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  • Elsevier  (116,549)
  • 2010-2014  (116,549)
  • 2012  (116,549)
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  • 1
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    Optimization and mathematical modeling of mass transfer between Zostera marina residues and supercritical CO2 modified with ethanol (2012)
    Elsevier
    Details
    Publication Date: 2023-06-19
    Description: Supercritical CO2 extraction of phenolic compounds from Zostera marina residues was optimized by developing a mathematical model based on mass transfer balances. A linear driving force model was applied considering model parameters such as solute concentration on the surface of the solid (Cs) and in the supercritical fluid phase (Cf), film mass transfer coefficient (kf) and molecular diffusivity (DAB) and axial dispersion (Dax) coefficients. Henry's law was used to describe the equilibrium state of solid and fluid phases. The results of the proposed model were compared to that of the experimental data in terms of transport properties and extraction yield at various temperatures (303.15, 323.15, 353.15 K), pressures (15, 25, 35 MPa) and co-solvent mass ratios (0, 10, 20%). The optimum parameters were elicited as 25 MPa, 353.15 K and a co-solvent ratio of 20% yielding 77.22 μg g−1 dry feed. The model satisfactorily described the extraction yield which can be used for scale-up purposes.
    Type: Article , PeerReviewed
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  • 2
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    An integrated process for conversion of Zostera marina residues to bioethanol (2012)
    Elsevier
    Details
    Publication Date: 2023-06-19
    Description: Zostera marina is an aquatic plant forming wide grasslands and considered as the lungs of the marine ecosystems. However, the residues reaching the coastlines create nuisance and high costs are required for their disposal. The objective was to investigate the potential of Z. marina residues as a source of secondary metabolites and feedstock in order to propose alternative solutions to the landfill. The supercritical CO2 extract had a total phenol value of 55.4 mg GAE/g extract and a radical scavenging capacity of 71.4%. Considering the raffinate phase, 3% higher hemicellulose content was reached after supercritical CO2 treatment. Enzymatic hydrolysis revealed 31.45% and the yield of simultaneous saccharification and fermentation was 8.72% corresponding to a productivity of 0.273 kg/(m3 h). An integrated process is proposed, where supercritical fluid extraction can act both as the main process to obtain solvent-free pharmaceutical compounds and a pretreatment method in order to loosen the lignin structure, thereby liberating some of the hemicellulose in the matrix.
    Type: Article , PeerReviewed
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  • 3
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    The hafnium and neodymium isotope composition of seawater in the Atlantic sector of the Southern Ocean (2012)
    Elsevier
    Details
    Publication Date: 2023-03-09
    Description: We present the first combined dissolved hafnium (Hf) and neodymium (Nd) concentrations and isotope compositions of deep water masses from the Atlantic sector of the Southern Ocean. Eight full depth profiles were analyzed for Hf and twelve for Nd. Hafnium concentrations are generally depleted in the upper few hundred meters ranging between 0.2 pmol/kg and 0.4 pmol/kg and increase to relatively constant values of around 0.6 pmol/kg in the deeper water column. At the stations north of the Polar Front (PF), Nd concentrations increase linearly from about 10 pmol/kg at depths of ~ 200 m to up to 31 pmol/kg close to the bottom indicating particle scavenging and release. Within the Weddell Gyre (WG), however, Nd concentrations are essentially constant at 25 pmol/kg at depths greater than ~ 1000 m. The distributions of both elements show a positive correlation with dissolved silicon implying a close linkage to diatom biogeochemistry. Hafnium essentially shows invariant isotope compositions with values averaging at εHf = + 4.6, whereas Nd isotopes mark distinct differences between water masses, such as modified North Atlantic Deep Water (NADW, εNd = − 11 to − 10) and Antarctic Bottom Water (AABW, εNd = − 8.6 to − 9.6), but also waters locally advected via the Agulhas Current can be identified by their unradiogenic Nd isotope compositions. Mixing calculations suggest that a small fraction of Nd is removed by particle scavenging during mixing of water masses north of the PF. Nevertheless, the Nd isotope composition has apparently not been significantly affected by uptake and release of Nd from particles, as indicated by mixing calculations. A mixing envelope of an approximated North Pacific and a North Atlantic end-member shows that Nd isotope and concentration patterns in the Lower Circumpolar Deep Water (LCDW) can be fully explained by ~ 30:70 percentage contributions of these respective end-members.
    Type: Article , PeerReviewed
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  • 4
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    The ecophysiology and bloom dynamics of Prymnesium spp. (2012)
    Elsevier
    Details
    Publication Date: 2023-02-15
    Description: Members of Prymnesium belong to the division Haptophyta, class Prymnesiophyceae, order Prymnesiales and family Prymnesiaceae. As most haptophytes, members of the genus Prymnesium are unicellular and planktonic. The most known of these species is the ichthyotoxic P. parvum, which may form nearly monospecific dense blooms in coastal and inland waters. This species possesses extraordinary plasticity concerning life survival strategies, and is specifically addressed in this review. Toxins produced by P. parvum have hemolytic properties, that not only kill fish but also co-existing plankton. These substances are allelopathic (when other algae are killed) and grazer deterrent (when grazers are killed). Allelopathy enables P. parvum to utilize inorganic nutrients present in the surrounding water without competition from other algal species; and by eliminating its grazers P. parvum reduces cell losses. The paralized microalgae and/or zooplankton, are therefter ingested by the P. parvum cells, a process called phagotrophy. P. parvum is also able of osmotrophy, i.e. utilization of dissolved organic matter. In this review, the cellular characteristics, life cycles, bloom formation, and factors affecting toxicity, allelopathy, phagotrophy, and osmotrophy of P. parvum are discussed.
    Type: Article , PeerReviewed
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  • 5
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    Transcriptomic response of the toxic prymnesiophyte Prymnesium parvum (N. Carter) to phosphorus and nitrogen starvation (2012)
    Elsevier
    Details
    Publication Date: 2023-02-15
    Description: The ichthyotoxic and mixotrophic prymnesiophyte Prymnesium parvum is known to produce dense virtually monospecific blooms in marine coastal, brackish, and inshore waters. Fish-killing Pyrmnesium blooms are often associated with macronutrient imbalanced conditions based upon shifts in ambient nitrogen (N):phosphorus (P) ratios. We therefore investigated nutrient-dependent cellular acclimation mechanisms of this microalga based upon construction of a normalized expressed sequence tag (EST) library. We then profiled the transcriptome of P. parvum under nutrient-replete conditions as well as under nitrogen (N) and phosphorus (P) limitation via microarray analyses. Twenty-three genes putatively involved in acclimation to low nutrient levels were identified, among them three phosphate transporters, which were highly upregulated under P-starvation. In contrast, the expression of genes involved in transport and acquisition of ammonium or nitrate/nitrite was unaltered in N-starved cells. We propose that genes upregulated under P- or N-starvation lend themselves as potential tools to monitor nutrient limitation effects at the cellular level and indirectly the potential for initiation and maintenance of toxic blooms of P. parvum.
    Type: Article , PeerReviewed
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  • 6
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    Effects of nitrogen supply and its composition on the growth of Prorocentrum donghaiense (2012)
    Elsevier
    Details
    Publication Date: 2023-02-15
    Description: In order to better understand the complex nitrogen (N) dynamics contributing to blooms of the harmful alga, Prorocentrum donghaiense, in eutrophic environments, we compared the growth of this organism on various forms of dissolved inorganic (nitrate and ammonium) and organic N (urea, glutamic acid, peptides and cyanate) compounds both individually and in combination. Growth rates of P. donghaiense were comparable in cultures grown with ammonium, nitrate, urea, glutamic acid, or the dipeptide phenylalanine-alanine as the sole source of N. P. donghaiense could also grow with cyanate or dialanine as sole sources of N, but at lower rates. Different DONurea, glutamic acid or diala:DINnitrate or ammonium ratios and nitrate:ammonium ratios also affected the growth of P. donghaiense. Growth rates of cultures acclimated on media with combinations of nitrate or ammonium and DON (urea, glutamic acid or alanine-alanine), grew faster than those growing on DON alone. The ratio of nitrate:ammonium in the growth media had little effect on the growth of P. donghaiense. Our uptake experiments exhibited complicated interactions among different nutrients. Nitrate uptake was inhibited by ammonium, glutamic acid and urea. In contrast, ammonium uptake was stimulated by urea and glutamic acid. Further research is needed to understand how the complex mixture of N compounds found in natural systems contributes to the growth and proliferation of P. donghaiense in the environment as this has implications for nutrient management. Because nitrate concentrations are elevated in areas prone to P. donghaiense blooms, nutrient reductions have targeted nitrate. The results presented here suggest that total N loads must be reduced to prevent blooms of this organism in coastal waters.
    Type: Article , PeerReviewed
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  • 7
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    Uptake of alkaline earth metals in Alcyonarian spicules (Octocorallia) (2012)
    Elsevier
    Details
    Publication Date: 2023-01-31
    Description: Alcyonarian corals (Octocorallia) living in shallow tropical seas produce spicules of high-Mg calcite with ∼13 mol% MgCO3. We cultured the tropical alcyonarian coral Rhythisma fulvum in experiments varying temperature (19–32 °C) and pH (8.15–8.44). Alkalinity depletion caused by spicule formation systematically varied in the temperature experiments increasing from 19 to 29 °C. Spicules were investigated for their elemental ratios (Mg/Ca, Sr/Ca) using ICP-OES, δ44/40Ca using TIMS, as well as δ18O and δ13C by IRMS. Mg/Ca increased with temperature from 146 to 164 mmol/mol, in good agreement with the range observed for marine inorganic calcite. Mg/Ca increased by 1.0 ± 0.4 mmol/mol/°C, similar to the sensitivity of Miliolid foraminifera. The pH experiments revealed a linear relationship between Mg/Ca and carbonate ion concentration of +0.03 ± 0.02 mmol/mol/μMol. Sr/Ca ranges from 2.5 to 2.9 mmol/mol being in good agreement with other high-Mg calcites. Temperature and pH experiments showed linear dependencies of Sr/Ca matching inorganic calcite trends and pointing to a decoupling of crystal precipitation rate and calcification rate. Ca isotopes range between 0.7‰ and 0.9‰ in good agreement with aragonitic scleractinian corals and calcitic coccoliths. Presumably Ca isotopes are fractionated by a biological mechanism that may be independent of the skeletal mineralogy. We observe no temperature trend, but a significant decrease of δ44/40Ca with increasing pH. This inverse correlation may characterise biologically controlled intracellular calcification. Oxygen isotope ratios are higher than expected for isotopic equilibrium with a temperature sensitivity of −0.15 ± 0.03‰/°C. Carbon isotope ratios are significantly lower than expected for equilibrium and positively correlated with temperature with a slope of 0.20 ± 0.04‰/°C. Many of our observations on trace element incorporation in R. fulvum may be explained by inorganic processes during crystal formation, which do not comply with the intracellular mode of calcification in Alcyonarian corals. The observed elemental and isotopic compositions, however, could be explained if the partitioning caused by biological mechanisms mimics the effects of inorganic processes.
    Type: Article , PeerReviewed
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  • 8
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    Dynamic plumbing system beneath volcanoes revealed by kinetic modeling, and the connection to monitoring data: An example from Mt. Etna (2012)
    Elsevier
    Details
    Publication Date: 2023-01-27
    Description: Our ability to monitor volcanoes (using seismic signals, ground deformation, gas fluxes, or other ground and satellite based observations) as well as our understanding of melt reservoirs that feed eruptions have evolved tremendously in recent years. The complex plumbing systems that are thought to feed eruptions are, however, difficult to relate to the monitoring signals. Here we show that the record preserved in compositional zoning of erupted minerals may be used to reconstruct sections of the plumbing system. Kinetic modeling of such zoning can yield information on the residence time of magma in different segments of the plumbing systems. This allows a more nuanced evaluation of the link between observed monitoring signals or eruption styles and the magmatic processes and movement of batches of melts at depth. The approach is illustrated through a study of the compositional zoning recorded in olivine crystals from the 1991–1993 SE-flank eruption products of Mt. Etna (Sicily). The zoning patterns in crystals reveal that the plumbing system of the volcano consisted of at least three different magmatic environments between which magma was transported and mixed in the year or two preceding the start of eruption. Quantification of this history indicates that two main pathways of melt migration and three timescales dominated the dynamics of the system. Combination of this information with the timing of observation of various monitoring signals allows a reconstruction of the dynamic evolution of this section of the plumbing system during the early stages of the 1991–1993 eruption. It is seen, for example, how the migration of melt through the same sections of the plumbing system can cause pre-eruptive triggering, enhance Strombolian activity, and through the ensuing eruption cleanse and flush the plumbing system. Different kinds of mixing occur simultaneously at different sections of the plumbing system on different timescales (a few days up to two years).
    Description: Published
    Description: 11-22
    Description: 1.5. TTC - Sorveglianza dell'attività eruttiva dei vulcani
    Description: 2.3. TTC - Laboratori di chimica e fisica delle rocce
    Description: 3.5. Geologia e storia dei vulcani ed evoluzione dei magmi
    Description: JCR Journal
    Description: reserved
    Keywords: Etna ; plumbing system ; olivine ; zoning ; timescales ; monitoring ; 04. Solid Earth::04.04. Geology::04.04.05. Mineralogy and petrology ; 04. Solid Earth::04.08. Volcanology::04.08.03. Magmas ; 04. Solid Earth::04.08. Volcanology::04.08.05. Volcanic rocks
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 9
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    Stratigraphic evidence for a “pluvial phase” between ca 8200–7100 ka from Renella cave (Central Italy) (2012)
    Elsevier
    Details
    Publication Date: 2022-08-25
    Description: A stratigraphic and chronological study of the upper level of Renella Cave (Apuan Alps, Central Italy) reveals that two episodes of flowstone accumulation bracket a thick clastic layer deposited between ca 8.2 and 7.1 ka. This layer, which represents a period of enhanced cave flooding, is substantially in phase with an interval of depleted oxygen isotope values previously recorded in a stalagmite from nearby Corchia Cave, interpreted to have resulted from an increase in local precipitation. These data confirm that during this period of time the region experienced relatively wetter conditions, including an increase in high-magnitude events capable of invading the higher passages of Renella Cave. The timing of the clastic phase occurred when the Eastern Mediterranean experienced deposition of sapropel layer S1, which is thought to reflect the stagnation of sea water produced largely by enhanced flood activity along the Nile in response to increased monsoon intensity in northern equatorial Africa. Recent estimates suggest that S1 may have lasted from ca 10.8 to ca 6.1 ka cal BP. Combined evidence from Renella and Corchia Cave indicates that the period corresponding to the wettest phase in the Apuan Alps was much shorter than this, and suggests that there is no straightforward connection between increased advection of water vapour from the Atlantic between 8.2 and 7.1 ka, as recorded in the Corchia and Renella records, and monsoon-driven enhancement of Nile discharge and S1 deposition in the eastern Mediterranean.
    Description: Published
    Description: 409-417
    Description: 3.7. Dinamica del clima e dell'oceano
    Description: JCR Journal
    Description: reserved
    Keywords: Speleothems ; Floods ; Paleoclimate ; Holocene ; Renella cave ; Italy ; 03. Hydrosphere::03.01. General::03.01.06. Paleoceanography and paleoclimatology
    Repository Name: Istituto Nazionale di Geofisica e Vulcanologia (INGV)
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  • 10
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    Environmental variability in northeastern Siberia during the last ~13,300 yr inferred from lake diatoms and sediment-geochemical parameters (2012)
    Elsevier
    In:  EPIC3Palaeogeography, Palaeoclimatology, Palaeoecology, Elsevier, 329-33, pp. 22-36
    Details
    Publication Date: 2022-08-12
    Repository Name: EPIC Alfred Wegener Institut
    Type: Article , NonPeerReviewed
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