ALBERT

Description: This study attempts a new identification of mechanisms of secondary ice production (SIP) based on the observation of small faceted ice crystals (hexagonal plates or columns) with typical sizes smaller than 100 µm. Due to their young age, such small ice crystals can be used as tracers for identifying the conditions for SIP. Observations reported here were conducted in oceanic tropical mesoscale convective systems (MCSs) and midlatitude frontal clouds in the temperature range from 0 to −15 ∘C and heavily seeded by aged ice particles. It was found that in both MCSs and frontal clouds, SIP was observed right above the melting layer and extended to higher altitudes with colder temperatures. The roles of six possible mechanisms to generate the SIP particles are assessed using additional observations. In most observed SIP cases, small secondary ice particles spatially correlated with liquid-phase, vertical updrafts and aged rimed ice particles. However, in many cases, neither graupel nor liquid drops were observed in the SIP regions, and therefore, the conditions for an active Hallett–Mossop process were not met. In many cases, large concentrations of small pristine ice particles were observed right above the melting layer, starting at temperatures as warm as −0.5 ∘C. It is proposed that the initiation of SIP above the melting layer is stimulated by the recirculation of large liquid drops through the melting layer with convective turbulent updrafts. After re-entering a supercooled environment above the melting layer, they impact with aged ice, freeze, and shatter. The size of the splinters generated during SIP was estimated as 10 µm or less. A principal conclusion of this work is that only the freezing-drop-shattering mechanism could be clearly supported by the airborne in situ observations.

Description: This study attempts identification of mechanisms of secondary ice production (SIP) based on the observation of small faceted ice crystals (hexagonal plates or columns) with characteristic sizes smaller than 100 μm. Due to their young age, such small ice crystals can be used as tracers for identifying the conditions for SIP. Observations reported here were conducted in oceanic tropical mesoscale convective systems (MCS) and mid-latitude frontal clouds in the temperature range from 0 °C to −15 °C heavily seeded by aged ice particles. It was found that both in MCSs and frontal clouds, SIP was observed right above the melting layer and extended to the higher altitudes with colder temperatures. It is proposed that the initiation of SIP above the melting layer is related to the circulation of liquid drops through the melting layer. Liquid drops formed via melting ice particles are advected by the convective updrafts above the melting layer, where they impact with aged ice, freeze and shatter. The ice splinters generated by shattering initiate the chain reaction of SIP. The size of the splinters generated during SIP were estimated as 10 μm or less. In most SIP cases, small secondary ice particles spatially correlated with liquid phase, vertical updrafts and aged rimed ice particles. However, in many cases neither graupel nor liquid drops were observed in the SIP regions, and therefore, the conditions for an active Hallett-Mossop process were not met. A principal conclusion of this work is that the freezing drop shattering mechanism is alone among established SIP mechanisms is plausibly accounting for the measured ice concentrations in the observed conditions. No other SIP mechanisms could be confidently identified from the airborne in-situ observations.

Description: Stratospheric water vapour (SWV) is a climatically important atmospheric constituent due to its impacts on the radiation budget and atmospheric chemical composition. Despite the important role of SWV in the climate system, the processes controlling the distribution and variation in water vapour in the upper troposphere and lower stratosphere (UTLS) are not well understood. In order to better understand the mechanism of transport of water vapour through the tropopause, this study uses the high-resolution Global Environmental Multiscale model of the Environment and Climate Change Canada to simulate a lower stratosphere moistening event over North America. Satellite remote sensing and aircraft in situ observations are used to evaluate the quality of model simulation. The main focus of this study is to evaluate the processes that influence the lower stratosphere water vapour budget, particularly the direct water vapour transport and the moistening due to the ice sublimation. In the high-resolution simulations with horizontal grid spacing of less than 2.5 km, it is found that the main contribution to lower stratospheric moistening is the upward transport caused by the breaking of gravity waves. In contrast, for the lower-resolution simulation with horizontal grid spacing of 10 km, the lower stratospheric moistening is dominated by the sublimation of ice. In comparison with the aircraft in situ observations, the high-resolution simulations predict the water vapour content in the UTLS well, while the lower-resolution simulation overestimates the water vapour content. This overestimation is associated with the overly abundant ice in the UTLS along with a sublimation rate that is too high in the lower stratosphere. The results of this study affirm the strong influence of overshooting convection on the lower stratospheric water vapour and highlight the importance of both dynamics and microphysics in simulating the water vapour distribution in the UTLS region.