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  • 1
    Publication Date: 2012-03-15
    Description: Retrievals of aerosol optical depth (AOD) and related parameters from satellite measurements typically involve prescribed models of aerosol size and composition, and are therefore dependent on how well these models are able to represent the radiative behavior of real aerosols. This study uses aerosol volume size distributions retrieved from Sun-photometer measurements at 11 Aerosol Robotic Network (AERONET) island sites, spread throughout the world's oceans, as a basis to define such a model for pure (unpolluted) maritime aerosol. Volume size distributions are observed to be bimodal and approximately lognormal, although the coarse mode is skewed with a long tail on the low-radius end. The relationship of AOD and size distribution parameters to meteorological conditions is also examined. As wind speed increases, so do coarse-mode volume and radius. The AOD and Ångström exponent show linear relationships with wind speed, although with considerable scatter. Links between aerosol properties and near-surface relative humidity, columnar water vapor, and sea surface temperature are also explored. A recommended bimodal maritime model, which is able to reconstruct the AERONET AOD with accuracy of order 0.01–0.02, is presented for use in aerosol remote sensing applications. This accuracy holds at most sites and for wavelengths between 340 nm and 1020 nm. Calculated lidar ratios are also provided, and are in the range of other studies, although differ more strongly from those currently used in Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) processing.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 2
    Publication Date: 2012-04-05
    Description: Large fine mode–dominated aerosols (submicron radius) in size distributions retrieved from the Aerosol Robotic Network (AERONET) have been observed after fog or low-altitude cloud dissipation events. These column-integrated size distributions have been obtained at several sites in many regions of the world, typically after evaporation of low-altitude cloud such as stratocumulus or fog. Retrievals with cloud-processed aerosol are sometimes bimodal in the accumulation mode with the larger-size mode often ∼0.4–0.5 μm radius (volume distribution); the smaller mode, typically ∼0.12 to ∼0.20 μm, may be interstitial aerosol that were not modified by incorporation in droplets and/or aerosol that are less hygroscopic in nature. Bimodal accumulation mode size distributions have often been observed from in situ measurements of aerosols that have interacted with clouds, and AERONET size distribution retrievals made after dissipation of cloud or fog are in good agreement with particle sizes measured by in situ techniques for cloud-processed aerosols. Aerosols of this type and large size range (in lower concentrations) may also be formed by cloud processing in partly cloudy conditions and may contribute to the “shoulder” of larger-size particles in the accumulation mode retrievals, especially in regions where sulfate and other soluble aerosol are a significant component of the total aerosol composition. Observed trends of increasing aerosol optical depth (AOD) as fine mode radius increased suggests higher AOD in the near-cloud environment and higher overall AOD than typically obtained from remote sensing owing to bias toward sampling at low cloud fraction.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 3
    Publication Date: 2016-01-17
    Description: Dominant aerosol types were classified using level 2 inversion products for the Anmyon Aerosol Robotic Network (AERONET) site in Korea for the period 1999–2007. The aerosol types were mineral dust (MD), MD mixed with carbon, and black carbon mixed coarse particles (BCCP) for coarse mode aerosols, black carbon (BC), organic carbon (OC), and secondary inorganic ions (SII) for fine mode aerosols, and mixed particles between. The classification was carried out using a clustering method based on parameters, including single scattering albedo (SSA), absorption Angstrom exponent (AAE), and fine mode volume fraction (FMVF). Among the seven aerosol types, MD was distinct, with the highest AAE and a very low FMVF and SII with the highest SSA and FMVF. BCCP was introduced to designate coarse particles mixed with BC, of which the AAE was lower than 1, despite a low FMVF. In addition to a large difference in AAE between BC and OC, the SSA of OC was larger than that of BC, indicating the effects of the white smoke produced from the smoldering phase of biomass burning. Monthly variations of the aerosol types were well interpreted by meteorology and emissions, and coincided with those in the previous studies. Applying our results to well-characterized global AERONET sites, we confirmed that the aerosol types at Anmyon were valid at other sites. However, the results also showed that the mean properties for aerosol types were influenced by the specific aerosols prevalent at the study sites.
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    Topics: Geosciences , Physics
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  • 4
    Publication Date: 2012-09-06
    Description: Partitioning of mineral dust, pollution, smoke, and mixtures using remote sensing techniques can help improve accuracy of satellite retrievals and assessments of the aerosol radiative impact on climate. Spectral aerosol optical depth (τ) and single scattering albedo (ωo) from Aerosol Robotic Network (AERONET) measurements are used to form absorption (i.e., ωo and absorption Ångström exponent (αabs)) and size (i.e., extinction Ångström exponent (αext) and fine mode fraction of τ) relationships to infer dominant aerosol types. Using the long-term AERONET data set (1999–2010), 19 sites are grouped by aerosol type based on known source regions to (1) determine the average ωo and αabs at each site (expanding upon previous work), (2) perform a sensitivity study on αabs by varying the spectral ωo, and (3) test the ability of each absorption and size relationship to distinguish aerosol types. The spectral ωo averages indicate slightly more aerosol absorption (i.e., a 0.0 〈 δωo ≤ 0.02 decrease) than in previous work, and optical mixtures of pollution and smoke with dust show stronger absorption than dust alone. Frequency distributions of αabs show significant overlap among aerosol type categories, and at least 10% of the αabs retrievals in each category are below 1.0. Perturbing the spectral ωo by ±0.03 induces significant αabs changes from the unperturbed value by at least ∼±0.6 for Dust, ∼±0.2 for Mixed, and ∼±0.1 for Urban/Industrial and Biomass Burning. The ωo440nm and αext440–870nm relationship shows the best separation among aerosol type clusters, providing a simple technique for determining aerosol type from surface- and future space-based instrumentation.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 5
    Publication Date: 2012-05-02
    Description: A synergy of satellite and ground-based radiometric observations, along with chemical transport modeling, was used for the assessment of the influence of drought monsoon conditions of 2002 and prolonged dry pre-monsoon period of 2003 on aerosol properties over south Asia, with emphasis over northern India. Reanalysis data are also examined for studying the dry anomalous period from the climatological mean, that show prevalence of westerlies under anticyclonic circulation and subsidence favoring the accumulation of aerosols. TRMM observations over south Asia indicate significant rainfall deficit over northwestern India in July 2002 and May–June 2003. Subsequently, the anomalous and prolonged dry conditions favored heavy aerosol buildup as indicated by strong positive anomalies (20–80%) of MODIS aerosol optical depth (AOD) as well as significant increase in TOMS aerosol index (AI) during July 2002 and May–June 2003 compared to the long-term monthly means. The largest increase in aerosol loading is observed over northern India, encompassing the Indo-Gangetic Plains (IGP) that is in the downwind region of dust outflow from the Thar Desert and long-range transport from Arabia and Middle East. Ground-based sunphotometer observations at Delhi and Kanpur also show enhanced presence of desert-dust aerosols during July 2002 and May–June 2003, characterized by large AOD and significantly low Angstrom Exponent. In addition, modifications in columnar aerosol size distribution toward larger coarse-mode fraction and higher single scattering albedo at longer wavelengths were observed, thus supporting the observation of enhanced dust influx. SPRINTARS model simulations also show the enhanced dust loading over northern India during the studied months, which is in general agreement with the satellite and ground-based observations.
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    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 6
    Publication Date: 2014-05-07
    Description: Single scattering albedo (SSA) retrievals obtained with CIMEL sun-sky radiometers from the AERONET aerosol monitoring network were used to make comparisons with simultaneous in-situ sampling from aircraft profiles carried out by the NASA Langley Aerosol Group Experiment (LARGE) team in the summer of 2011 during the coincident DRAGON-MD (Distributed Regional Aerosol Gridded Observational Network-Maryland) and DISCOVER-AQ (Deriving Information on Surface conditions from Column and Vertically Resolved Observations Relevant to Air Quality) experiments. The single scattering albedos (interpolated to 550 nm) derived from AERONET measurements for aerosol optical depth (AOD) at 440 nm ≥ 0.4 (mean SSA: 0.979) were on average 0.011 lower than the values derived from the LARGE profile measurements (mean SSA: 0.99). The maximum difference observed was 0.023 with all the observed differences within the combined uncertainty for the stated SSA accuracy (0.03 for AERONET; 0.02 for LARGE). Single scattering albedo averages were also analyzed for lower aerosol loading conditions (AOD ≥ 0.2) and a dependence on aerosol optical depth was noted with significantly lower single scattering albedos observed for lower AOD in both AERONET and LARGE datasets. Various explanations for the SSA trend were explored based on other retrieval products including volume median radius and imaginary refractive index as well as column water vapor measurements. Additionally, these SSA trends with AOD were evaluated for one of the DRAGON-MD study sites, Goddard Space Flight Center, and two other Mid-Atlantic AERONET sites over the long-term record dating to 1999.
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    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 7
    Publication Date: 2014-04-01
    Description: As part of TIGERZ campaign, latitudinal variation of aerosol optical properties were analysed over Indo-Gangetic Plains (IGP) to central Himalayas during pre-monsoon of 2008 and 2009. Measurements of aerosol optical depth (AOD) were performed using AERONET Sunphotometer at four sites with different aerosol environments. The AOD increases from Nainital located in central Himalayas to Kanpur located in IGP region. Further, aerosol size varies spatially with dominance of coarse mode aerosols at Kanpur compared to fine mode aerosols dominated at Nainital. Spectral variation of single scattering albedo suggests that during pre-monsoon, dust is the dominant species in the IGP with exception of Pantnagar, where absorbing aerosols are dominant. The optical properties of aerosols are calculated and shortwave clear sky aerosol radiative forcing (ARF) is estimated. An insignificant difference is found in columnar ARF and columnar heating rate (HR) when vertical profiles of aerosols are included in radiative transfer models. Over Nainital, average ARF is estimated to be -7.61, -45.75 and 38.14 Wm -2 at top of atmosphere (TOA), surface (SUR) and in the atmosphere (ATM), respectively. Average ARF is less negative at Kanpur compared to Pantnagar and Bareilly with values -17.63, -73.06, and 55.43 Wm -2 at TOA, SUR, and ATM, respectively. ARF shows positive gradient from the highlands to the IGP sites; larger TOA and SUR cooling were observed at the three sites compared to the highland site. This translates into large columnar HR with estimated average values as 1.07, 1.41, 1.58, and 1.56 Kday -1 for Nainital, Pantnagar, Bareilly and Kanpur, respectively.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
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  • 8
    Publication Date: 2012-02-15
    Description: The Sea-viewing Wide Field-of-view Sensor (SeaWiFS) provides a well-calibrated 13-year (1997–2010) record of top-of-atmosphere radiance, suitable for use in retrieval of atmospheric aerosol optical depth (AOD). This paper presents and validates a SeaWiFS Ocean Aerosol Retrieval (SOAR) algorithm, which retrieves the AOD at 550 nm and the partition of aerosol particle volume between fine and coarse modes. The algorithm has been applied over water to the whole SeaWiFS record. The data set includes quality flags to identify those retrievals suitable for quantitative use. SOAR has been validated against Aerosol Robotic Network (AERONET) and Maritime Aerosol Network (MAN) data and found to compare well (correlation 0.86 at 550 nm and 0.88 at 870 nm for AERONET, and 0.87 at 550 nm and 0.85 at 870 nm for MAN, using recommended quality control settings). These comparisons are used to identify the typical level of uncertainty on the AOD, estimated as 0.03 + 15% at 550 nm and 0.03 + 10% at 870 nm. The data set also includes the Ångström exponent, although as expected this is noisy for low aerosol loadings (correlation 0.50; 0.78 for points where the AOD at 550 nm is 0.3 or more). Retrieved AOD is compared with colocated observations from other satellite sensors; regional and seasonal patterns are found to be common between all data sets, and differences generally linked to factors such as cloud screening and retrieval assumptions.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 9
    Publication Date: 2014-08-02
    Description: Several heavy atmospheric haze pollution episodes occurred over eastern and northern China during January of 2013. The pollution covered more than 100 km 2 and caused serious impacts on environmental quality, human health, and transportation. In this study, we characterize aerosol microphysical, optical and radiative characteristics using a combination of ground-based sun/sky radiometer retrievals and a radiative transfer model. Our results show that about half of the total number days of daily PM 2.5 and PM 10 concentrations are larger than 100 µg/m 3 , with maxima of 462 and 433 µg/m 3 , respectively, during the haze events. Fine mode (PM 2.5 ) particles dominated the aerosol size during the episodes. The volume size distribution and median radius of fine-mode particles generally increase as aerosol optical depth at 440 nm (AOD 440 ) increases. The median effective radius of fine-mode particles increases from 0.15 µm at low AOD value (AOD 440  ~ 0.3) to a radius of 0.25-0.30 µm at high AOD value (AOD 440  ≥ 1.0). The daily mean single scattering albedo (SSA), imaginary part of refractive index (RI), and asymmetry factor (ASY) display pronounced spectral behaviors. The overall mean SSA 440 and SSA 675 are 0.892 and 0.905, respectively. The corresponding RI 440 and RI 675 are 0.016 and 0.011, respectively. This indicates that a significant amount of absorption occurred under the haze event in Beijing during January 2013. Approximately half of the incident solar radiation energy went into heating the atmosphere as a result of strong aerosol loading and absorption. The daily averaged heating rate in the haze particle layer (0–3.2 km) varies from 0.12 to 0.81 K/day in Beijing, which might exert profound impact on the atmospheric thermodynamic and dynamical structures and cloud development, which should be further studied.
    Print ISSN: 0148-0227
    Topics: Geosciences , Physics
    Published by Wiley on behalf of American Geophysical Union (AGU).
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  • 10
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    American Association for the Advancement of Science (AAAS)
    Publication Date: 1997-06-20
    Description: 〈br /〉〈span class="detail_caption"〉Notes: 〈/span〉Mims, F M 3rd -- Holben, B N -- Eck, T F -- Montgomery, B C -- Grant, W B -- New York, N.Y. -- Science. 1997 Jun 20;276(5320):1774-5.〈br /〉〈span class="detail_caption"〉Record origin:〈/span〉 〈a href="http://www.ncbi.nlm.nih.gov/pubmed/9206832" target="_blank"〉PubMed〈/a〉
    Keywords: Aerosols ; Brazil ; Fires ; Humans ; Infection/epidemiology/*etiology ; Photosynthesis ; Respiratory Tract Diseases/epidemiology/*etiology ; Smoke/*adverse effects ; Sunlight ; *Ultraviolet Rays
    Print ISSN: 0036-8075
    Electronic ISSN: 1095-9203
    Topics: Biology , Chemistry and Pharmacology , Computer Science , Medicine , Natural Sciences in General , Physics
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