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  • 1
    Publication Date: 2016-01-05
    Description: For many decades, phonon transport at interfaces has been interpreted in terms of phonons impinging on an interface and subsequently transmitting a certain fraction of their energy into the other material. It has also been largely assumed that when one joins two bulk materials, interfacial phonon transport can be described in terms of the modes that exist in each material separately. However, a new formalism for calculating the modal contributions to thermal interface conductance with full inclusion of anharmonicity has been recently developed, which now offers a means for checking the validity of this assumption. Here, we examine the assumption of using the bulk materials' modes to describe the interfacial transport. The results indicate that when two materials are joined, a new set of vibrational modes are required to correctly describe the transport. As the modes are analyzed, certain classifications emerge and some of the most important modes are localized at the interface and can exhibit large conductance contributions that cannot be explained by the current physical picture based on transmission probability.
    Print ISSN: 0021-8979
    Electronic ISSN: 1089-7550
    Topics: Physics
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  • 2
    Publication Date: 2016-05-06
    Description: We studied the heat conduction at InGaAs/InP interfaces and found that the total value of interface conductance was quite high ∼830 MW m −2  K −1 . The modal contributions to the thermal interface conductance (TIC) were then investigated to determine the mode responsible. Using the recently developed interface conductance modal analysis method, we showed that more than 70% of the TIC arises from extended modes in the system. The lattice dynamics calculations across the interface revealed that, unlike any other interfaces previously studied, the different classes of vibration around the interface of InGaAs/InP naturally segregate into distinct regions with respect to frequency. In addition, interestingly, the entire region of frequency overlap between the sides of the interface is occupied by extended modes, whereby the two materials vibrate together with a single frequency. We also mapped the correlations between modes, which showed that the contribution by extended modes to the TIC primarily arises from coupling to the modes that have the same frequencies of vibration (i.e., autocorrelations). Moreover, interfacial modes despite their low population still contribute more than 6% to interfacial thermal transport. The analysis sheds light on the nature of heat conduction by different classes of vibration that exist in interfacial systems, which has technological relevance to applications such as thermophotovoltaics and optoelectronics.
    Print ISSN: 0003-6951
    Electronic ISSN: 1077-3118
    Topics: Physics
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