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  • Articles  (8)
  • Wiley  (8)
  • Cell Press
  • Frontiers Media
  • National Academy of Sciences
  • 2015-2019  (8)
  • 1995-1999
  • 1980-1984
  • 1955-1959
  • Journal of Geophysical Research JGR - Atmospheres  (4)
  • Journal of Geophysical Research: Atmospheres  (4)
  • 7528
  • 1
    Publication Date: 2019
    Description: Abstract The width of the tropical Hadley circulation (HC) has garnered intense interest in recent decades, owing to the emerging evidence for its expansion in observations and models and to the anticipated impacts on surface climate in its descending branches. To better clarify the causes and impacts of tropical widening, this work generalizes the zonal mean HC to the regional level by defining meridional overturning cells (RC) using the horizontally divergent wind. The edges of the RC are more closely connected to surface hydroclimate than more traditional metrics of regional tropical width (such as the sea level pressure ridge) or even than the zonal mean HC. Simulations reveal a robust weakening of the RC in response to greenhouse gas increases, along with a widening of the RC in some regions. For example, simulated widening of the zonal mean HC in the Southern Hemisphere appears to arise in large part from regional overturning anomalies over the Eastern Pacific, where there is no clear RC. Unforced interannual variability in the position of the zonal mean HC edge is associated with a more general regional widening. These distinct regional signatures suggest that the RCs may be well suited for the attribution of observed circulation trends. The spatial pattern of regional meridional overturning trends in reanalyses corresponds more closely to the pattern associated with unforced interannual variability than to the pattern associated with CO2 forcing, suggesting a large contribution of natural variability to the recent observed tropical widening trends.
    Print ISSN: 2169-897X
    Electronic ISSN: 2169-8996
    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 2
    Publication Date: 2016-04-08
    Description: Based on a uniquely dense network of surface towers measuring continuously the atmospheric concentrations of Greenhouse Gases (GHG's), we developed the first comprehensive monitoring systems of CO 2 emissions at high resolution over the city of Indianapolis. The urban inversion evaluated over the 2012-2013 dormant season, showed a statistically significant increase of about 20% (from 4.5 to 5.7 MtC ±0.23 MtC) compared to the Hestia CO 2 emission estimate, a state-of-the-art building-level emission product. Spatial structures in prior emission errors, mostly undetermined, appeared to affect the spatial pattern in the inverse solution and the total carbon budget over the entire area by up to 15%, while the inverse solution remains fairly insensitive to the CO 2 boundary inflow and to the different prior emissions ( i.e. ODIAC). Preceding the surface emission optimization, we improved the atmospheric simulations using a meteorological data assimilation system also informing our Bayesian inversion system through updated observations error variances. Finally, we estimated the uncertainties associated with undetermined parameters using an ensemble of inversions. The total CO 2 emissions based on the ensemble mean and quartiles (5.26 - 5.91 MtC) were statistically different compared to the prior total emissions (4.1 to 4.5 MtC). Considering the relatively small sensitivity to the different parameters, we conclude that atmospheric inversions are potentially able to constrain the carbon budget of the city, assuming sufficient data to measure the inflow of GHG over the city, but additional information on prior emission error structures are required to determine the spatial structures of urban emissions at high resolution.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 3
    Publication Date: 2019
    Description: Abstract Production and transport of NOx by convection is critical as it serves as a precursor to tropospheric ozone, an important greenhouse gas. Lightning serves as the largest source of nitrogen oxides (NOx = NO + NO2) to the upper troposphere (UT) and is one of the largest natural sources of NOx. Interest is placed on the vertical advection of NOx because its lifetime increases to several days in the UT compared to roughly three hours in the lower troposphere and boundary layer. Thus, lightning can play an important role in ozone production within the UT. However, the amount of NOx produced per flash and NOx advection in storms remain uncertain. This study investigates lightning NOx (LNOx) production and transport processes in anomalous (mid‐level positive charge) and normal polarity (mid‐level negative charge) thunderstorms by advecting parcels containing LNOx from the flash channels of over 5600 lightning flashes observed during the Deep Convective Clouds and Chemistry (DC3) field campaign. Results reveal most flash channels occur near 6‐8 km in the normal polarity thunderstorms and 5‐6 km within anomalous polarity thunderstorms. Larger flash rates and stronger updrafts in anomalous storms result in considerably larger LNOx mixing ratios (peaks of 0.75‐1.75 ppb) in the UT compared to normal polarity storms (peaks 〈 0.5 ppb). A slightly lower mean flash LNOx production was also found among all five storms in this study (storm mean values of 72‐158 moles per flash) compared to previous estimates, which generally parameterize LNOx by flash rate rather than flash rate.
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  • 4
    Publication Date: 2019
    Description: Abstract This study systematically examines the regional uncertainties and biases in carbon dioxide (CO2) mole fractions from two of the state‐of‐the‐art global CO2 analysis products, namely the Copernicus Atmosphere Monitoring Service (CAMS) real‐time atmospheric analysis from the European Centre for Medium‐Range Weather Forecasts and the CarbonTracker Near‐Real Time (CT‐NRT) reanalysis from the National Oceanic and Atmospheric Administration, by evaluation against hundreds of hours of airborne in situ measurements from the summer 2016 and winter 2017 Atmospheric Carbon and Transport (ACT) ‐‐ America field campaigns. Both the CAMS and CT‐NRT analyses agree reasonably well with the independent ACT‐America airborne CO2 measurements in the free troposphere, with root‐mean‐square deviations (RMSDs) between analyses and observations generally between 1‐‐2 ppm, but show considerably larger uncertainties in the atmospheric boundary layer where the RMSDs exceed 8 ppm in the lowermost 1 km of the troposphere in summer. There are strong variations in accuracy and bias between seasons, and across three different subregions in the United States (Mid‐Atlantic, Midwest and South), with the largest uncertainties in the Mid‐Atlantic region in summer. Overall, the RMSDs of the CAMS and CT‐NRT analyses against airborne data are comparable to each other, and largely consistent with the differences between the two analyses. The current study provides uncertainty estimates for both analysis products over North America and suggests that these two independent estimates can be used to approximate regional CO2 analysis uncertainties. Both statistics are important in future studies in quantifying the uncertainties in regional CO2 mole fraction and flux estimates.
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  • 5
    Publication Date: 2018-02-18
    Description: An optimization algorithm is developed to retrieve liquid water cloud properties including cloud optical depth (COD), droplet size distribution and cloud top height (CTH), and aerosol above cloud properties including aerosol optical depth (AOD), single scattering albedo and microphysical properties from sweep-mode observations by JPL's AirMSPI instrument. The retrieval is composed of three major steps: (1) retrieval of an initial estimate of the mean droplet size distribution across the entire image of 80-100 km along-track by 10-25 km across-track from polarimetric cloudbow observations; (2) coupled retrieval of image-scale cloud and above-cloud aerosol properties by fitting the polarimetric data at all observation angles; and (3) iterative retrieval of 1D-RT based COD and droplet size distribution at pixel-scale (25 m) by establishing relationships between COD and droplet size and fitting the total radiance measurements. Our retrieval is tested using 134 AirMSPI datasets acquired during the NASA ORACLES field campaign. The retrieved above-cloud AOD and CTH are compared to coincident HSRL-2 (NASA LaRC) data, and COD and droplet size distribution parameters (effective radius r eff and effective variance v eff ) are compared to coincident RSP (NASA GISS) data. Mean absolute differences (MADs) between AirMSPI and HSRL-2 retrievals of above-cloud AOD at 532 nm and CTH are 0.03 and 〈 0.5 km, respectively. At RSP's footprint scale (323 m), MADs between RSP and AirMSPI retrievals of COD, r eff and v eff in the cloudbow area are 2.33, 0.69 μm and 0.020, respectively. Neglect of smoke aerosols above cloud leads to an underestimate of image-averaged COD by ~15%.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
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  • 6
    Publication Date: 2016-11-12
    Description: We investigate the impact of cirrus cloud heterogeneity on the direct emission by cloud or surface and on the scattering by ice particles in the thermal infrared (TIR). Realistic 3D cirri are modeled with the 3DCLOUD code and top-of-atmosphere radiances are simulated by the 3D Monte Carlo radiative transfer (RT) algorithm 3DMCPOL for two (8.65  μ m and 12.05  μ m) channels of the Imaging Infrared Radiometer (IIR) on CALIPSO. At nadir, comparisons of 1D and 3D RT show that 3D radiances are larger than their 1D counterparts for direct emission but smaller for scattered radiation. For our cirrus cases, 99% of the 3D total radiance is computed by the third scattering order, which corresponds to 90% of the total computational effort, but larger optical thicknesses need more scattering orders. To radically accelerate the 3D RT computations (using only few percent of 3D RT time with a Monte Carlo code), even in presence of large optical depths, we develop a hybrid model based on exact 3D direct emission, the first scattering order from 1D in each homogenized column, and an empirical adjustment linearly dependent on the optical thickness to account for higher scattering orders. Good agreement is found between the hybrid model and the exact 3D radiances for two very different cirrus models without changing the empirical parameters. We anticipate that a future deterministic implementation of the hybrid model will be fast enough to process multi-angle thermal imagery in a practical tomographic reconstruction of 3D cirrus fields.
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  • 7
    Publication Date: 2017-09-19
    Description: Data collected between 1974 and 2016 from snow pits and core samples from two Peruvian ice fields demonstrate the effect of the recent warming over the tropical Andes, augmented by El Niño, on the preservation of the climate record. As the 0 o C isotherm is approaching the summit of the Quelccaya ice cap in the Andes of southern Peru (5670 masl), the distinctive seasonal δ 18 O oscillations in the fresh snow deposited within each thermal year are attenuated at depth due to melting and percolation through the firn. This has become increasingly pronounced over 43 years. In the Andes of northern Peru, the ice field on the col of Nevado Huascarán (6050 masl) has retained its seasonal δ 18 O variations at depth due to its higher elevation. During the 2015/16 El Niño, snow on Quelccaya and Huascarán was isotopically (δ 18 O) enriched and the net sum of accumulation over the previous year (NSA) was below the mean for non-El Niño years, particularly on Quelccaya (up to 64% below the mean) which was more pronounced than the NSA decrease during the comparable 1982/83 El Niño. Interannual large-scale oceanic and middle to upper level atmospheric temperatures influence δ 18 O in precipitation on both ice fields, although the influences are variably affected by strong El Niño-Southern Oscillation events, especially on Quelccaya. The rate of ice wastage along Quelccaya's margin was dramatically higher during 2015/16 compared with that of the previous 15 years, suggesting that warming from future El Niños may accelerate mass loss on Peruvian glaciers.
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  • 8
    Publication Date: 2019
    Description: Abstract Unique in situ observations of atmospheric conditions over the Red Sea and the coastal Arabian Peninsula are examined to study the dynamics and regional impacts of the local land‐sea breeze cycle (LSBC). During a 26 month data record spanning 2008‐2011, observed LSBC events occurred year‐round, frequently exhibiting cross‐shore wind velocities in excess of 8 m/s. Observed onshore and offshore features of both the land‐breeze and sea‐breeze phases of the cycle are presented, and their seasonal modulation is considered. Weather Research and Forecasting (WRF) climate downscaling simulations and satellite measurements are used to extend the analysis. In the model, the amplitude of the LSBC is significantly larger in the vicinity of the steeper terrain elements encircling the basin, suggesting an enhancement by the associated slope winds. Observed and simulated conditions also reflected distinct gravity‐current characteristics of the intrinsic moist marine air mass during both phases of the LSBC. Specifically, the advance and retreat of marine air mass was directly tied to the development of internal boundary layers (IBLs) onshore and offshore throughout the period of study. Convergence in the lateral moisture flux resulting from this air mass ascending the coastal topography (sea breeze phase) as well as colliding with air masses from the opposing coastline (land breeze phase) further resulted in cumulous cloud formation and precipitation.
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