 ± 46 Gt C. This provides an estimate that is almost independent of, and consistent, within the uncertainties, with previous estimates.
    Print ISSN: 0886-6236
    Electronic ISSN: 1944-9224
    Topics: Biology , Chemistry and Pharmacology , Geography , Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 5
    Publication Date: 2017-02-14
    Description: We present a global ocean climatology of dissolved inorganic carbon δ 13 C (‰) corrected for the 13 C-Suess effect, preindustrial δ 13 C. This was constructed by first using Olsen and Ninnemann's [2010] back-calculation method on data from 25 World Ocean Circulation Experiment cruises to reconstruct the preindustrial δ 13 C on sections spanning all major oceans. Next, we developed five multilinear regression equations, one for each major ocean basin, which were applied on the World Ocean Atlas data to construct the climatology. This reveals the natural δ 13 C distribution in the global ocean. Compared to the modern distribution, the preindustrial δ 13 C spans a larger range of values. The maxima, of up to 1.8‰, occurs in the subtropical gyres of all basins, in the upper and intermediate waters of the North Atlantic, as well as in mode waters with a Southern Ocean origin. Particularly strong gradients occur at intermediate depths, revealing a strong potential for using δ 13 C as a tracer for changes in water mass geometry at these levels. Further, we identify a much tighter relationship between δ 13 C and Apparent Oxygen Utilization (AOU) than between δ 13 C and phosphate. This arises because, in contrast to phosphate, AOU and δ 13 C are both partly reset when waters are ventilated in the Southern Ocean, and underscores that δ 13 C is a highly robust proxy for past changes in ocean oxygen content and ocean ventilation. Our global preindustrial δ 13 C climatology is openly accessible, and can be used for example for improved model evaluation and interpretation of sediment δ 13 C records.
    Print ISSN: 0886-6236
    Electronic ISSN: 1944-9224
    Topics: Biology , Chemistry and Pharmacology , Geography , Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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