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  • 1
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    Near-surface sediment structures at cold seeps and their physical control on seepage (2010)
    Univ. Bremen
    Details
    Publication Date: 2021-03-29
    Description: The major objective of the study is to investigate how near-surface sediment structures and other geological aspects control the nature and occurrence of cold fluid seepage. Mainly high resolution multichannel seismic data and swatch bathymetry data were used to study nearsurface seismostratigraphy, structure and seismic fluid-indicating features in two different fluid seepage provinces: Campeche Knolls, southern Gulf of Mexico and the frontal Makran, offshore Pakistan. The two areas have fundamentally different tectonic settings: The Campeche Knolls, southern Gulf of Mexico represents a passive margin influenced by salt tectonism, while the frontal Makran is the most basinward part of the Makran accretionary prism, characterized by plate subduction, sediment accretion, thrust faulting and development of sediment imbricate slices. However, they share quite a few similarities in shallow sediment structures and fluid seepage patterns...
    Description: thesis
    Keywords: 551.23 ; 553.28 ; 550 ; TSZ 100 ; VAE 880 ; TSZ 200 ; Atlantischer Ozean {Geophysik} ; Passive und aktive Kontinentalränder {Geologie} ; Indischer Ozean {Geophysik}
    Language: English
    Type: monograph , publishedVersion
    Format: 125 S.
    Format: application/pdf
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    CITATION GEO-LEO
  • 2
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    Evaporation Study Based on Micromodel Experiments: Comparison of Theory and Experiment (2021)
    Details
    Publication Date: 2021-10-11
    Description: Abstract Evaporation—a key process for water exchange between soil and atmosphere—is controlled by internal water fluxes and surface vapor fluxes. Recent studies demonstrated that the dynamics of the water flow in corners determine the time behavior of the evaporation rate. The internal water flux of the porous media is often described by capillary flow assuming complete wetting. Particularly, the crucial influence of partial wetting, that is, the nonlinear contact angle dependency of the capillary flow has been neglected so far. The focus of the paper is to demonstrate that SiO2-surfaces can exhibit contact angles of about 40°. This reduces the internal capillary flow by 1 order of magnitude compared to complete wetting. First, we derived the contact angle by inverse modeling. We conducted a series of evaporation experiments in a 2-D square lattice microstructure connected by lognormal distributed throats. We used an explicit analytical power series solution of the single square capillary model. A contact angle of 38° ± 1° was derived. Second, we directly measured the contact angle of the Si-SiO2 wafer using the Drop Shape Analyzer Krüss 100 and obtained an averaged contact angle of 42° ± 2°. The results support the single square capillary model as an appropriate model for the description of the evaporation process in an ideal square capillary.
    Keywords: 550.724 ; 551.5 ; evaporation ; experiments
    Language: English
    Type: map
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    CITATION GEO-LEO
  • 3
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    The Impact of Wettability and Surface Roughness on Fluid Displacement and Capillary Trapping in 2-D and 3-D Porous Media: 2. Combined Effect of Wettability, Surface Roughness, and Pore Space Structure on Trapping Efficiency in Sand Packs and Micromodels (2021)
    Details
    Publication Date: 2021-10-13
    Description: A comprehensive understanding of the combined effects of surface roughness and wettability on the dynamics of the trapping process is lacking. This can be primarily attributed to the contradictory experimental and numerical results regarding the impact of wettability on the capillary trapping efficiency. The discrepancy is presumably caused by the surface roughness of the inner pore-solid interface. Herein, we present a comparative μ-CT study of the static fluid-fluid pattern in porous media with smooth (glass beads) and rough surfaces (natural sands). For the first time, a global optimization method was applied to map the characteristic geometrical and morphological properties of natural sands to 2-D micromodels that exhibit different degrees of surface roughness. A realistic wetting model that describes the apparent contact angle of the rough surface as a function surface morphology and the intrinsic contact angle was also proposed. The dynamics of the trapping processes were studied via visualization micromodel experiments. Our results revealed that sand and glass beads displayed opposite trends in terms of the contact angle dependence between 5° and 115°. Sand depicted a nonmonotonous functional contact angle dependency, that is, a transition from maximal trapping to no trapping, followed by an increase to medium trapping. In contrast, glass beads showed a sharp transition from no trapping to maximal trapping. Since both porous media exhibit similar morphological properties (similar Minkowski functions: porosity, surface density, mean curvature density, Euler number density), we deduce that this difference in behavior is caused by the difference in surface roughness that allows complete wetting and hence precursor thick-film flow for natural sands. Experimental results on micromodels verified this hypothesis.
    Keywords: 550.724 ; impact of wettability on trapping efficiency ; impact of surface roughness and pore space structure on trapping efficiency ; porous media with rough surface ; natural sand and glass ceramic micromodels ; wettability-controlled crossover from snap-off to bypass trapping ; spontaneous precursor thick-film flow (Wenzel's argument)
    Language: English
    Type: map
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    CITATION GEO-LEO
  • 4
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    Chemical characteristics of air masses from different urban and industrial centers in the Huabei region of China (2013)
    In:  Atmospheric Environment
    Details
    Publication Date: 2023-07-18
    Type: info:eu-repo/semantics/article
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  • 5
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    Tropospheric Ozone Assessment Report: Database and Metrics Data of Global Surface Ozone Observations (2017)
    In:  Elementa : Science of the Anthropocene
    Details
    Publication Date: 2023-07-18
    Description: In support of the first Tropospheric Ozone Assessment Report (TOAR) a relational database of global surface ozone observations has been developed and populated with hourly measurement data and enhanced metadata. A comprehensive suite of ozone data products including standard statistics, health and vegetation impact metrics, and trend information, are made available through a common data portal and a web interface. These data form the basis of the TOAR analyses focusing on human health, vegetation, and climate relevant ozone issues, which are part of this special feature.Cooperation among many data centers and individual researchers worldwide made it possible to build the world's largest collection of in-situ hourly surface ozone data covering the period from 1970 to 2015. By combining the data from almost 10,000 measurement sites around the world with global metadata information, new analyses of surface ozone have become possible, such as the first globally consistent characterisations of measurement sites as either urban or rural/remote. Exploitation of these global metadata allows for new insights into the global distribution, and seasonal and long-term changes of tropospheric ozone and they enable TOAR to perform the first, globally consistent analysis of present-day ozone concentrations and recent ozone changes with relevance to health, agriculture, and climate.Considerable effort was made to harmonize and synthesize data formats and metadata information from various networks and individual data submissions. Extensive quality control was applied to identify questionable and erroneous data, including changes in apparent instrument offsets or calibrations. Such data were excluded from TOAR data products. Limitations of a posteriori data quality assurance are discussed. As a result of the work presented here, global coverage of surface ozone data for scientific analysis has been significantly extended. Yet, large gaps remain in the surface observation network both in terms of regions without monitoring, and in terms of regions that have monitoring programs but no public access to the data archive. Therefore future improvements to the database will require not only improved data harmonization, but also expanded data sharing and increased monitoring in data-sparse regions.
    Language: English
    Type: info:eu-repo/semantics/article
    Format: application/pdf
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  • 6
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    Upper tropospheric warming intensifies sea surface warming (2014)
    In:  Climate Dynamics
    Details
    Publication Date: 2023-07-18
    Type: info:eu-repo/semantics/article
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  • 7
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    The striking effect of vertical mixing in the planetary boundary layer on new particle formation in the Yangtze River Delta (2022)
    In:  The science of the total environment
    Details
    Publication Date: 2023-07-18
    Description: New particle formation (NPF) induces a sharp increase in ultrafine particle number concentrations and potentially acts as an important source of cloud condensation nuclei (CCN). As the densely populated area of China, the Yangtze River Delta (YRD) region shows a high frequency of observed NPF events at the ground level, especially in spring. Although recent observational studies suggested a possible connection between NPF at the higher altitudes and ground level, the role played by vertical mixing, particularly in the planetary boundary layer (PBL) is not fully understood. Here we integrate measurements in Nanjing on 15–20 April 2018, and the NPF-explicit Weather Research and Forecast coupled with chemistry (WRF-Chem) model simulations to better understand the governing mechanisms of the NPF and CCN. Our results indicate that newly formed particles at the boundary layer top could be transported downward by vertical mixing as the PBL develops. A numerical sensitivity simulation created by eliminating aerosol vertical mixing suppresses both the downward transport of particles formed at a higher altitude and the dilution of particles at the ground level. The resulting higher Fuchs surface area at the ground level, together with the lack of downward transport, yields a sharp weakening of NPF strength and delayed start of NPF therein. The aerosol vertical mixing, therefore, leads to a more than double increase of surface CN10–40 and a one third decrease of boundary layer top CN10–40. Additionally, the continuous growth of nucleated ultrafine particles at the boundary layer top is strongly steered by the upward transport of condensable gases, with close to half increase of particle number concentrations in Aitken mode and CCN at a supersaturation rate of 0.75%. The findings may bridge the gap in understanding the complex interaction between PBL dynamics and NPF events, reducing the uncertainty in assessing the climate impact of aerosols.
    Language: English
    Type: info:eu-repo/semantics/article
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