Electronic Resource
College Park, Md.
:
American Institute of Physics (AIP)
The Journal of Chemical Physics
105 (1996), S. 6141-6146
ISSN:
1089-7690
Source:
AIP Digital Archive
Topics:
Physics
,
Chemistry and Pharmacology
Notes:
Recently the anti-Stokes spectroscopy after strong vibrational excitation via resonant absorption was rediscovered, for the study of population relaxation dynamics. A closer theoretical inspection of this experimental approach reveals that properly chosen polarization conditions allow the study of molecular reorientational motion. Furthermore the sign of a/γ (the invariants of the Raman polarizability tensor) can be determined. Experimental data for chlorinated alkanes will be presented. © 1996 American Institute of Physics.
Type of Medium:
Electronic Resource
URL:
http://dx.doi.org/10.1063/1.472473
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