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  • 1
    Electronic Resource
    Electronic Resource
    The ozone sensitized oxidative conversion of methane to methanol and ethane to ethanol (1992)
    Springer
    Catalysis letters 16 (1992), S. 217-221 
    Details
    ISSN: 1572-879X
    Keywords: Methane ; ethane ; methanol ; ethanol ; ozone ; oxygen atom ; oxidation ; sensitization
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology
    Notes: Abstract The reaction of O2, O3, and CH4 or C2H6 of 7.76, 0.24 and 92% of the hydrocarbon respectively (residence time of 8.8 min) at 1 atm, and 400 °C for CH4 and 300 °C for C2H6 gave CO, CO2, H2O, CH2O and CH3OH from CH4 and in addition CH4, C2H4, CH3CHO and C2H5OH from C2H6. No reaction occurred when O3 was absent indicating that the partial oxidation was sensitized (initiated) by the oxygen atoms formed by the decomposition of ozone.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF00764374
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    Paper (German National Licenses)
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  • 2
    Electronic Resource
    Electronic Resource
    Light paraffin oxidative conversion in a silent electric discharge (1993)
    Springer
    Plasma chemistry and plasma processing 13 (1993), S. 479-488 
    Details
    ISSN: 1572-8986
    Keywords: Silent discharge ; oxidation of light paraffins ; experimental ; methanol ; ethanol ; formaldehyde ; acetaldehyde
    Source: Springer Online Journal Archives 1860-2000
    Topics: Chemistry and Pharmacology , Mechanical Engineering, Materials Science, Production Engineering, Mining and Metallurgy, Traffic Engineering, Precision Mechanics , Technology
    Notes: Abstract Methane, ethane, and their mixtures with oxygen have been passed through the silent electric discharge at various operating conditions Beside.carbon oxides and water, formaldehyde and methane, and acetaldehyde and ethanol from ethane were the other major products. The effect of temperature, pressure, discharge voltage, contact time, and oxygen concentration have been examined. The rate of oxygen consumption is almost independent of oxygen concentration and depends mainly on the discharge voltage. The selectivities of methanol formation from methane and ethanol/formation from ethane were 20 and 15%, respectively.
    Type of Medium: Electronic Resource
    URL: http://dx.doi.org/10.1007/BF01465877
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    Paper (German National Licenses)
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