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  • 1995-1999  (98)
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  • 1
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 81 (1997), S. 5778-5780 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: Antiferromagnetic uranium intermetallic compound UNiGa shows a large reduction of electrical resistivity in conjunction with the metamagnetic transition in fields below 1 T. On the basis of specific heat, Hall effect and thermopower measurements in various fields we suggest that the reason for the giant magnetoresistance is a substantial Fermi surface reconstruction at the transition. © 1997 American Institute of Physics.
    Materialart: Digitale Medien
    Standort Signatur Erwartet Verfügbarkeit
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  • 2
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 79 (1996), S. 6358-6360 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: Magnetization, magnetic susceptibility, electrical resistivity, and specific heat measurements of UNiAl point to antiferromagnetic ordering below 19.3 K, which is confirmed by neutron-diffraction experiments. The enhanced γ value of 167 mJ/mol K2 is reflecting pronounced presence of magnetic fluctuations, which influence also the other electronic properties down to low temperatures. The thermal expansion of UNiAl was measured in the temperature range 1.5–210 K on a single crystal along the a and c axis. Similar to other bulk properties, also the thermal expansion of UNiAl is highly anisotropic. The a axis is monotonously expanding with increasing temperature in the whole temperature range. Along the c axis, the lattice first collapses with increasing temperature up to 35 K. Around this temperature, the thermal expansion coefficient αc changes sign and continuous expansion with further increasing temperature is then observed. The sharp anomaly of α near 19.3 K present in both directions is consistent with the magnetic phase transition. The results are discussed in terms of the presence of anisotropic magnetic fluctuations. © 1996 American Institute of Physics.
    Materialart: Digitale Medien
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  • 3
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: As a result of combined magnetization, specific heat, electrical resistivity, and neutron-scattering studies on single crystals, we present a complex magnetic phase diagram of UNiGa that exhibits several antiferromagnetic (AF) phases below TN=39 K. A relatively low magnetic field (∼1–1.5 T) applied along the c-axis induces metamagnetic transitions from the zero-field AF structures to an uncompensated AF and/or to a ferromagnetic (F) phase. All the magnetic structures are collinear (uranium magnetic moments parallel to the c-axis of the hexagonal structure). They consist of F basal-plane sheets which are coupled along c in various ways. The strongly anisotropic magnetism in UNiGa causes anisotropy of the electrical resistivity. The magnetic phase transitions are reflected in pronounced resistivity anomalies especially for current along the c-axis. The metamagnetic transitions are accompanied by giant magnetoresistance (GMR) effects which can be correlated with respective changes of the magnetic periodicity. This implies an important feature of the mechanism responsible for GMR phenomena in UNiGa. The strong resistance enhancement in the paramagnetic range when approaching TN is connected with AF short-range ordering with propagation along the c-axis. © 1996 American Institute of Physics.
    Materialart: Digitale Medien
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  • 4
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 79 (1996), S. 6408-6410 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: Crystallographic analysis shows that UCuSn does not form in the hexagonal CaIn2 structure as reported previously, but is an ordered ternary compound and forms in an orthorhombic structure (space group: P21cn). Bulk and neutron-diffraction measurements reveal that UCuSn orders antiferromagnetically below 62 K. At 4.2 K, high-field magnetization reveals a complex magnetization process with two metamagnetic transitions. Furthermore, bulk investigations show an additional anomaly at 25 K, but a smooth temperature dependence of various magnetic peaks down to the lowest temperature gives no evidence for a second magnetic transition. Possible scenarios responsible for the drastic changes in the electronic properties around 25 K are discussed. © 1996 American Institute of Physics.
    Materialart: Digitale Medien
    Standort Signatur Erwartet Verfügbarkeit
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  • 5
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 79 (1996), S. 5221-5223 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: Our neutron-powder-diffraction experiment revealed that URhSi crystallizes in the orthorhombic TiNiSi (space group Pnma) structure and orders ferromagnetically at low temperatures with the U magnetic moments of 0.11 μB aligned along the c axis. Anomalies in the temperature dependence of the magnetic susceptibility, specific heat and electrical resistivity indicate that URhSi orders below 9.5 K. The enhanced Cp/T value (extrapolated to 0 K) of 186 mJ/mol K2 can be partially reduced in magnetic fields, which indicates a considerable magnetic contribution even at very low temperatures. The ferromagnetic ground state is documented also by magnetization measurements at low temperatures. The high-field magnetization data obtained on oriented powder reveal a strong magnetocrystalline anisotropy. All the results obtained on polycrystalline samples classify URhSi as an itinerant 5f ferromagnet with very reduced U magnetic moments. © 1996 American Institute of Physics.
    Materialart: Digitale Medien
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  • 6
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: U2Pt2Sn is crystallizing in an ordered version (space group P42/mnm) of the tetragonal U3Si2 type of structure. Clear anomalies in the magnetic susceptibility, specific heat, and electrical resistivity around 15 K indicate that U2Pt2Sn orders antiferromagnetically below this temperature. As expected for an antiferromagnet, the susceptibility and specific heat anomalies are shifted to lower temperatures upon application of external magnetic field. The specific-heat coefficient γ=327 mJ/mol f.u. K2 remains unchanged in fields up to 5 T. The antiferromagnetic ground state of U2Pt2Sn can be concluded also from the metamagnetic transition around 22 T in the magnetization at 4.2 K and from magnetic reflections in the neutron-diffraction pattern at low temperatures. © 1996 American Institute of Physics.
    Materialart: Digitale Medien
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  • 7
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 85 (1999), S. 4554-4555 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: We report on electrical resistivity measurements for an UNi2Si2 single crystal in the temperature range 4.2–140 K and magnetic fields up to 8.4 T parallel to the c axis. The anomalies in the temperature and field dependencies of the resistivity are associated with magnetic phase transitions and allow one to complete the B–T magnetic phase diagram. The relationship between the electrical resistivity and the periodicity of particular magnetic phases is discussed in light of magnetoresistance behavior in other antiferromagnetic U compounds. © 1999 American Institute of Physics.
    Materialart: Digitale Medien
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  • 8
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 81 (1997), S. 4221-4223 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: We report on magnetic, transport, and cohesive properties of Er(Co1−xSix)2 compounds in varying external conditions (T,H,p). The localized Er 4f magnetic moments in ErCo2 order ferromagnetically below TC=33 K. The Co 3d band states form no moment above TC, but below TC the majority and minority 3d sub-bands split due to strong 4f−3d exchange interaction. Consequently, Co moments of ∼1 μB appear coupled antiparallel to the Er moments. This is accompanied by a ∼50% resistivity drop and an abrupt lattice expansion. The sharp magnetization, resistivity, and volume anomalies in the critical temperature region indicate a first order magnetic phase transition. Detailed comparative studies reveal that the onset of Co magnetizm appears at T0∼(TC−1) K. Si substitution for Co enhances both, TC (up to 66 K for x=0.1) and ΔT=TC−T0, but the lattice parameter remains unchanged. In opposite, both the magnetovolume and resistivity anomaly at T0 become reduced. Pressure effect on TC(T0) is large and negative, ∂ ln TC/∂p∼−28 Mbar−1 for all x≤0.1. Also the resistivity drop at T0 and the magnetovolume effect (ωs=3 ΔL/L=4.2×10−3 in ErCo2) below T0 become reduced with increasing pressure. The latter is reflecting reduction of the Co moment gained below T0. © 1997 American Institute of Physics.
    Materialart: Digitale Medien
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  • 9
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 83 (1998), S. 6964-6966 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: We report on a comparative study of the effects of Si doping and of external pressure on magnetism and related phenomena in Nd(Co1−xSix)2 and Ho(Co1−xSix)2 compounds. The lattice volume in the Ho system is almost composition invariable for x up to 0.1, whereas an increase of (approximate)6% is observed in the Nd system. Si substitutions for Co cause a dramatic increase of TC in the Ho system for x≤0.075 and a gradual reduction of TC in Nd analogs, whereas the Co moment becomes suppressed for x〉0.05 in both cases. Negative pressure effects both on TC and the Co magnetic moment, although quantitatively different, are found in both systems. Expected changes of electronic structure and their influence on the hierarchy of exchange interactions and formation of the Co moment are discussed. © 1998 American Institute of Physics.
    Materialart: Digitale Medien
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  • 10
    Digitale Medien
    Digitale Medien
    [S.l.] : American Institute of Physics (AIP)
    Journal of Applied Physics 83 (1998), S. 6435-6437 
    ISSN: 1089-7550
    Quelle: AIP Digital Archive
    Thema: Physik
    Notizen: Electrical resistivity and ac magnetic susceptibility studies of the 5f-metamagnet UCoAl reveal the presence of strong spin fluctuation effects for temperatures below 30 K and magnetic fields below the critical metamagnetic field μ0Hc(approximate)1 T, where a non-Fermi liquid term ∼T3/2 is prominent in the electrical resistivity. A step-wise increase of the residual resistivity and an increasingly prominent Fermi liquid T2 term of the resistivity is observed as the field is increased though the metamagnetic transition. © 1998 American Institute of Physics.
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